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Bilayers formed of two species of amphiphile of different chain lengths may segregate into thinner and thicker domains composed predominantly of the respective species. Using a coarse-grained mean-field model, we investigate how mixing oil…

软凝聚态物质 · 物理学 2014-06-13 M. J. Greenall , C. M. Marques

Extensive microscopic molecular dynamics simulations have been performed to study the effects of short-chain alcohols, methanol and ethanol, on two different fully hydrated lipid bilayer systems in the fluid phase at 323 K. It is found that…

软凝聚态物质 · 物理学 2007-05-23 Michael Patra , Emppu Salonen , Emma Terama , Roland Faller , Bryan W. Lee , Juha Holopainen , Mikko Karttunen

Hypothesis. Isoniazid is one of the primary drugs used in tuberculosis treatment. Isoniazid encapsulation in liposomal vesicles can improve drug therapeutic index and minimize toxic and side effects. In this work, we consider mixtures of…

Electrochemical devices such as solid oxide fuel cells (SOFC) may greatly benefit from the implementation of nanoengineered thin-film multifunctional layers providing, alongside enhanced electrochemical activity, improved mechanical, and…

Molecular adhesion promoters are a central component of modern coating systems for the corrosion protection of structural materials. They are interface active and form ultrathin corrosion inhibiting and adhesion-promoting layers. Here we…

材料科学 · 物理学 2022-01-05 Dominik Dworschak , Carina Brunnhofer , Markus Valtiner

Two-dimensional (2D) crystals' edge structures not only influence their overall properties but also dictate their formation due to edge-mediated synthesis and etching processes. Edges must be carefully examined because they often display…

介观与纳米尺度物理 · 物理学 2022-08-03 Sol Lee , Yangjin Lee , Li Ping Ding , Kihyun Lee , Feng Ding , Kwanpyo Kim

Bridging the gap between atomistic detail and continuum mechanics is a central challenge in modeling biological membranes, particularly for mesoscopic phenomena spanning large length and time scales. In this work, we introduce a new,…

软凝聚态物质 · 物理学 2026-03-02 Pietro Sillano , Siewert-Jan Marrink , Timon Idema

We use a coarse-grained molecular model to study the self-assembly process of complexes of cationic and neutral lipids with DNA molecules ("lipoplexes") - a promising nonviral carrier of DNA for gene therapy. We identify the resulting…

软凝聚态物质 · 物理学 2011-05-31 Oded Farago , Niels Grønbech-Jensen

The presence and the properties of lipid bilayer nanometer-scale domains might be important for understanding the membranes of living cells. We used molecular dynamics (MD) simulations to investigate perturbations of a small patch of…

软凝聚态物质 · 物理学 2011-06-01 Frederick A. Heberle , David G. Ackerman , Gerald W. Feigenson

In a recent publication, we have highlighted the potential of phosphonic acid terminated PEG oligomers to functionalize strong UV absorption cerium oxide nanoparticles[1], which yield suspensions that are stable in aqueous or organic…

材料科学 · 物理学 2013-05-07 L. Qi , J. Fresnais , P. Muller , O. Theodoly , J. -F. Berret , J. -P. Chapel

Soluble alpha-amylases play an important role in the catabolism of polysaccharides. In this work, we show that the enzyme can interact with the lipid membrane and further alter its mechanical properties. Vesicle fluctuation spectroscopy is…

We investigate the finite-temperature phase diagram of polar molecules confined in a quasi-two-dimensional geometry by a harmonic potential along the polarization axis. We employ Quantum Monte Carlo simulations to explore the strongly…

量子气体 · 物理学 2026-05-19 Vinicius Zampronio , Matteo Ciardi , Fabio Cinti

We consider a theoretical model for a binary mixture of colloidal particles and spherical emulsion droplets. The hard sphere colloids interact via additional short-ranged attraction and long-ranged repulsion. The droplet-colloid interaction…

软凝聚态物质 · 物理学 2012-01-11 Ingmar Schwarz , Andrea Fortini , Claudia Simone Wagner , Alexander Wittemann , Matthias Schmidt

Motivated by the experimental study of Tayebi et al. [Nature Mater. 11, 1074 (2012)] on phase separation of stacked multi-component lipid bilayers, we propose a model composed of stacked two-dimensional Ising spins. We study both its static…

软凝聚态物质 · 物理学 2015-12-14 T. Hoshino , S. Komura , D. Andelman

We study the indentation of a free-standing lipid membrane suspended over a nanopore on a hydrophobic substrate by means of molecular dynamics simulations. We find that in the course of indentation, the membrane bends at the point of…

软凝聚态物质 · 物理学 2011-08-26 Chen-Hsi Huang , Pai-Yi Hsiao , Fan-Gang Tseng , Shih-Kang Fan , Chien-Chung Fu , Rong-Long Pan

Recent experiments with amyloid-beta (Abeta) peptide suggest that formation of toxic oligomers may be an important contribution to the onset of Alzheimer's disease. The toxicity of Abeta oligomers depends on their structure, which is…

生物物理 · 物理学 2009-11-10 B. Urbanc , L. Cruz , F. Ding , D. Sammond , S. Khare , S. V. Buldyrev , H. E. Stanley , N. V. Dokholyan

Phospholipid bilayers are a major component of the cell membrane that is in contact with physiological electrolyte solutions including salt ions. The effect of salt on the phospholipid bilayer mechanics is an active research area due to its…

软凝聚态物质 · 物理学 2023-10-16 Yaoqi Huang , Vineeth Chandran Suja , Layaa Amirthalingam , Gerald G. Fuller

The folding of the cholesterol trapping apolipoprotein A1 in aqueous solution at increasing ionic strength is studied using atomically detailed molecular dynamics simulations. We calculate various structural properties to characterize the…

软凝聚态物质 · 物理学 2014-06-12 M. A. Balderas Altamirano , A. Gama Goicochea , E. Pérez

Pore-forming toxins (PFT) are cytolytic proteins belonging to the molecular warfare apparatus of living organisms. The assembly of the functional transmembrane pore requires several intermediate steps ranging from a water-soluble monomeric…

A mesoscopic coarse-grain model for computationally-efficient simulations of biomembranes is presented. It combines molecular dynamics simulations for the lipids, modeled as elastic chains of beads, with multiparticle collision dynamics for…

软凝聚态物质 · 物理学 2015-06-04 Mu-Jie Huang , Raymond Kapral , Alexander S. Mikhailov , Hsuan-Yi Chen