相关论文: Electron Doping a Kagome Spin Liquid

New physics can emerge in magnetic materials where quantum fluctuations are enhanced due to reduced dimensionality and strong frustration. One long sought example is the resonating-valence-bond (RVB) state, where atomic magnetic moments are…

We employ real-space variational quantum Monte Carlo methods with resonating valence bond many-body wave functions to investigate electron correlation effects in the Kagome system $Zn_xCu_{4-x}O_6$. Using three trial wave functions of the…

We investigate the lattice dynamics in the spin-1/2 frustrated kagome compound herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$ by a combination of infrared spectroscopy measurements and ab initio density functional theory calculations, and provide…

The spin-1/2 kagome lattice antiferromagnet herbertsmithite, ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, is a candidate material for a quantum spin liquid ground state. We show that the magnetic response of this material displays an unusual scaling…

Arguably the most favorable situation for spins to enter the long-sought quantum spin liquid (QSL) state is when they sit on a kagome lattice. No consensus has been reached in theory regarding the true ground state of this promising…

Iridates are characterized by a fascinating interplay of spin-orbit and electron-electron interactions. The honeycomb-lattice materials A2IrO3 (A=Na,Li) have been proposed to realize pseudospin-1/2 Mott insulating states with strongly…

We report thermodynamic measurements of the S=1/2 kagome lattice antiferromagnet ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$, a promising candidate system with a spin-liquid ground state. Using single crystal samples, the magnetic susceptibility both…

We report magnetization, electron spin resonance (ESR), and muon spin relaxation ($\mu $SR) measurements on single crystals of the $S=1/2$ (Cu$% ^{+2}$) kagom\'{e} compound Cu(1,3-benzendicarboxylate). The $\mu $SR is carried to…

Based on experimental data and our theoretical analysis, we provide a strategy for unambiguous establishing of gapless quantum spin liquid state (QSL) in herbertsmithite and other materials. To clarify the nature of QSL, we recommend…

Despite tremendous investigations, a quantum spin liquid state realized in spin-1/2 kagome Heisenberg antiferromagnet remains largely elusive. In herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$, a quantum spin liquid candidate on the perfect kagome…

Electronic structure calculations indicate that the Sr2FeSbO6 double perovskite has a flat-band set just above the Fermi level that includes contributions from ordinary sub-bands with weak kinetic electron hopping plus a flat sub-band that…

We present a theory of the dynamic magnetic susceptibility of quantum spin liquid. The obtained results are in good agreement with experimental facts collected on herbertsmithite ZnCu3(OH)6Cl2 and on heavy-fermion metals, and allow us to…

Very recently, a 3$d$ based honeycomb cobaltate Na$_2$Co$_2$TeO$_6$ has garnered tremendous attention due to the proposed proximity to the Kitaev spin-liquid state as its 4$d$/5$d$ counterparts. Here, we use Zn to substitute Co in a broad…

We report the magnetic properties in the Co- and Zn-doped spin-1/2 honeycomb-lattice compound In$_3$Cu$_2$VO$_9$. The magnetic susceptibility and specific heat experiments show no long-range ordering down to 2 K in In$_3$Cu$_2$VO$_9$. In…

The metal-organic-framework (MOF) compound Cu$_3$(HOTP)$_2$, a.k.a. Cu$_3$(HHTP)$_2$, is a small-gap semiconductor containing a kagome lattice of antiferromagnetically coupled $S$=1/2 Cu$^\mathrm{II}$ spins with intra-layer nearest-neighbor…

The Dirac spin liquid was proposed to be the ground state of the spin-1/2 Kagome antiferromagnets. In a magnetic field $B$, we show that the state with Fermi pocket is unstable to the Landau level (LL) state. The LL state breaks the spin…

The search for quantum spin liquid (QSL) materials has attracted significant attention in the field of condensed matter physics in recent years, but until now only a handful of them are considered as candidates hosting QSL ground state.…

Doping carriers into a correlated quantum ground state offers a promising route to generate new quantum states. The recent advent of moir\'{e} superlattices provided a versatile platform with great tunability to explore doping physics in…

Strongly correlated Fermi systems are among the most intriguing and fundamental systems in physics, whose realization in some compounds is still to be discovered. We show that herbertsmithite ZnCu_3(OH)_6Cl_2 can be viewed as a strongly…

Nearest-neighbor interacting S = 1/2 spins on the ideal Kagom\'{e} lattice are predicted to form a variety of novel quantum entangled states, including quantum spin-liquid (SL) and valence bond solid (VBS) phases. In real materials, the…