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Black phosphorus nitrogen (BP-N) is an attractive high-energy-density material. However, high-pressure synthesized BP-N will decompose at low-pressure and cannot be quenched to ambient conditions. Finding a method to stabilize it at 0 GPa…

材料科学 · 物理学 2025-01-03 Guo Chen , Chengfeng Zhang , Yuanqin Zhu , Bingqing cao , Jie Zhang , Xianlong Wang

We use molecular dynamics simulations to study a semidilute, unentangled polymer solution containing well dispersed, weakly attractive nanoparticles (NP) of size ($\sigma_N$) smaller than the polymer radius of gyration $R_g$. We find that…

软凝聚态物质 · 物理学 2018-09-18 Valerio Sorichetti , Virginie Hugouvieux , Walter Kob

Understanding the behavior of molecular systems under pressure is a fundamental problem in condensed matter physics. In the case of nitrogen, the determination of the phase diagram and in particular of the melting line, are largely open…

材料科学 · 物理学 2010-07-27 Davide Donadio , Leonardo Spanu , Ivan Duchemin , Francois Gygi , Giulia Galli

Diatomic nitrogen is an archetypal molecular system known for its exceptional stability and complex behavior at high pressures and temperatures, including rich solid polymorphism, formation of energetic states, and an insulator-to-metal…

Using molecular dynamics simulations we study the static and dynamic properties of spherical nanoparticles (NPs) embedded in a disordered and polydisperse polymer network. Purely repulsive (RNP) as well as weakly attractive (ANP) polymer-NP…

软凝聚态物质 · 物理学 2023-02-15 Valerio Sorichetti , Virginie Hugouvieux , Walter Kob

Nitrogen oxides are textbook class of molecular compounds, with extensive industrial applications. Nitrogen and oxygen are also among the most abundant elements in the universe. We explore the N-O system at 0 K and up to 500 GPa though ab…

材料科学 · 物理学 2015-06-30 Dongxu Li , Artem R. Oganov , Xiao Dong , Xiang-Feng Zhou , Qiang Zhu , Guangrui Qian , Huafeng Dong

Polymer-grafted nanoparticles (PGNPs) can provide property profiles than cannot be obtained individually by polymers or nanoparticles (NPs). Here, we have studied the mixing--demixing transition of symmetric copolymer melts of…

软凝聚态物质 · 物理学 2020-01-23 Peter Yatsyshin , Nikolaos G. Fytas , Panagiotis E. Theodorakis

The 12%-S doped FeSe system has a high Tc of 30 K at a pressure of 3.0 GPa. We have successfully investigated its microscopic properties for the first time via $^{77}$Se-NMR measurements under pressure. The antiferromagnetic (AFM)…

Polymeric nitrogen with single bonds can be created from the molecular form at high pressure and due to large energy difference between triple and single bonds it is interesting as energetic material. Its structure and properties are,…

材料科学 · 物理学 2018-11-21 Dominika Melicherová , Oto Kohulák , Dušan Plašienka , Roman Martoňák

Carbon monoxide and nitrogen are among the potentially interesting high-energy density materials. However, in spite of the physical similarities of the molecules, they behave very differently at high pressures. Using density functional…

材料科学 · 物理学 2013-12-06 Zamaan Raza , Chris J. Pickard , Carlos Pinilla , A. Marco Saitta

The pressure-induced metallic states of light elements attract significant attention, because of potential applications as high-temperature superconductor and high-energy-density material, especially for hydrogen and nitrogen1-10. Several…

In this work, molecular dynamics simulations are performed to estimate the equilibrium pressure of liquid confined in nanopores. The simulations show that the pressure is highly sensitive to the pore size and can significantly change from…

软凝聚态物质 · 物理学 2021-04-21 An Zou , Shalabh C. Maroo

The phase diagram and equation of state of dense nitrogen are of interest in understanding the fundamental physics and chemistry under extreme conditions, including planetary processes, and in discovering new materials. We predict several…

Fluid phase equilibria involving nano-dispersed phases, where at least one of the coexisting phases is confined to a small volume, are investigated by molecular dynamics simulation. Complementing previous studies on nanoscopic droplets,…

介观与纳米尺度物理 · 物理学 2013-07-23 Martin Horsch , Hans Hasse

Nitrogen represents an archetypal example of material exhibiting a pressure driven transformation from molecular to polymeric state. Detailed investigations of such transformations are challenging because of a large kinetic barrier between…

Based on first-principles calculations and ab initio molecular dynamics simulations, the polymerisation of the unsaturated cis dinitrogen-difluoride (cis-N2F2) molecular compound is investigated. The thermodynamic, dynamical and thermal…

材料科学 · 物理学 2025-03-14 Guo Chen , Ling Lin , Chengfeng Zhang , Jie Zhang , Gilles Frapper , Xianlong Wang

The paper concerns the nanopowder high-speed, $10^4$ - $10^9$ s${}^{-1}$, compaction processes modeling by a two-dimensional granular dynamics method. Nanoparticles interaction, in addition to known contact laws, included dispersive…

材料科学 · 物理学 2018-11-09 G. Sh. Boltachev , N. B. Volkov , A. V. Spirin , E. A. Chingina

The structural properties of Na2RuO3 under pressure are studied using density functional theory within the generalized gradient approximation (GGA). We found that one may expect a structural transition at ~ 3 GPa. This structure at the…

强关联电子 · 物理学 2018-05-04 D. D. Gazizova , A. V. Ushakov , S. V. Streltsov

We report a study of the effects of pressure on the diffusivity of water molecules confined in single- wall carbon nanotubes (SWNT) with average mean pore diameter of 16 Angstroms. The measurements were carried out using high-resolution…

软凝聚态物质 · 物理学 2015-06-16 S. O. Diallo , M. Jazdzewska , J. C. Palmer , E. Mamontov , K. E. Gubbins , M. Sliwinska-Bartkowiak

The equations of state at room temperature as well as the energies of crystal structures up to pressures exceeding 100 GPa are calculated for Na and K . It is shown that the allowance for generalized gradient corrections (GGA) in the…

材料科学 · 物理学 2009-10-31 M. I. Katsnelson , G. V. Sinko , N. A. Smirnov , A. V. Trefilov , K. Yu. Khromov
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