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We report single crystal growth and magnetic susceptibility and neutron diffraction studies of the S=1/2 quasi-1D antiferromagnet CaCu2O3. The structure of this material is similar to that of the prototype two-leg spin-ladder compound…

凝聚态物理 · 物理学 2009-10-31 V. Kiryukhin , Y. J. Kim , K. J. Thomas , F. C. Chow , R. W. Erwin , Q. Huang , M. A. Kastner , R. J. Birgeneau

We report on the microscopic model of the recently synthesized one-dimensional quantum magnet (NO)Cu(NO3)3. Applying density functional theory band structure calculations, we obtain a leading antiferromagnetic exchange coupling J ~ 200 K,…

强关联电子 · 物理学 2010-11-15 O. Janson , A. A. Tsirlin , H. Rosner

Exploring the physics of low-dimensional spin systems and their pressure-driven electronic and magnetic transitions are thriving research field in modern condensed matter physics. In this context, recently antiferromagnetic Cr-based…

强关联电子 · 物理学 2024-01-02 Kuldeep Kargeti , Aadit Sen , S. K. Panda

We report the signatures of dynamic spin fluctuations in the layered honeycomb Li$_3$Cu$_2$SbO$_6$ compound, with a 3$d$ S = 1/2 $d^9$ Cu$^{2+}$ configuration, through muon spin rotation and relaxation ($\mu$SR) and neutron scattering…

We present results based on local spin density calculations of a computational search for half-metallic (HM) antiferromagnetic (AFM) materials within the class of double perovskite structure oxides LaM'M''O3 that incorporate open shell 3d…

材料科学 · 物理学 2009-10-30 Warren E. Pickett

We report experimental results of the static magnetization, ESR and NMR spectroscopic measurements of the Ni-hybrid compound NiCl$_3$C$_6$H$_5$CH$_2$CH$_2$NH$_3$. In this material NiCl$_3$ octahedra are structurally arranged in chains along…

The electronic and magnetic structure, including the Heisenberg model exchange interaction parameters, was explored for the recently proposed novel cuprate Cu$_2$F$_5$. Using the DFT+U calculation, it is shown that the compound is formed by…

强关联电子 · 物理学 2021-08-11 Dmitry M. Korotin , Dmitry Y. Novoselov , Vladimir I. Anisimov , Artem R. Oganov

In this work we study the interplay between the crystal structure and magnetism of the pyroarsenate \alpha-Cu_2As_2O_7 by means of magnetization, heat capacity, electron spin resonance and nuclear magnetic resonance measurements as well as…

The magnetic phase diagram and the thermodynamic properties of a square lattice containing antiferromagnetically coupled spin-1/2 triangles are studied. A Heisenberg Hamiltonian with three strong intra-triangle exchange coupling constants…

强关联电子 · 物理学 2009-10-31 Stefan Wessel , Stephan Haas

Two-dimensional honeycomb lattices, characterized by their low coordination numbers, provide a fertile platform for exploring various quantum phenomena due to the intricate interplay between competing magnetic interactions, spin-orbit…

Using thermodynamic measurements and density-functional band-structure calculations, we explore magnetic behavior of SrCuTe2O6. Despite being a structural sibling of a three-dimensional frustrated system PbCuTe2O6, this spin-1/2 quantum…

材料科学 · 物理学 2015-06-29 N. Ahmed , A. A. Tsirlin , R. Nath

Elastic and inelastic neutron scattering were used to study the ordered phase of the quasi-one-dimensional spin-1/2 antiferromagnet ${\rm BaCu_{2}Si_{2}O_{7}}$. The previously proposed model for the low-temperature magnetic structure was…

LiCu$_3$O$_3$ is a novel 2D S=1/2 antiferromagnet with randomly depleted square lattice. The crystal structure contains two types of square planes with different Cu$^{2+}\rightarrow$ Li$^{+}$ substitution rates (20% and 40%). $^7$Li NMR and…

强关联电子 · 物理学 2024-09-09 A. A. Bush , S. K. Gotovko , V. Yu. Ivanov , V. I. Kozlov , E. G. Nikolaev , L. E. Svistov

Spin-1/2 Heisenberg antiferromagnetic frustrated spin chain systems display exotic ground states with unconventional excitations and distinct quantum phase transitions as the ratio of next-nearest-neighbor to nearest-neighbor coupling is…

Two quasi-1-dimensional S=1 quantum antiferromagnetic materials, PbNi2V2O8 and SrNi2V2O8, are studied by inelastic neutron scattering on powder samples. While magnetic interactions in the two systems are found to be very similar, subtle…

强关联电子 · 物理学 2009-10-31 A. Zheludev , T. Masuda , I. Tsukada , Y. Uchiyama , K. Uchinokura , P. Boni , S. -H. Lee

The recent synthesis of the chromium selenide compound LiCrSe$_2$ constitutes a valuable addition to the ensemble of two-dimensional triangular lattice antiferromagnets (2D-TLA). In this work we present the very first comprehensive study of…

An $S=1$ antiferromagnetic polymeric chain, [Ni(HF$_2$)(3-Clpy)$_4$]BF$_4$ (py = pyridine), has previously been identified to have intrachain, nearest-neighbor antiferromagnetic interaction strength $J/k_{\mathrm{B}} = 4.86$ K and…

We have investigated Haldane's conjecture for the S=2 isotropic antiferromagnetic quantum spin chain with nearest-neighbor exchange J. Using a density matrix renormalization group algorithm for chains up to L=350 spins, we find in the…

凝聚态物理 · 物理学 2014-10-13 U. Schollwoeck , Th. Jolicoeur

The ground states of two types of distorted mixed diamond chains with spins 1 and 1/2 are investigated using exact diagonalization, DMRG, and mapping onto low-energy effective models. In the undistorted case, the ground state consists of an…

强关联电子 · 物理学 2010-11-11 Kazuo Hida , Ken'ichi Takano , Hidenori Suzuki

A comprehensive theoretical and experimental study is presented of the magnetic susceptibility versus temperature \chi(T) of spin S = 1/2 two- and three-leg Heisenberg ladders and ladder oxide compounds. Extensive quantum Monte Carlo…

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