相关论文: Optimizing impulsive X-ray Raman scattering for po…

Scattering of ultraintense short laser pulses off relativistic electrons allows one to generate a large number of X- or $\gamma$-ray photons with the expense of the spectral width---temporal pulsing of the laser inevitable leads to…

We analyze ultrafast electron dynamics in the time domain upon optical excitation of propagating surface plasmon-polaritons (SPs) in metal-dielectric heterostructures. Developing a kinetic model where both local and non-local electron…

In this work we investigate the theory for three different uni-directional population transfer schemes in trapped multilevel systems which can be utilized to cool molecular ions. The approach we use exploits the laser-induced coupling…

Achieving coherent population transfer in the solid-state is challenging compared to atomic systems due to closely spaced electronic states and fast decoherence. Here, within an atomistic pseudopotential theory, we offer recipes for the…

Considering a two-level quantum system, we have proposed and represented a new approach for robust population transfer. In this scheme, the laser frequency has been swept in a finite time interval which simplifies the experimental…

We use an optically dense, anisotropic magneto-optical trap to study recoil-induced resonances (RIRs) in the transient, high-gain regime. We find that two distinct mechanisms govern the atomic dynamics: the finite, frequency-dependent…

We propose an optical pumping scheme to prepare trapped $\mathrm{AlH}^+$ molecules in a pure state, the stretched hyperfine state $\lvert F=\frac{7}{2},\, m_F=\frac{7}{2}\rangle$ of the rovibronic ground manifold $\lvert…

Photoinduced charge-transfer processes play a key role for novel photovoltaic phenomena and devices. Thus, the development of ab initio methods that allow for an accurate and computationally inexpensive treatment of charge-transfer…

We propose a model to study quantum population transfer via a structural continuum. The model is composed of two spins which are coupled to two bosonic modes separately by two control pulses, and the two bosonic modes are coupled to a…

Non-radiative optical energy transfer from a GaAs quantum well to a thin overlayer of an infrared organic semiconductor dye is unambiguously demonstrated. The dynamics of exciton transfer are studied in the time-domain using pump-probe…

We present a unified view of the frequency dependence of the various scattering processes involved when a neutral hydrogen atom interacts with a monochromatic, linearly-polarized photon. A computational approach is employed of the atom…

On the basis of optimal control theory, we numerically study how to optimally manipulate molecular vibrational dynamics by using cycle-averaged polarizability interactions induced by mildly intense non-resonant laser (NR) pulses. As the…

Accurate population transfer of uncoupled or weakly coupled spin states is crucial for many quantum information processing tasks. In this paper, we propose a fast and robust scheme for population transfer which combines invariant-based…

Femtosecond high-order harmonic transient absorption spectroscopy is used to resolve the complete |j,m> quantum state distribution of Xe+ produced by optical strong-field ionization of Xe atoms at 800nm. Probing at the Xe N_4/5 edge yields…

For molecules and materials responding to femtosecond-scale optical laser pulses, we predict maximum relative excitation of a Raman-active vibrational mode with period T when the pulse has an FWHM duration of 0.42 T. This result follows…

The Stimulated Raman Adiabatic Passage (STIRAP) procedure is a robust and complete population transfer method which have various application in chemistry and atomic physics. Here, we study the effects of one-photon detuning, transition…

Optimal control theory implementations for an efficient population transfer and creation of a maximum coherence in three-level system are considered. We demonstrate that the half-STIRAP (stimulated Raman adiabatic passage) scheme for…

Energies of np (n=6-9), ns (n=7-9), nd (n=6-8), and nf (n=5-6) states in Tl I and Pb II are obtained using relativistic many-body perturbation theory. Reduced matrix elements, oscillator strengths, transition rates, and lifetimes are…

It is demonstrated by single-atom simulations that X-ray signals in the 3.4 to 4 keV region from an 8 micron laser driven high harmonic generation can be increased by more than two orders of magnitude when a single-cycle pulse centered at…

We demonstrate a technique based on optical heterodyne detection to measure Rydberg population in thermal atomic vapour. The technique used a probe beam far off resonant to the D2 line of rubidium along with a reference beam with frequency…