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Solution-processed, lead halide-based perovskite solar cells have overcome important challenges over the recent years, offering low-cost and high solar power conversion efficiencies. However, they still undergo unoptimized light collection…

Despite the youthfulness of hybrid halide perovskite solar cells, their efficiencies are currently comparable to commercial silicon and have surpassed quantum-dots solar cells. Yet, the scalability of these devices is a challenge due to…

Perovskite solar cells (PSCs) are the most promising technology for advancing current photovoltaic performance. However, the main challenge for their practical deployment and commercialization is their operational stability, affected by…

We predict the structural, electronic and optic properties of the inorganic Ge-based halide perovskites AGeX3 (A = Cs, Rb; X = I, Br, Cl) by using first-principles method. In particular, absolute electronic energy band levels are calculated…

材料科学 · 物理学 2018-10-08 Un-Gi Jonga , Chol-Jun Yu , Yun-Hyok Kye , Yong-Guk Choe , Hao Wei , Shuzhou Li

The widespread use of lead-based materials in tandem solar cells raises critical environmental and health concerns due to their inherent toxicity and risk of contamination. To address this challenge, we focused on lead-free tandem…

The enhancement of the fill factor in the current generation of perovskite solar cells is the key for further efficiency improvement. Thus, methods to quantify the fill factor losses are urgently needed. A classical method to quantify Ohmic…

应用物理 · 物理学 2022-07-07 David Grabowski , Zhifa Liu , Gunnar Schöpe , Uwe Rau , Thomas Kirchartz

Lead (Pb) halide perovskites have achieved great success in recent years due to their excellent optoelectronic properties, which is largely attributed to the lone-pair s orbital-derived antibonding states at the valence band edge. Guided by…

材料科学 · 物理学 2021-05-07 Gang Tang , Philippe Ghosez , Jiawang Hong

The decrease of solar cell efficiency with temperature is a known problem for photovoltaics (PV). Temperature sensitivity can lead to a considerable amount of energy losses over the lifetime of solar panels. In this perspective Hybrid…

应用物理 · 物理学 2023-11-01 Bruno Lorenzi , Paolo Mariani , Andrea Reale , Aldo Di Carlo , Gang Chen , Dario Narducci

An optoelectronic optimization was carried out for an AlGaAs solar cell containing (i) an n-AlGaAs absorber layer with a graded bandgap and (ii) a periodically corrugated Ag backreflector combined with localized ohmic Pd-Ge-Au backcontacts.…

应用物理 · 物理学 2020-03-17 Faiz Ahmad , Akhlesh Lakhtakia , Peter B. Monk

With rapidly growing photoconversion efficiencies, hybrid perovskite solar cells have emerged as promising contenders for next generation, low-cost photovoltaic technologies. Yet, the presence of nanoscale defect clusters, that form during…

Fundamental working mechanisms of perovskite solar cells remain an elusive topic of research. Impedance Spectroscopy (IS) application to perovskite-based devices generates uncommon features and misleading outputs, mainly due to the lack of…

应用物理 · 物理学 2019-08-19 So-Min Yoo , Seog Joon Yoon , Juan A. Anta , Hyo Joong Lee , Pablo P. Boix , Iván Mora-Seró

Halide perovskites have emerged as promising candidates for high-performance solar cells. This study investigates the temperature-dependent optoelectronic properties of mixed-cation mixed-halide perovskite solar cells using…

In recent years, organic-inorganic hybrid perovskites have attracted wide attention due to their excellent optoelectronic properties in the application of optoelectronic devices. In the manufacturing process of perovskite solar cells,…

材料科学 · 物理学 2020-04-01 Lei Guo , Gao Xu , Gang Tang , Daining Fang , Jiawang Hong

Perovskite films have rapidly emerged as leading active materials in optoelectronic devices due to their strong optical absorption, high carrier mobility and ease of fabrication. Whilst proving to be promising materials for solar cells and…

Many recent advances in metal halide perovskite solar cell (PSC) performance are attributed to surface treatments which passivate interfacial trap states, minimise charge recombination and boost photovoltages. Surprisingly, these…

An effective method, performed adding external electric field (EEF) on CH3NH3PbI3-xClx (OPIC) perovskite layer during the annealing process, is proposed to improve the performance of the solar cell. By harmonizing EEF direction with the…

材料科学 · 物理学 2015-07-10 Xiu Gong , Heng Ma , Yu-Rong Jiang , Meng Li , Zhao-Kui Wang , Tetsuo Soga

Lead-halide perovskites exhibit remarkable efficiency in photovoltaics, driven by exceptionally long carrier diffusion lengths and recombination times. Paradoxically, this performance persists even in defect-rich, solution-grown samples.…

材料科学 · 物理学 2025-03-17 Dmytro Rak , Dusan Lorenc , Ayan A. Zhumekenov , Osman M. Bakr , Zhanybek Alpichshev

Hybrid organic-inorganic perovskites have been established as good candidate materials for emerging photovoltaics, with device efficiencies of over 22 % being reported. There are currently only two organic cations, methylammonium and…

Halide perovskites is a new class of semiconductors with exceptional optoelectronic properties. Among many advantages offered by halide perovskites, the bandgap energy can be tuned in a much broader range than what was possible in…