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Excitons and their complexes govern optical-related behaviors in semiconductors. Here, using angle-resolved photoemission spectroscopy (ARPES), we have elucidated the light-matter interaction mediated by quasi-steady excitonic complexes…

Most photocatalytic and photovoltaic devices operate under broadband, constant illumination. Electron and hole dynamics in these devices, however, are usually measured using ultrafast pulsed lasers in a narrow wavelength range. In this…

化学物理 · 物理学 2024-04-26 Levi D. Palmer , Wonseok Lee , Chung Li Dong , Ru-Shi Liu , Nianqiang Wu , Scott K. Cushing

Single-photon emitters in two-dimensional semiconductors offer a versatile platform for integrated quantum photonics, yet their performance is strongly influenced by local dielectric environments and substrate-induced disorder. Here, we…

Atom specific valence electronic structures at interface are elucidated successfully using soft x-ray absorption and emission spectroscopy. In order to demonstrate the versatility of this method, we investigated SiO2/Si interface as a…

A notable role in understanding of microscopic electronic properties of high temperature superconductors (HTSC) belongs to angle resolved photoemission spectroscopy (ARPES). This technique supplies a direct window into reciprocal space of…

超导电性 · 物理学 2007-05-23 A. A. Kordyuk , S. V. Borisenko

Multi-molecular excited states accompanied by an intra- and inter-molecular geometric relaxation are commonly encountered in optical and electrooptical studies and applications of organic semiconductors as, for example excimers or charge…

Since the earliest implementations of the various GW approximations and cumulant expansion in the calculations of quasiparticle propagators and spectra, several attempts have been made to combine the advantageous properties and results of…

材料科学 · 物理学 2016-08-03 Branko Gumhalter , Vjekoslav Kovač , Fabio Caruso , Henry Lambert , Feliciano Giustino

Atomically sharp 2D in-plane heterostructures with nanoscale interfaces provide a powerful platform for tailoring optical and electrical properties at the nanoscale, enabling novel device engineering and the exploration of new physical…

The implementation of a wide range of novel concepts for next-generation high-efficiency solar cells is based on nanostructures with configuration-tunable optoelectronic properties. On the other hand, effective nano-optical light-trapping…

材料科学 · 物理学 2018-04-04 Urs Aeberhard

This paper reviews the most recent ARPES results on the cuprate superconductors and their insulating parent and sister compounds, with the purpose of providing an updated summary of the extensive literature in this field. The low energy…

超导电性 · 物理学 2009-11-07 Andrea Damascelli , Zhi-Xun Shen , Zahid Hussain

Following the lifespan of optical excitations from their creation to decay into photons is crucial in understanding materials optical properties. Macroscopically, techniques such as the photoluminescence excitation spectroscopy provide…

The recent angle-resolved photoemission measurements performed up to binding energies of the order of 1eV reveals a very robust feature: the nodal quasi-particle dispersion breaks up around 0.3-0.4eV and reappears around 0.6-0.8eV. The…

超导电性 · 物理学 2015-06-25 Qiang-Hua Wang , Fei Tan , Yuan Wan

Relative cross sections for the valence shell photoionisation (PI) of $\rm ^2S$ ground level and $\rm ^2D$ metastable Ca$^{+}$ ions were measured with high energy resolution by using the ion-photon merged-beams technique at the Advanced…

In high-performance solar cells based on polymeric semiconductors, the mechanism of photocarrier generation on $<100$-fs timescales is yet to be unravelled. In particular the dynamics of early-time electronic coupling between excitons on…

Exciton and polaron pair dissociation is a key functional aspect of photovoltaic devices. To improve upon the current state of interfacial transport models, we augment the existing classical models of dielectric interfaces by incorporating…

材料科学 · 物理学 2017-05-08 Michael J. Waters , Daniel Hashemi , John Kieffer

We present a quantum optics theory, numerical calculations, and experiments on coupled quantumdots in semiconductor nanowire waveguides. We first present an analytical Green function theory tocompute the emitted spectra of two coupled…

At photoelectrosynthetic interfaces, an electrochemical reaction is driven by excited charge-carriers from a semiconducting photoabsorber. Structure and composition of this interface determine both the electronic and electrochemical…

化学物理 · 物理学 2022-05-30 Matthias M. May , Wolfram Jaegermann

Performing an in-depth analysis of the photoemission spectra along the nodal direction of the high temperature superconductor Bi-2212 we have developed a procedure to determine the underlying electronic structure and established a precise…

强关联电子 · 物理学 2007-05-23 A. A. Kordyuk , S. V. Borisenko , A. Koitzsch , J. Fink , M. Knupfer , H. Berger

The aim of the present paper is twofold. The first goal is to show that high resolution angle-resolved photoelectron spectra from cuprates indicate the presence of string-like excitations of the quasihole excitation in a quantum…

强关联电子 · 物理学 2009-11-13 Efstratios Manousakis

Surface photovoltage (SPV) spectroscopy, which is a versatile method to analyze the energetic distribution of electronic defect states at surfaces and interfaces of wide-bandgap semiconductor (hetero-)structures, is applied to comparatively…

材料科学 · 物理学 2013-12-31 Elke Beyreuther , Domenico Paparo , Andreas Thiessen , Stefan Grafström , Lukas M. Eng