相关论文: Observation of four-photon absorption and determin…
Recent \textit{ab initio} calculations predict 1D dispersive electronic bands confined to the atomic scale cores of dislocations in the wide bandgap (3.84 eV) semiconductor ZnS. We test these predictions by correlating sub-bandgap optical…
We investigate a four-state system interacting with long and short laser pulses in a weak probe beam approximation. We show that when all lasers are tuned to the exact unperturbed resonances, part of the four-wave mixing (FWM) field is…
We present the two kinds of experimental results. One is a continuous variable dense coding experiment, and the other is a photon number detector with high linearity response, the so called charge integration photon detector (CIPD). They…
We report the ultrafast and large third-order nonlinear optical properties of CdS nanocrystals (NCs) embedded in a polymeric film. The CdS NCs of 2-nm radius are synthesized by an ion exchange method and highly concentrated in the two…
We study coherent perfect absorption (CPA) of light in a Kerr nonlinear metal-dielectric composite medium, illuminated from the opposite ends. Elementary symmetry considerations reveal that equality of the incident light intensities is a…
We describe a high-resolution spectroscopy method, in which the detection of single excitation events is enhanced by a complete loss of coherence of a superposition of two ground states. Thereby, transitions of a single isolated atom nearly…
We have studied the electronic and optical properties of three low-symmetry graphene quantum dots (GQDs), with the point-group symmetries $C_{2v}$, and $C_{2h}$. For the calculations of linear optical absorption spectra, we employed both…
Femtosecond pump-probe measurements find pronounced dimensionality dependence of the optical nonlinearity in cuprates. Although the coherent two-photon absorption (TPA) and linear absorption bands nearly overlap in both quasi-one and…
The development of new quantum light sources requires robust and convenient methods of characterizing their joint spectral properties. Measuring the joint spectral intensity between a photon pair ignores any correlations in spectral phase…
We theoretically study the conditions under which two laser fields can undergo Coherent Perfect Absorption (CPA) when shined on a single-mode bi-directional optical cavity coupled with two two- level quantum emitters (natural atoms,…
Quaternary chalcogenide crystal Cu2CdGeS4 was studied both experimentally and theoretically in the present paper. Investigations of polarized fundamental absorption spectra demonstrated a high sensitivity to external light illumination. The…
In this paper, we present a theoretical study of the nonlinear optical response of the newly discovered conjugated polymer poly(diphenyl)polyacetylene (PDPA). In particular, we compute the third-order nonlinear susceptibility corresponding…
Two-pulse correlation experiments performed using pulses of different intensities on Pd(111) with different CO coverages showed that the CO photodesorption probability depends on whether the strong or the weak pulse arrives first to the…
We present a detailed study of the absolute Doppler-broadened absorption of a probe beam scanned across the potassium D lines in a thermal vapour. Spectra using a weak probe were measured on the 4S $\rightarrow$ 4P transition and compared…
First-principles dynamical CPA (Coherent-Potential Approximation) for electron correlations has been developed further by taking into account higher-order dynamical corrections with use of the asymptotic approximation. The theory is applied…
We show that two major carrier excitation mechanisms are present in II-VI self-assembled quantum dots. The first one is related to direct excited state - ground state transition. It manifests itself by the presence of sharp and intense…
Distinguishing photon-arrival time and position is crucial for advancing quantum technology. However, capturing spatial and temporal information efficiently remains challenging. Here, we present a novel photon-detection technique to achieve…
In quasi-1D $\pi$-conjugated polymers such as \emph{trans}-polyacetylene and polyenes, electron correlation effects determine the "reversed" excited state ordering in which the lowest two-photon $2A_{g}$ state lies below the lowest…
Hybrid interfaces between distinct quantum systems play a major role in the implementation of quantum networks. Quantum states have to be stored in memories to synchronize the photon arrival times for entanglement swapping by projective…
We report an experimental demonstration of photon switching by quantum interference in a four-level atomic system proposed by Harris and Yamamoto (Phys. Rev. Lett. 81, 3611 (1998)). Quantum interference inhibits single-photon absorption but…