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Imaging the structure of molecules in transient excited states remains a challenge due to the extreme requirements for spatial and temporal resolution. Ultrafast electron diffraction from aligned molecules (UEDAM) provides atomic resolution…

原子物理 · 物理学 2015-10-23 Jie Yang , Joshua Beck , Cornelis J. Uiterwaal , Martin Centurion

Photons experience mirror asymmetry of macroscopic chiral media, as in circular dichroism and polarization rotation, since left and right handed circular polarizations differently couple with matter handedness. Conversely, free relativistic…

量子物理 · 物理学 2022-04-08 Alessandro Ciattoni

Coherent Diffractive Imaging is a lensless technique that allows imaging of matter at a spatial resolution not limited by lens aberrations. This technique exploits the measured diffraction pattern of a coherent beam scattered by periodic…

Several laser techniques have been suggested and demonstrated recently for preparing polarizable molecules in rapidly spinning states with a disc-like angular distribution. We consider motion of these spinning discs in inhomogeneous fields,…

化学物理 · 物理学 2015-05-20 Johannes Floss , Erez Gershnabel , Ilya Sh. Averbukh

Interfaces between molecules and 2D materials exhibit energy-driven functionalities, wherein charge transfer directs molecular motion. Unlike equilibrium systems, where molecular assemblies settle into static configurations, continuous…

Friedel's law guarantees an inversion-symmetric diffraction pattern for thin, light materials where a kinematic approximation or a single-scattering model holds. Typically, breaking Friedel symmetry is ascribed to multiple scattering events…

We show that circularly polarized femtosecond laser pulses produce field-free alignment in linear and planar molecules. We study the rotational wavepacket evolution of O$_2$ and benzene created by circularly polarized light. For benzene, we…

化学物理 · 物理学 2014-06-06 C T L Smeenk , P B Corkum

We demonstrate that angle-resolved soft x-ray spectroscopy can resolve absorption by inequivalent oxygen sites and by different orbitals belonging to the same site in NaV2O5. By rotating the polarization direction, we see a dramatic change…

强关联电子 · 物理学 2009-11-07 G. P. Zhang , G. T. Woods , Eric L. Shirley , T. A. Callcott , L. Lin , G. S. Chang , B. C. Sales , D. Mandrus , J. He

To what extent can particulate random media be characterised using direct wave backscattering from a single receiver/source? Here, in a two dimensional setting, we show using a machine learning approach that both the particle radius and…

Intermolecular correlations in liquid acetonitrile (CH3CN) have been revisited by calculating orientational correlation functions. In the present approach, hydrogen atoms are included, so that a concept applicable for molecules of (nearly)…

化学物理 · 物理学 2019-06-12 Szilvia Pothoczki , László Pusztai

We provide new insights into backbending phenomenon within the symmetry-adapted framework which naturally describes the intrinsic deformation of atomic nuclei. For $^{20}\text{Ne}$, the canonical example of backbending in light nuclei, the…

The potential scattering of electrons carrying non--zero quanta of the orbital angular momentum (OAM) is studied in a framework of the generalized Born approximation, developed in our recent paper by Karlovets \textit{et al.}, Phys. Rev. A.…

量子物理 · 物理学 2017-03-21 D. V. Karlovets , G. L. Kotkin , V. G. Serbo , A. Surzhykov

We investigate the orientation dependence of molecular high-order harmonic generation (HHG) both numerically and analytically. We show that the molecular recollision electronic wave packets (REWPs) in the HHG are closely related to the…

原子物理 · 物理学 2009-11-13 Yanjun. Chen , Yan. Li , Shiping. Yang , Jie. Liu

We observe energy-dependent angle-resolved diffraction patterns in protons from strong-field dissociation of the molecular hydrogen ion H$_2^+$. The interference is a characteristic of dissociation around a laser-induced conical…

原子与分子团簇 · 物理学 2016-04-11 Adi Natan , Matthew R Ware , Vaibhav S. Prabhudesai , Uri Lev , Barry D. Bruner , Oded Heber , Philip H Bucksbaum

The scattering of light observed through the turbid underwater channel is often regarded as the leading challenge when designing underwater electro-optical imaging systems. There have been many approaches to address the effects of…

光学 · 物理学 2018-04-17 Chensheng Wu , Robert Lee , Christopher C. Davis

In this theoretical paper, we investigate coherence properties of the near-resonant light scattered by two atoms exposed to a strong monochromatic field. To properly incorporate saturation effects, we use a quantum Langevin approach. In…

量子物理 · 物理学 2016-08-24 Benoît Grémaud , Thomas Wellens , Dominique Delande , Christian Miniatura

We demonstrate that the spatial resolution of images in optical tomography is not limited to the fundamental length scale of one transport mean free path. This result is facilitated by the introduction of novel corrections to the standard…

光学 · 物理学 2007-05-23 George Y. Panasyuk , Vadim A. Markel , John C. Schotland

A solution to the inversion problem of scattering would offer aberration-free diffraction-limited 3D images without the resolution and depth-of-field limitations of lens-based tomographic systems. Powerful algorithms are increasingly being…

We introduce a novel reflection-mode diffraction tomography technique that enables simultaneous recovery of forward and backward scattering information for high-resolution 3D refractive index reconstruction. Our technique works by imaging a…

光学 · 物理学 2025-02-12 Tongyu Li , Jiabei Zhu , Yi Shen , Lei Tian

We study interaction of generic asymmetric molecules with a pair of strong time-delayed short laser pulses with crossed linear polarizations. We show that such an excitation not only provides unidirectional rotation of the most polarizable…

化学物理 · 物理学 2018-02-28 E. Gershnabel , I. Sh. Averbukh