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A moderately intense $450$ fs laser pulse is used to create rotational wave packets in gas phase $\rm{I_2}$ molecules. The ensuing time-dependent alignment, measured by Coulomb explosion imaging with a delayed probe pulse, exhibits the…

We show that dressing of diatomic molecules by running laser waves gives rise to conical intersections (CIs). Due to presence of such CIs, the rovibronic molecular motions are strongly coupled. A pronounced impact of the CI on the spectrum…

原子物理 · 物理学 2015-05-19 Milan Sindelka , Nimrod Moiseyev , Lorenz S. Cederbaum

We use an optical centrifuge to align asymmetric top $\mathrm{SO_2}$ molecules by adiabatically spinning their most polarizable O-O axis. The effective centrifugal potential in the rotating frame confines sulfur atoms to the plane of the…

化学物理 · 物理学 2016-05-11 A. Korobenko , V. Milner

We coincidently measure the molecular frame photoelectron angular distribution and the ion sum-momentum distribution of single and double ionization of CO molecules by using circularly and elliptically polarized femtosecond laser pulses,…

原子物理 · 物理学 2015-06-04 J. Wu , L. Ph. H. Schmidt , M. Kunitski , M. Meckel , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

Observing the motion of the nuclear wavepackets during a molecular reaction, in both space and time, is crucial for understanding and controlling the outcome of photoinduced chemical reactions. We have imaged the motion of a vibrational…

In this paper we demonstrate a computational method to solve the inverse scattering problem for a star-shaped, smooth, penetrable obstacle in 2D. Our method is based on classical ideas from computational geometry. First, we approximate the…

Emerging coherent X-ray scattering patterns of single-particles have shown dominant morphological signatures in agreement with predictions of the scattering model used for conventional protein crystallography. The key question is if and to…

生物大分子 · 定量生物学 2014-07-28 Aliakbar Jafarpour

Ring quantum cascade lasers have recently gained considerable attention, showing ultrastable frequency comb and soliton operation, thus opening a way to integrated spectrometers in the midinfrared and terahertz fingerprint regions. Thanks…

We consider imaging of fast moving small objects in space, such as low earth orbit satellites, which are also rotating around a fixed axis. The imaging system consists of ground based, asynchronous sources of radiation and several passive…

信号处理 · 电气工程与系统科学 2021-11-03 Matan Leibovich , George Papanicolaou , Chrysoula Tsogka

Electron quantum path interferences in strongly laser-driven aligned molecules and their dependence on the molecular alignment is an essential open problem in strong-field molecular physics. Here, we demonstrate an approach which provides…

The Quantitative Rescattering Theory (QRS) for high-order harmonic generation (HHG) by intense laser pulses is presented. According to the QRS, HHG spectra can be expressed as a product of a returning electron wave packet and the…

原子物理 · 物理学 2009-08-05 Anh-Thu Le , R. R. Lucchese , S. Tonzani , T. Morishita , C. D. Lin

Thick biological tissues give rise to not only the scattering of incoming light waves, but also aberrations of the remaining unscattered waves. Due to the inability of existing optical imaging methodologies to overcome both of these…

We review experimental and theoretical studies of coherent backscattering of near resonant radiation from an ultracold atomic gas in the weak localization regime. Recent accomplishments in high resolution spectroscopy of atomic ensembles…

原子物理 · 物理学 2017-02-01 I. M. Sokolov , D. V. Kupriyanov , C. I. Sukenik , M. D. Havey

Understanding the scattering properties of various media is of critical importance in many applications, from secure, high-bandwidth communications to extracting information about biological and mineral particles dissolved in sea water. In…

光学 · 物理学 2020-02-05 Duncan McArthur , Alison Yao , Francesco Papoff

We study the direct and an inverse source problem for the radiative transfer equation arising in optical molecular imaging. We show that for generic absorption and scattering coefficients, the direct problem is well-posed and the inverse…

偏微分方程分析 · 数学 2008-03-31 Plamen Stefanov , Gunther Uhlmann

A theoretical study of the rotational dynamics of a linear polar molecule in a two-color non-resonant cw laser field is presented. By systematically considering the interactions of this field with the electric dipole moment, polarizability…

量子物理 · 物理学 2020-08-26 David Mellado-Alcedo , Niurka R. Quintero , Rosario González-Férez

The tomographic imaging of arbitrary molecular orbitals via high-order harmonic generation requires that electrons recollide from one direction only. Within a semi-classical model, we show that extremely short phase-stabilized laser pulses…

原子物理 · 物理学 2009-11-13 Elmar V. van der Zwan , Manfred Lein

Our visual perception of our surroundings is ultimately limited by the diffraction limit, which stipulates that optical information smaller than roughly half the illumination wavelength is not retrievable. Over the past decades, many…

Achieving quantum-limited motional control of optically trapped particles beyond the sub-micrometer scale is an outstanding problem in levitated optomechanics. A key obstacle is solving the light scattering problem and identifying particle…

光学 · 物理学 2025-07-15 Moosung Lee , Benjamin A. Stickler , Thomas Pertsch , Sungkun Hong

Light propagating in an optically thick sample experiences multiple scattering. It is now known that interferences alter this propagation, leading to an enhanced backscattering, a manifestation of weak localization of light in such diffuse…

原子物理 · 物理学 2009-10-31 G. Labeyrie , F. de Tomasi , J. -C. Bernard , C. A. Mueller , C. Miniatura , R. Kaiser
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