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Ferromagnetic insulators (FMIs) are one of the most important components in developing dissipationless electronic and spintronic devices. However, since ferromagnetism generally accompanies metallicity, FMIs are innately rare to find in…

We have investigated magneto-transport properties in a single crystal of pyrochore-type Nd2Ir2O7. The metallic conduction is observed on the antiferromagnetic domain walls of the all-in all-out type Ir-5d moment ordered insulating bulk…

材料科学 · 物理学 2016-10-31 K. Ueda , J. Fujioka , B. -J. Yang , J. Shiogai , A. Tsukazaki , S. Nakamura , S. Awaji , N. Nagaosa , Y. Tokura

Transport and magnetic properties along with high resolution valence band photoemission study of disordered double perovskite Sr$_{2}$TiIrO$_{6}$ has been investigated. Insulator to insulator transition along with a magnetic transition…

强关联电子 · 物理学 2023-01-18 B. H. Reddy , Asif Ali , Ravi Shankar Singh

Coupling between different interactions allows to control physical aspects in multifunctional materials by perturbing any of the degrees of freedom. Here, we aim to probe the correlation among structural, electronic and magnetic observables…

The emergence of ferro- and ferrimagnetic behavior in insulating materials is uncommon, largely due to Hund's rules. Utilizing symmetry analysis, first-principles methods, and classical Monte Carlo simulations, \textcolor{black}{we report…

We investigate the metal-insulator transition in the layered Ruddelsden Popper series of strontium iridates Srn+1IrnO3n+1. Tight-binding models of t2g orbitals for n = 1, 2, and infinity are constructed, and changes in band dispersion due…

强关联电子 · 物理学 2015-06-05 Jean-Michel Carter , V. Vijay Shankar , Hae-Young Kee

The coexistence of the strongly correlated 3$d$ transition metal (TM) atom and the strong spin-orbit coupling (SOC) of 5$d$ TM atom is potential to host exotic physical phenomena. In the present work, we have studied the magnetism resulting…

强关联电子 · 物理学 2020-02-19 Shreemoyee Ganguly , Sayantika Bhowal

Using density functional calculations we explore the properties of as-yet-unsynthesized $3d - 5d$ ordered double perovskites ($A_2BB'$O$_6$) with highly polarizable Bi$^{3+}$ ions on the $A$ site. We find that the Bi$_2$NiReO$_6$ and…

材料科学 · 物理学 2015-03-13 Marjana Ležaić , Nicola A. Spaldin

Exchange bias properties are observed in a double perovskite compound, Sr2LuRuO6. The observed exchange bias properties have been analyzed on the basis of some of the available theoretical models. Detailed magnetization measurements show…

强关联电子 · 物理学 2010-09-17 Ravi. P. Singh , C. V. Tomy

The search for room-temperature magnetocaloric materials for refrigeration has led to investigations of double perovskites. In particular, a puzzle has appeared in the La$_2$MnNiO$_6$, La$_2$MnCoO$_6$ and La$_2$MnFeO$_6$ family of…

We report electron spin resonance (ESR) spectroscopy results on the double perovskite Ba$_2$YIrO$_6$. On general grounds, this material is expected to be nonmagnetic due to the strong coupling of the spin and orbital momenta of Ir$^{5+}$…

强关联电子 · 物理学 2018-06-12 S. Fuchs , T. Dey , G. Aslan-Cansever , A. Maljuk , S. Wurmehl , B. Büchner , V. Kataev

The magnetic susceptibility, crystal and magnetic structures, and electronic structure of double perovskite Sr2ScOsO6 are reported. Using both neutron and x-ray powder diffraction we find that the crystal structure is monoclinic P21/n from…

强关联电子 · 物理学 2015-04-06 A. E. Taylor , R. Morrow , D. J. Singh , S. Calder , M. D. Lumsden , P. M. Woodward , A. D. Christianson

We report an unusual magnetic ground state in single-crystal, double-perovskite Ba2YIrO6 and Sr doped Ba2YIrO6 with Ir5+(5d4) ions. Long-range magnetic order below 1.7 K is confirmed by DC magnetization, AC magnetic susceptibility and heat…

强关联电子 · 物理学 2017-09-01 J. Terizc , H. Zheng , Feng Ye , H. D. Zhao , P. Schlottmann , L. De Long , G. Cao

Hybrid transition metal oxides continue to attract attention due to their multiple degrees of freedom ($e.g.$, lattice, charge, spin, and orbital) and versatile properties. Here we investigate the magnetic and electronic properties of the…

强关联电子 · 物理学 2022-05-17 Ke Yang , Wenjing Xu , Di Lu , Yuxuan Zhou , Lu Liu , Yaozhenghang Ma , Guangyu Wang , Hua Wu

The electronic and magnetic properties of monoclinic double perovskite Sr$_2$CeIrO$_6$ were examined based on both experiments and first-principles density functional theory calculations. From the calculations we conclude that…

材料科学 · 物理学 2016-07-13 Sudipta Kanungo , Kailash Mogare , Binghai Yan , Claudia Felser , Martin Jansen

Using density-functional theory calculations, we investigated the electronic structure and magnetic exchange interactions of the ordered 3d-5d double perovskite Sr2FeOsO6, which has recently drawn attention for interesting antiferromagnetic…

材料科学 · 物理学 2014-07-24 Sudipta Kanungo , Binghai Yan , Martin Jansen , Claudia Felser

The synthesis and physical properties of the double perovskite (DP) compound Ba2CdReO6 with the 5d1 electronic configuration are reported. Three successive phases originating from a spin-orbit-entangled Jeff = 3/2 state, confirmed by the…

强关联电子 · 物理学 2021-04-06 Daigorou Hirai , Zenji Hiroi

In this work, we report the synthesis and investigation of structural, electronic, and magnetic properties of La$_{1.5}$Ca$_{0.5}$(Co$_{0.5}$Fe$_{0.5}$)IrO$_6$. Our polycrystalline sample forms as a single-phase double perovskite in…

Perovskite iridates of 6H hexagonal structure present a plethora of possibilities in terms of the variety of ground states resulting from a competition between spin-orbit coupling (SOC), hopping, noncubic crystal field ($\Delta_{CFE}^{NC}$)…

强关联电子 · 物理学 2019-08-15 Md Salman Khan , Abhisek Bandyopadhyay , Abhishek Nag , Vinod Kumar , A. V. Mahajan , Sugata Ray

Double perovskite iridates $A_2$ZnIrO$_6$ ($A$ = alkaline or lanthanide) show complex magnetic behaviors ranging from weak ferromagnetism to successive antiferromagnetic transitions. Here we report the static ($dc$) and dynamic ($ac$)…

强关联电子 · 物理学 2021-02-24 H. Guo , C. Ritter , Y. Su , A. C. Komarek , J. S. Gardner