相关论文: Radiation Pressure Force from Optical Cycling on a…
Optical cycling transitions and direct laser cooling have recently been demonstrated for a number of alkaline-earth dimers and trimer molecules. This is made possible by diagonal Franck-Condon factors between the vibrational modes of the…
We consider propagation, storing and retrieval of slow light (probe beam) in a resonant atomic medium illuminated by two control laser beams of larger intensity. The probe and two control beams act on atoms in a tripod configuration of the…
We propose a method to generate a source of spin-polarized cold atoms which are continuously extracted and guided from a magneto-optical trap using an atom-diode effect. We show that it is possible to create a pipe-like potential by…
A study of the intensity-borrowing mechanisms important to optical cycling transitions in laser-coolable polyatomic molecules arising from non-adiabatic coupling, contributions beyond the Franck-Condon approximation, and Fermi resonances is…
We demonstrate a three-dimensional magneto-optical trap (MOT) of a metal hydride molecule, CaH. We are able to scatter $\sim$$10^{4}$ photons with vibrational loss covered up to vibrational quantum number $\nu=2$. This allows us to laser…
A circularly polarized laser beam is used to levitate and control the rotation of microspheres in high vacuum. At low pressure, rotation frequencies as high as 6 MHz are observed for birefringent vaterite spheres, limited by centrifugal…
We report on the generation of optical vortices with few-cycle pulse durations, 500$\mu$J per pulse, at a repetition rate of 1 kHz. To do so, a 25 fs laser beam at 800 nm is shaped with a helical phase and coupled into a hollow core fiber…
The interaction of atoms with higher-order Poincar\'e optical vortex modes of order $m\geq 0$ is explored for light close to resonance with atomic dipole transitions. It is well-known that atoms subject to optical vortex modes experience…
We report on the realization of a transversely loaded two-dimensional magneto-optical trap serving as a source for cold strontium atoms. We analyze the dependence of the source's properties on various parameters, in particular the intensity…
Laser cooling by collisional redistribution of radiation has been successfully applied in the past for cooling dense atomic gases. Here we report on progress of work aiming at the demonstration of redistribution laser cooling in a molecular…
The nature of light-matter interaction is governed by the spatial-temporal structures of a light field and material wavefunctions. The emergence of the light beam with transverse phase vortex, or equivalently orbital angular momentum (OAM)…
In the presence of an external static magnetic field, an atomic gas becomes optically active, showing magneto-optical rotation. In the saturated regime, the coherences among the excited substates give a nonlinear contribution to the…
We present a faster repumping scheme for strontium magneto-optical traps operating on the broad ${\mathrm{5s^2} ^1\mathrm{S}_0} - {\mathrm{5s5p} ^1\mathrm{P}_1}$ laser cooling transition. Contrary to existing repumping schemes, we directly…
We demonstrate rotational excitation of molecular ions that are sympathetically cooled by laser-cooled atomic ions to a temperature as low as ca. 10 mK. The molecular hydrogen ions HD+ and the fundamental rotational transition $(v=0,\,…
A special class of molecules that are important to many subfields in molecular dynamics and chemical physics, namely free radical molecules, now enjoy a significant degree of center-of-mass motion control in the laboratory frame. The…
Employing a two-stage cryogenic buffer gas cell, we produce a cold, hydrodynamically extracted beam of calcium monohydride molecules with a near effusive velocity distribution. Beam dynamics, thermalization and slowing are studied using…
We present a high-resolution laser spectroscopic study of the $\tilde{A}\,^2B_2- \tilde{X}\,^2A_1$ and $\tilde{B}\,^2B_1- \tilde{X}\,^2A_1$ transitions of calcium (I) phenoxide, CaOPh (CaOC$_6$H$_5$). The rotationally resolved band systems…
The pressure dependence of light-induced effects in single-crystalline BiFeO$_3$ is studied by optical spectroscopy. At low pressures, we observe three light-induced absorption features with energies just below the two crystal field…
Ultracold molecular gases are promising as an avenue to rich many-body physics, quantum chemistry, quantum information, and precision measurements. This richness, which flows from the complex internal structure of molecules, makes the…
Light-matter interaction allows to achieve non-equilibrium states that are otherwise inaccessible. Motivated by recent experiments that report ferroelectricity -- and even multiferroicity -- in the prototypical diamagnetic band insulator…