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Rydberg alkaline earth atoms are promising tools for quantum simulation and metrology. When one of the two valence electrons is promoted to long-lived circular states, the second valence electron can be optically manipulated without…

原子物理 · 物理学 2024-06-04 L. Lachaud , B. Muraz , A. Couto , J. -M. Raimond , M. Brune , S. Gleyzes

Optical control of polyatomic molecules promises new opportunities in precision metrology, fundamental chemistry, quantum information, and many-body science. Contemporary experimental and theoretical efforts have mostly focused on cycling…

原子物理 · 物理学 2022-12-26 Phelan Yu , Adrian Lopez , William A. Goddard , Nicholas R. Hutzler

Optical circulators are important components of modern day communication technology. With their ability to route photons directionally, these nonreciprocal elements provide useful functionality in photonic circuits and offer prospects for…

We report bunching, slowing, and acceleration of a supersonically cooled beam of diatomic hydroxyl radicals (OH). \textit{In situ} observation of laser-induced fluorescence along the beam propagation path allows for detailed…

原子物理 · 物理学 2009-11-10 J. R. Bochinski , Eric R. Hudson , H. J. Lewandowski , Jun Ye , Gerard Meijer

We report magneto-optical trapping (MOT) of a polyatomic molecule, calcium monohydroxide (CaOH). The MOT contains $2.0(5)\times 10^4$ CaOH molecules at a peak density of $3.0(8)\times10^{6}$ cm$^{-3}$. CaOH molecules are further sub-Doppler…

Triatomic molecule RaOH combines the advantages of laser-coolability and the spectrum with close opposite-parity doublets. This makes it a promising candidate for experimental study of the $\mathcal{P}$,$\mathcal{T}$-violation. Previous…

原子物理 · 物理学 2021-03-17 Anna Zakharova , Alexander Petrov

Herein, we show that single molecules containing multiple optical cycling centers (CaO moieties) can exhibit superradiant phenomena. We demonstrate the accuracy of the Frenkel exciton model at describing these superradiant states via…

Vacuum-stimulated Raman transitions are driven between two magnetic substates of a rubidium-87 atom strongly coupled to an optical cavity. A magnetic field lifts the degeneracy of these states, and the atom is alternately exposed to laser…

量子物理 · 物理学 2007-05-23 T. Wilk , S. C. Webster , H. P. Specht , G. Rempe , A. Kuhn

In this work we demonstrate vibrational spectroscopy of polyatomic ions that are trapped and sympathetically cooled by laser-cooled atomic ions. We use the protonated dipeptide tryptophane-alanine (HTyrAla+) as a model system, cooled by…

化学物理 · 物理学 2017-09-13 Ch. Wellers , A. Borodin , S. Vasilyev , D. Offenberg , S. Schiller

The high chemical reactivity of strontium, which can opacify a viewport exposed to a strontium atomic source, is a concern for some atomic physics experiments where it is sometimes necessary to send a laser beam counter-propagating relative…

We present an analysis of the deceleration and trapping of heavy diatomic molecules in low-field seeking states by a moving electric potential. This moving potential is created by a 'ring-decelerator', which consists of a series of…

We demonstrate that strong-field ionization of atoms driven by circularly polarized light becomes an adiabatic process when described in the frame rotating with the laser field. As a direct consequence, a conservation law emerges: in the…

A new means of incorporating radiative transfer into smoothed particle hydrodynamics (SPH) is introduced, which builds on the success of two previous methods - the polytropic cooling approximation as devised by Stamatellos et al (2007), and…

天体物理学 · 物理学 2009-11-13 Duncan Forgan , Ken Rice , Dimitris Stamatellos , Anthony Whitworth

We report on the design and characterization of a cold atom source for strontium (Sr) based on a two-dimensional magneto-optical trap (MOT) that is directly loaded from the atom jet of a dispenser. We characterize the atom flux of the…

We propose a method of stimulated laser cooling of diatomic molecules by counter-propagating $\pi$-trains of ultrashort laser pulses. The cooling cycles occur on the rovibrational transitions inside the same ground electronic manifold, thus…

原子物理 · 物理学 2015-03-13 Ekaterina Ilinova , Jonathan Weinstein , Andrei Derevianko

Based on an experimental study of two-body and three-body collisions in ultracold strontium samples, a novel optical-sympathetic cooling method in isotopic mixtures is demonstrated. Without evaporative cooling, a phase-space density of…

原子物理 · 物理学 2007-05-23 G. Ferrari , R. E. Drullinger , N. Poli , F. Sorrentino , G. M. Tino

We have probed the fragmentation dynamics in a bent triatomic molecule, water, a non-planar molecule, methanol, and a planar ring-structured molecule, benzene, using 100 fs duration pulses of linearly and circularly polarized, infrared,…

原子物理 · 物理学 2009-11-10 F A Rajgara , M Krishnamurthy , D Mathur

Optical dynamic nuclear polarization (DNP) offers an attractive approach to enhancing the sensitivity of nuclear magnetic resonance (NMR) spectroscopy. Efficient, optically-generated electron polarization can be leveraged to operate across…

Single-layer transition-metal dichalcogenides provide an unique intrinsic entanglement between the spin/valley/orbital degrees of freedom and the polarization of scattered photons. This scenario gives rise to the well-assessed optical…

材料科学 · 物理学 2025-01-13 Habib Rostami , Federico Cilento , Emmanuele Cappelluti

We present a new radiative transfer method (SPH-M1RT) that is coupled dynamically with smoothed particle hydrodynamics (SPH). We implement it in the (task-based parallel) SWIFT galaxy simulation code but it can be straightforwardly…

天体物理仪器与方法 · 物理学 2021-07-06 T. K. Chan , Tom Theuns , Richard Bower , Carlos Frenk