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相关论文: Rovibrationally-Resolved Photodissociaton of SH$^+…

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Accurate photodissociation cross sections have been computed for transitions from the X $^1\Sigma^+$ ground electronic state of CS to six low-lying excited electronic states. New ab initio potential curves and transition dipole moment…

Accurate photodissociation cross sections have been obtained for the A-X electronic transition of HeH+ using ab initio potential curves and dipole transition moments. Partial cross sections have been evaluated for all rotational transitions…

星系天体物理 · 物理学 2015-05-28 S. Miyake , C. D. Gay , P. C. Stancil

We illustrate some of the difficulties that may be encountered when computing photodissociation and radiative association cross sections from the same time-dependent approach based on wavepacket propagation. The total and partial…

化学物理 · 物理学 2015-06-12 S. Vranckx , J. Loreau , M. Desouter-Lecomte , N. Vaeck

Total and partial cross sections for breakup of ground rovibronic state of H$_2^+$by photon impact are calculated using the exact nonadiabatic nonrelativistic Hamiltonian without approximation. The converged results span six orders of…

化学物理 · 物理学 2013-08-09 Daniel J. Haxton

Experiments are conducted to investigate the role of the avoided crossing seam in the photodissociation of H$_3^+$. Three-dimensional imaging of dissociation products is used to determine the kinetic energy release and branching ratio among…

化学物理 · 物理学 2019-08-09 X. Urbain , A. Dochain , R. Marion , T. Launoy , J. Loreau

The opacity due to photodissociation of 24MgH is investigated in the atmospheres of cool stars. The lowest two electronic transitions A 2Pi -- X 2Sigma+ and B' 2Sigma+ -- X 2 Sigma+ are considered where the cross sections for the latter…

天体物理学 · 物理学 2009-11-07 P. F. Weck , A. Schweitzer , P. C. Stancil , P. H. Hauschildt , K. Kirby

Photodissociation is one of the main destruction pathways for dicarbon (C$_{2}$) in astronomical environments such as diffuse interstellar clouds, yet the accuracy of modern astrochemical models is limited by a lack of accurate…

星系天体物理 · 物理学 2022-07-27 Zhongxing Xu , S. R. Federman , William M. Jackson , Cheuk-Yiu Ng , Lee-Ping Wang , Kyle N. Crabtree

Photodissociation by ultraviolet radiation is the key destruction pathway for CS in photon-dominated regions, such as diffuse clouds. However, the large uncertainties of photodissociation cross sections and rates of CS, resulting from a…

星系天体物理 · 物理学 2019-09-11 Zhongxing Xu , Nan Luo , S. R. Federman , William M. Jackson , Cheuk-Yiu Ng , Lee-Ping Wang , Kyle N. Crabtree

We investigate the dynamics of the photodissociation of the hydrohelium cation HeH$^+$ by XUV radiation with the aim to establish a detailed comparison with a recent experimental work carried out at the FLASH free electron laser using both…

原子物理 · 物理学 2015-05-28 J. Loreau , J. Lecointre , X. Urbain , N. Vaeck

The matrix elements and energies needed to calculate vibrational-rotational state resolved cross sections and rate coefficients for radiative association of H and p and for photodissociation of H${}_2^+$ are presented for applications to…

原子物理 · 物理学 2015-01-21 James F. Babb

The radiative association of C(${}^3P$) and H${}^+$ is investigated by calculating cross sections for photon emission into bound ro-vibrational states of CH${}^+$ from the vibrational continua of initial triplet d$\,{}^3\Pi$ or…

原子物理 · 物理学 2017-05-04 James F. Babb , Brendan M. McLaughlin

The cross section for dissociative recombination of BeH^+ is calculated by solution of the time-dependent Schrodinger equation in the local complex potential approximation. The effects of couplings between resonant states and the Rydberg…

原子物理 · 物理学 2009-04-02 J. B. Roos , M. Larsson , AA. Larson , A. E Orel

We used the multichannel quantum defect theory to compute cross sections and rate coefficients for the dissociative recombination of CH$^+$ initially in its lowest vibrational level $v_i^+ = 0$ with electrons of incident energy bellow $0.2$…

天体物理仪器与方法 · 物理学 2022-03-08 J. Zs. Mezei , M. D. Epée Epée , O. Motapon , I. F. Schneider

A quantitative theoretical study of the dissociative recombination of SH$^+$ with electrons has been carried out. Multireference, configuration interaction calculations were used to determine accurate potential energy curves for SH$^+$ and…

天体物理仪器与方法 · 物理学 2024-05-31 D. O. Kashinski , D. Talbi , A. P. Hickman , O. E. Di Nallo , F. Colboc , K. Chakrabarti , I. F. Schneider , J. Zs Mezei

Photoionization cross sections and rate coefficients have been calculated for all bound vibrational levels of the 1s$\sigma_{\mathrm{g}}$ state of H$_{2}^{+}$, HD$^{+}$, and D$_{2}^{+}$. The Born-Oppenheimer approximation is employed in our…

原子物理 · 物理学 2023-11-03 Adam Singor , Liam H. Scarlett , Mark C. Zammit , Igor Bray , Dmitry V. Fursa

We investigate the photodissociation of the metastable triplet state of HeH+ as well as its formation through the inverse process, radiative association. In models of astrophysical plasmas, HeH+ is assumed to be present only in the ground…

化学物理 · 物理学 2015-06-12 J. Loreau , S. Vranckx , M. Desouter-Lecomte , N. Vaeck , A. Dalgarno

The vibrational branching ratios of SrOH for radiative decay to the ground electronic state, $X^{2}\Sigma^{+}$, from the first two electronically excited states, $A^{2}\Pi$ and $B^{2}\Sigma^{+}$, are determined experimentally at the…

原子物理 · 物理学 2022-08-17 Zack Lasner , Annika Lunstad , Chaoqun Zhang , Lan Cheng , John M. Doyle

The electronic structure of six low-lying electronic states of scandium hydride, $X\,{}^{1}\Sigma^+$, $a\,{}^{3}\Delta$, $b\,{}^{3}\Pi$, $A\,{}^{1}\Delta$ $c\,{}^{3}\Sigma^+$, and $B\,{}^{1}\Pi$, is studied using multi-reference…

星系天体物理 · 物理学 2015-04-17 Lorenzo Lodi , Sergei N. Yurchenko , Jonathan Tennyson\

The high resolution rovibronic line list of MgH+ molecular cation are presented in our work. The potential energy curves are calculated by the method of multireference configuration interaction plus Davidson correction (MRCI+Q) and…

太阳与恒星天体物理 · 物理学 2024-01-03 Huagang Xiao , Tao Gao

The photodissociation cross section of the molecular ion HeH$^+$ was calculated within the Born-Oppenheimer approximation for a parallel, a perpendicular, and an isotropic orientation of the molecular axis with respect to the field,…

原子物理 · 物理学 2015-05-13 Irina Dumitriu , Alejandro Saenz
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