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The rutile TiO$_2$ (110) surface reduced by the bridging oxygen vacancy, bridging hydroxyl group or Ti interstitial atom has been investigated by calculating their electronic structures using the density functional theory plus U method. It…

材料科学 · 物理学 2015-10-13 Daoyu Zhang , Minnan Yang , Shuai Dong

Hydroxylation of the rutile TiO$_2$ (110) surface has attracted much attention as the excess unpaired electrons introduced by hydroxyls play a critical role in surface chemistry and photocatalysis process of this material. In this work,…

材料科学 · 物理学 2015-10-13 Daoyu Zhang , Minnan Yang , Shuai Dong

Eutectic NiTiO$_3$-TiO$_2$ samples and their H$_2$ reduced Ni-TiO$_2$ samples, where high aspect ratio TiO$_2$ nanostructures are axially decorated with nodular Ni globules, are thoroughly explored to understand their effect in…

Atomic and electronic structures of TiO_2(110) surface with possible adsorptional, substitutional and interstitial Au or Pt elemental impurities at full and one-sixth monolayer concentrations were investigated by density functional theory…

强关联电子 · 物理学 2012-11-19 Ersen Mete , Oğuz Gülseren , Şinasi Ellialtıoğlu

The presence of small hematite (Fe2O3) clusters at low coverage on titanium dioxide (TiO2) surface has been observed to enhance photocatalytic activity, while excess loading of hematite is detrimental. We conduct a comprehensive density…

材料科学 · 物理学 2024-04-09 Kati Asikainen , Matti Alatalo , Marko Huttula , Bernardo Barbiellini , S. Assa Aravindh

We apply high-energy proton ion-implantation to modify TiO2 nanotubes selectively at their tops. In the proton-implanted region we observe the creation of intrinsic co-catalytic centers for photocatalytic H2-evolution. We find proton…

We use first-principles calculations to investigate the adsorption and incorporation of non-metal impurities (N, C) at the anatase TiO$_2$(001)-(1$\times$4) reconstructed surface. We analyze in detail the influence of the surface structure…

材料科学 · 物理学 2015-06-11 Jun Hee Lee , Daniel Fernandez Hevia , Annabella Selloni

Surfaces of homoepitaxially grown TiO2-terminated SrTiO3(001) were studied in situ with scanning tunneling microscopy and spectroscopy. By controlling the Ti/Sr ratio, two-dimensional domains of highly ordered linear nanostructures,…

材料科学 · 物理学 2017-10-25 W. Yan , W. Sitaputra , M. Skowronski , R. M. Feenstra

Photocatalytic nitrogen fixation provides a promising route to produce reactive nitrogen compounds at benign conditions. Titania has been reported as an active photocatalyst for reduction of dinitrogen to ammonia; however there is little…

化学物理 · 物理学 2018-02-01 Benjamin M. Comer , Andrew J. Medford

In the present work we investigate various optical properties (such as light absorption and reflectance) of anodic TiO2 nanotubes layers directly transferred as self-standing membranes onto quartz substrates. This allows investigation in a…

材料科学 · 物理学 2016-10-18 Gihoon Cha , Patrik Schmuki , Marco Altomare

In this work we study the optoelectronic properties of individual TiO2 fibres produced through coupled sol-gel and electrospinning, by depositing them onto pre-patterned Ti/Au electrodes on SiO2/Si substrates. Transport measurements in the…

Titanium dioxide (TiO$_2$) thin films are commonly used as photocatalytic materials. Here, we enhance the photocatalytic activity of devices based on TiO$_2$ by combining nanostructured glass substrates with metallic plasmonic…

Colloidal cobalt-doped TiO2 (anatase) nanocrystals were synthesized and studied by electronic absorption, magnetic circular dichroism, transmission electron microscopy, magnetic susceptibility, cobalt K-shell X-ray absorption spectroscopy,…

材料科学 · 物理学 2007-05-23 J. Daniel Bryan , Steve M. Heald , Scott A. Chambers , Daniel R. Gamelin

A comprehensive phase diagram of lowest-energy structures and compositions of the rutile TiO_2(110) surface in equilibrium with a surrounding gas phase at finite temperatures and pressures has been determined using density functional theory…

材料科学 · 物理学 2009-11-13 Piotr M. Kowalski , Bernd Meyer , Dominik Marx

The efforts in the optimization of the physical and chemical properties related to the photocatalytic efficiency of TiO2 nanoparticles relies mainly on defect engineering strategies, been the structural and the doping the most common ones.…

材料科学 · 物理学 2022-03-07 M. P. Ferreira , H. B. de Carvalho

Low-dose nitrogen implantation induces in TiO2 nanotubes a co-catalytic activity for photocatalytic H2-evolution. The use of an ion implantation process leads to a N-implanted zone only at the top part of the tubes. The coupling of this top…

The conversion efficiency of dye-sensitized solar cells (DSSCs) is optimized by modifying the optical design and improving absorbance within the cell. These objectives are obtained by creating different sized cavities in TiO2 photoanode.…

化学物理 · 物理学 2015-03-24 Elham Bayatloo , Esmaiel Saievar-Iranizad

Titanium dioxide is one of the most widely investigated oxides. This is due to its broad range of applications, from catalysis to photocatalysis to photovoltaics. Despite this large interest, many of its bulk properties have been sparsely…

材料科学 · 物理学 2010-03-12 L. Chiodo , J. M. García-Lastra , D. J. Mowbray , A. Iacomino , A. Rubio

Converting CO$_2$ to useful compounds through the solar photocatalytic reduction has been one of the most promising strategies for artificial carbon recycling. The highly relevant photocatalytic substrate for CO$_2$ conversion has been the…

化学物理 · 物理学 2015-05-28 Shijing Tan , Yan Zhao , Jin Zhao , Zhuo Wang , Chuanxu Ma , Aidi Zhao , Bing Wang , Yi Luo , Jinlong Yang , Jianguo Hou

Adsorption of CO$_2$ on a semiconductor surface is a prerequisite for its photocatalytic reduction. Owing to superior photocorrosion resistance, nontoxicity and suitable band edge positions, TiO$_2$ is considered to be the most efficient…

材料科学 · 物理学 2018-12-05 Shashi B. Mishra , Aditya Choudhary , Somnath C. Roy , B. R. K. Nanda
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