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Exciton transfer along a polymer is essential for many biological processes, for instance light harvesting in photosynthetic biosystems. Here we apply a new witness of non-classicality to this phenomenon, to conclude that, if an exciton can…

量子物理 · 物理学 2024-09-12 Giuseppe Di Pietra , Vlatko Vedral , Chiara Marletto

Strong light--matter interactions forming hybrid quasiparticles termed polaritons can specifically tailor molecular photophysics. In this spirit, enhancing energy transport has recently been of special interest. Exciton--exciton…

化学物理 · 物理学 2026-01-14 Luca Nils Philipp , Julian Lüttig , Roland Mitric

Floquet engineering of electronic systems is a promising way of controlling quantum material properties on an ultrafast time scale. So far, the energy structure of Floquet states in solids has been observed through time and angle-resolved…

其他凝聚态物理 · 物理学 2023-05-02 Kento Uchida , Satoshi Kusaba , Kohei Nagai , Tatsuhiko N. Ikeda , Koichiro Tanaka

Photosynthesis is the basic process used by plants to convert light energy in reaction centers into chemical energy. The high efficiency of this process is not yet understood today. Using the formalism for the description of open quantum…

生物物理 · 物理学 2017-06-12 Hichem Eleuch , Ingrid Rotter

In this work we report the results of theoretical analysis of the effect of thermal environment on the thermoelectric efficiency of molecular junctions. The environment is represented by two thermal phonon baths associated with the…

材料科学 · 物理学 2014-06-25 Natalya A. Zimbovskaya

In coupled quantum systems pure dephasing mechanisms acting on one constituent of the hybrid system break symmetry and enable optical transitions which are forbidden in the non-coupled system, i.e., the pure dephasing bath opens a cascaded…

量子物理 · 物理学 2022-07-26 Ruben Pompe , Matthias Hensen , Matthew Otten , Stephen K. Gray , Walter Pfeiffer

Heat transport in open quantum systems is particularly susceptible to the modeling of system-reservoir interactions. It thus requires to consistently treat the coupling between a quantum system and its environment. While perturbative…

统计力学 · 物理学 2017-06-07 Thomas Motz , Joachim Ankerhold , Jürgen T. Stockburger

An asymptotic scaling theory is presented using the conceptual basis of trapping-free subspace (i.e., orthogonal subspace) to establish the generic mechanism of optimal efficiency of excitation energy transfer (EET) in light-harvesting…

量子物理 · 物理学 2013-05-16 Jianlan Wu , Jianshu Cao , Robert J. Silbey

Understanding the mechanisms of efficient and robust energy transfer in light-harvesting systems provides new insights for the optimal design of artificial systems. In this paper, we use the Fenna-Matthews-Olson (FMO) protein complex and…

化学物理 · 物理学 2011-09-27 Jianlan Wu , Fan Liu , Young Shen , Jianshu Cao , Robert J. Silbey

This study investigates quantum energy teleportation (QET) using stochastic bi-partitioning in an $N-$body Hamiltonian system. In this protocol, project measurements are performed on $(N - m)$ qubits to capture quantum fluctuation…

量子物理 · 物理学 2024-10-08 Zhirong Xun , Changliang Ren

The theory of energy transfer dynamics of a pair of donor and acceptor molecules located in the plasmonic hot spots is developed by means of the master equation approach and the electromagnetic Green's tensor technique. A nonlocal effect…

光学 · 物理学 2017-12-29 Jun Ren , Tian Chen , Bo Wang , Xiangdong Zhang

A pure-dephasing reservoir acting on an individual quantum system induces loss of coherence without energy exchange. When acting on composite quantum systems, dephasing reservoirs can lead to a radically different behavior. Transport of…

量子物理 · 物理学 2015-02-03 T. Werlang , D. Valente

The interplay between exctions and vibrations is considered to be a key factor in determining the exciton transfer properties in light-harvesting exciton transfer complexes. Here we study this interplay theoretically in a model for exciton…

介观与纳米尺度物理 · 物理学 2018-05-25 Omer Goldberg , Yigal Meir , Yonatan Dubi

The possibility to exploit quantum coherence to strongly enhance the efficiency of charge transport in solid state devices working at ambient conditions would pave the way to disruptive technological applications. In this work, we tackle…

Exciton transport in molecular aggregates with magic-angle orientation is expected to be strongly suppressed due to their negligible dipole-dipole interactions. However, recent reports show that light-matter interactions can significantly…

化学物理 · 物理学 2026-03-10 Siwei Wang , Liang-Yan Hsu , Hsing-Ta Chen

In quantum systems, one usually seeks to minimize dephasing noise and disorder. The efficiency of transport in a quantum system is usually degraded by the presence of noise and disorder. However, it has been shown that the combination of…

量子物理 · 物理学 2015-06-11 M. Zhang , Tony E. Lee , H. R. Sadeghpour

The light-harvesting is a problem of long interest. It becomes active again in recent years stimulated by suggestions of quantum effects in energy transport. Recent experiments found evidence that BChla 1 and BChla 6 are the first to be…

生物物理 · 物理学 2015-06-04 B. Cui , X. X. Yi , C. H. Oh

The fluctuation-dissipation relation is well known for the quantum open system with energy dissipation. In this paper a similar underlying relation is found between the bath fluctuation and the dephasing of the quantum open system, of which…

量子物理 · 物理学 2013-05-29 Y. B. Gao , C. P. Sun

Following the calculation of optimal energy transfer in thermal environment in our first paper (Wu et al., New J. Phys., 2010, 12, 105012), full quantum dynamics and leading-order `classical' hopping kinetics are compared in the seven-site…

化学物理 · 物理学 2015-05-30 Jianlan Wu , Fan Liu , Jian Ma , Robert J. Silbey , Jianshu Cao

We present a detailed theoretical study of the transfer of electronic excitation energy through the Fenna-Matthews-Olson (FMO) pigment-protein complex, using the new developed modified scaled hierarchical approach [Shi Q. et al, J Chem Phys…

化学物理 · 物理学 2011-03-17 Jing Zhu , Sabre Kais , Patrick Rebentrost , Alán Aspuru-Guzik