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Photoionization cross sections calculations on the halogen-like ions; Kr$^+$ and Xe$^+$ have been performed for a photon energy range from each ion threshold to 15 eV, using large-scale close-coupling calculations within the Dirac-Coulomb…

地球与行星天体物理 · 物理学 2012-04-02 B. M. McLaughlin , C. P. Ballance

We present a unique experimental design that enables the measurement of photoelectron circular dichroism (PECD) from chiral molecules in aqueous solution. The effect is revealed from the intensity difference of photoelectron emission into a…

We discuss the theory of coupled ionization--dissociation fronts produced when molecular clouds are exposed to $\lambda < 1110$\AA\ radiation from hot stars. A steady, composite structure is developed, which generally includes an ionized…

天体物理学 · 物理学 2009-10-28 Frank Bertoldi , B. T. Draine

The electric dipole moments of $(H_{2}O)_{n}DCl$ ($n=3-9$) clusters have been measured by the beam deflection method. Reflecting the (dynamical) charge distribution within the system, the dipole moment contributes information about the…

原子与分子团簇 · 物理学 2015-02-06 Nicholas Guggemos , Petr Slavíček , Vitaly V. Kresin

New approach to highly accurate calculations of the photodetachment cross-sections of the negatively charged hydrogen ions is developed. This effective, fast and numerically stable method is based on the use of the Rayleigh's formula for…

太阳与恒星天体物理 · 物理学 2015-09-09 Alexei M. Frolov

The two-body photodisintegration of 3He has been investigated using tagged photons with energies from 14 -- 31 MeV at MAX-lab in Lund, Sweden. The two-body breakup channel was unambiguously identified by the (nonsimultaneous) detection of…

The mechanisms for photodissociation of methyl halides (CH$_3$X, X= Cl, Br, I) have been studied for these molecules when adsorbed on thin films of C$_6$H$_6$ or C$_6$F$_6$ on copper single crystals, using time-of-flight spectroscopy with…

化学物理 · 物理学 2021-01-29 E. T. Jensen

We demonstrate spectroscopy and thermometry of individual motional modes in a mesoscopic 2D ion array using entanglement-induced decoherence as a method of transduction. Our system is a $\sim$400 $\mu$m-diameter planar crystal of several…

We present velocity map imaging data on intramolecular ion-pair dissociation (IPD) of carbonyl sulfide (OCS) induced by electron impact over the 20 eV to 45 eV energy range. Two distinct IPD pathways were resolved: CO+ + S- (threshold 14.8…

原子与分子团簇 · 物理学 2026-04-21 Narayan Kundu , Soumya Ghosh , Dhananjay Nandi

Differential Phase Contrast (DPC) imaging, in which deviations in the bright field beam are in proportion to the electric field, has been extensively studied in the context of pure elastic scattering. Here we discuss differential phase…

其他凝聚态物理 · 物理学 2024-08-29 Michael Deimetry , Timothy C. Petersen , Hamish G. Brown , Matthew Weyland , Scott D. Findlay

Experimental and theoretical cross sections are reported for single-photon single ionization of W$^{5+}$ ions. Absolute measurements were conducted employing the photon-ion merged-beams technique. Detailed photon-energy scans were performed…

原子物理 · 物理学 2020-01-08 A Müller , S Schippers , J Hellhund , A L D Kilcoyne , R A Phaneuf , B M McLaughlin

In a joint experimental and theoretical endeavour, photoionization of metastable C4+(1s 2s 3S1) ions via intermediate levels with hollow, double-K-vacancy configurations 2s2p, 2s3p, 2p3s, 2p3d, 2s4p, 2p4s and 2p4d has been investigated.…

The dipole strength of the nuclide $^{76}$Ge was studied in photon-scattering experiments using bremsstrahlung produced with electron beams of energies of 7.8 and 12.3 MeV at the $\gamma$ELBE facility. We identified 210 levels up to an…

In a double-slit experiment with a bipartite system, the visibility of interference fringes depends on the availability of which-way information. Here, we report the formation of a Bell-like state of photoelectron and residual ion in the…

Using the photon-ion merged-beams technique at the PETRA\,III synchrotron light source, we have measured cross sections for double and up to tenfold photoionization of La$^{+}$ ions by a single photon in the energy range 820--1400~eV, where…

We consider an ensemble of diatomic molecules resonantly coupled to an optical cavity under strong coupling conditions at normal incidence. Photodissociation dynamics is examined via direct numerical integration of the coupled…

化学物理 · 物理学 2023-03-08 Maxim Sukharev , Joseph Subotnik , Abraham Nitzan

[Background] Photon strength functions are an important ingredient in calculations relevant for the nucleosynthesis of heavy elements. The relation to the photoabsorption cross section allows to experimentally constrain photon strength…

Several diatomic transition metal oxides, rare-earth metal oxides and fluorides have the unusual property that their bond dissociation energy is larger than their ionization energy. In these molecules, bound levels above the ionization…

原子与分子团簇 · 物理学 2024-06-06 Sascha Schaller , Johannes Seifert , Giacomo Valtolina , André Fielicke , Boris G. Sartakov , Gerard Meijer

The reaction pp->{pp}_s\gamma, where {pp}_s is a proton pair with an excitation energy E_{pp}<3 MeV, has been observed with the ANKE spectrometer at COSY-Juelich for proton beam energies of T_p=0.353, 0.500, and 0.550 GeV. This is…

Joint electron-ion energy spectra for the dissociative ionization of a model H$_2^+$ in few-cycle, infrared laser pulses are calculated via the numerical ab initio solution of the time-dependent Schr\"odinger equation. A strong,…

原子物理 · 物理学 2017-11-21 V. Mosert , D. Bauer