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Exciton transfer dynamics between chromophores depends on excitonic coupling, which is governed by relative orientation between the chromophores. While the excitonic coupling is treated as a static parameter in many cases, structural…

化学物理 · 物理学 2026-05-06 Hiroki Uratani , Hirofumi Sato

We analyse the size and density of thermally induced regions of close contact in cell:cell contact interfaces within a harmonic potential approximation, estimating these regions to be below one-tenth of a micron across. Our calculations…

生物物理 · 物理学 2013-04-01 Amit K Chattopadhyay , Nigel J Burroughs

Until recently it was believed that photosynthesis, a fundamental process for life on earth, could be fully understood with semi-classical models. However, puzzling quantum phenomena have been observed in several photosynthetic…

We investigate the electronic dynamics of model organic photovoltaic (OPV) system consisting of polyphenylene vinylene (PPV) oligomers and [6,6]-phenyl C61-butyric acid methylester (PCBM) blend using a mixed molecular mechanics/quantum…

材料科学 · 物理学 2015-09-21 Eric R. Bittner , Allen C. Kelley

We present a theory of the electronic structure and photophysics of 1:1 blends of derivatives of polyparaphenylenevinylene and fullerenes. Within the same Coulomb-correlated Hamiltonian applied previously to interacting chains of…

强关联电子 · 物理学 2015-05-13 K. Aryanpour , D. Psiachos , S. Mazumdar

Approximate expressions for correlation functions in binary inhomogeneous mixtures are derived in a framework of the mesoscopic theory [Ciach A., Mol. Phys., 2011, {\textbf{109}}, 1101]. Fluctuation contribution is taken into account in a…

软凝聚态物质 · 物理学 2020-05-26 A. Ciach , O. Patsahan , A. Meyra

Organic semiconductors have the remarkable property that their optical excitation not only generates charge-neutral electron-hole pairs (excitons) but also charge-separated polaron pairs with high yield. The microscopic mechanisms…

We review the studies of a wide range of optical phenomena resulting from near-field coupling between excitons and localized surface plasmon-polaritons in hybrid nanostructures. Modern physical approaches and theoretical models reported…

光学 · 物理学 2025-02-28 V. S. Lebedev , A. D. Kondorskiy

We model energy transfer between two coupled four-level chromophores with arbitrarily spaced energy levels. Our analysis takes into account the crucial---yet often ignored---process of initial excitation by light that is incident on the…

量子物理 · 物理学 2012-02-17 Chi-Han Chang , Agata M. Branczyk , Gregory D. Scholes , Daniel F. V. James

Exciton plasmon polaritons have gained increasing interests over recent years due to their versatile properties emerging by the underlying light-matter coupling and making them potential candidates for new photonic applications. We have…

Entanglement of excitons holds great promise for the future of quantum computing, which would use individual molecular dyes as building blocks of their circuitry. Even though entangled excitonic eigenstates emerging in coupled molecular…

原子与分子团簇 · 物理学 2021-12-23 Jiří Doležal , Sofia Canola , Prokop Hapala , Rodrigo C. de Campos Ferreira , Pablo Merino , Martin Švec

Optical properties of transition metal dichalcogenides monolayers are controlled by the Wannier-Mott excitons forming a series of $1s$, $2s$, $2p$,... hydrogen-like states. We develop the theory of the excited excitonic states energy…

介观与纳米尺度物理 · 物理学 2017-02-01 M. M. Glazov , L. E. Golub , G. Wang , X. Marie , T. Amand , B. Urbaszek

Chromatin and associated proteins constitute the highly folded structure of chromosomes. We consider a self-avoiding polymer model of the chromatin, segments of which may get cross-linked via protein binders that repel each other. The…

软凝聚态物质 · 物理学 2019-06-13 Amit Kumar , Debasish Chaudhuri

The absorption of ultraviolet light creates excitations in DNA, which subsequently start moving in the helix. Their fate is important for an understanding of photo damage, and is determined by the interplay of electronic couplings between…

化学物理 · 物理学 2015-05-18 Arend G. Dijkstra , Yoshitaka Tanimura

Excitons in the weakly interacting regime can be well-described by many-body perturbation theories such as the Bethe-Salpeter equation formalism. However, for materials such as transition metal dichalcogenides moir\'e heterostructures under…

材料科学 · 物理学 2026-03-16 Fangzhou Zhao , Carlos Mejuto-Zaera , Angel Rubio , Vojtěch Vlček

Emergent strongly-correlated electronic phenomena in atomically-thin transition metal dichalcogenides are an exciting frontier in condensed matter physics, with examples ranging from bilayer superconductivity~\cite{zhao2023evidence} and…

Randomly rotating particles that have been isotropically labeled with rigidly linked fluorophores will undergo non-isotropic (patchy) photobleaching under illumination due to the dipole coupling of fluorophores with light. For a rotational…

化学物理 · 物理学 2017-11-08 Swadhin Taneja , Andrew D. Rutenberg

In the crowded eukaryotic nucleus, euchromatin and heterochromatin segregate into distinct compartments, a phenomenon often attributed to homotypic interactions mediated by liquid liquid phase separation of chromatin associated proteins.…

软凝聚态物质 · 物理学 2025-05-27 Luming Meng , Boping Liu , Qiong Luo

Chiral pair fluctuation are considered near the phase boundary of the inhomogeneous chiral phase (iCP). The fluctuations are then bosonized and an effective action for the chiral pair fluctuation is basically constructed by considering the…

高能物理 - 唯象学 · 物理学 2017-02-28 T. Tatsumi , R. Yoshiike , T. -G. Lee

We have studied the exciton states in two coupled conjugated polymer chains which are modeled individually by the Su-Schrieffer-Heeger Hamiltonian and coupled by an interchain electron-transfer term. Both the intra- and inter-chain long…

软凝聚态物质 · 物理学 2009-10-30 Z. G. Yu , M. W. Wu , X. S. Rao , X. Sun , A. R. Bishop