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Dynamical correlations of Jeff = 1/2 isospins in the paramagnetic state of spin-orbital Mott insu- lator Sr2IrO4 was revealed by resonant magnetic x-ray diffuse scattering. We found two-dimensional antiferromagnetic fluctuation with a large…

强关联电子 · 物理学 2015-06-04 S. Fujiyama , H. Ohsumi , T. Komesu , J. Matsuno , B. J. Kim , M. Takata , T. Arima , H. Takagi

Sr2IrO4 has been suggested as a Mott insulator from a single J_eff=1/2 band, similar to the cuprates. However this picture is complicated by the measured large magnetic anisotropy and ferromagnetism. Based on a careful mapping to the…

强关联电子 · 物理学 2011-03-31 Fa Wang , T. Senthil

Time-of-flight inelastic neutron scattering measurements on Sr2IrO4 single crystals were performed to access the spin Hamiltonian in this canonical Jeff=1/2 spin-orbital Mott insulator. The momentum of magnetic scattering at all inelastic…

强关联电子 · 物理学 2018-12-12 S. Calder , D. M. Pajerowski , M. B. Stone , A. F. May

The collective magnetic excitations in the spin-orbit Mott insulator (Sr$_{1-x}$La$_x$)$_2$IrO$_4$ ($x=0,\,0.01,\,0.04,\, 0.1$) were investigated by means of resonant inelastic x-ray scattering. We report significant magnon energy gaps at…

We report magnetic and thermodynamic properties of a $4d^1$ (Mo$^{5+}$) magnetic insulator MoOPO$_4$ single crystal, which realizes a $J_1$-$J_2$ Heisenberg spin-$1/2$ model on a stacked square lattice. The specific-heat measurements show a…

The 5d iridates have been the subject of much recent attention due to the predictions of a large array of novel electronic phases driven by twisting strong spin-orbit coupling and Hubbard correlation. As a prototype, the single layered…

材料科学 · 物理学 2015-03-10 Chengliang Lu , Shuai Dong , Andy Quindeau , Daniele Preziosi , Ni Hu , Marin Alexe

We have investigated the temperature evolution of magnetism and its interrelation with structural parameters in perovskite-based layered compound Sr$_2$IrO$_4$, which is believed to be a $J_{eff}$ = 1/2 Mott insulator. The structural…

强关联电子 · 物理学 2014-12-15 Imtiaz Noor Bhatti , R. Rawat , A. Banerjee , A. K. Pramanik

Spin-orbit entangled magnetic dipoles, often referred to as pseudospins, provide a new avenue to explore novel magnetism inconceivable in the weak spin-orbit coupling limit, but the nature of their low-energy interactions remains to be…

The motion of doped electrons or holes in an antiferromagnetic lattice with strong on-site Coulomb interactions touches one of the most fundamental open problems in contemporary condensed matter physics. The doped charge may strongly couple…

Based on the microscopic model including strong spin-orbit coupling, on-site Coulomb and Hund's interactions, as well as crystal field effects, we have investigated magnetic and optical properties of Sr2IrO4. Taking into account all…

强关联电子 · 物理学 2012-12-11 Beom Hyun Kim , G. Khaliullin , B. I. Min

The infrared transmission measurement was performed for a two-dimensional spin-orbit coupling induced Mott insulator Sr$_{2}$IrO$_{4}$ with a layered-perovskite structure. A phonon-assisted magnon mode was observed at around 1870 cm$^{-1}$…

强关联电子 · 物理学 2015-06-12 Yasuyuki Hirata , Hiroyuki Tajima , Kenya Ohgushi

Sr$_{2}$IrO$_{4}$ has often been described via a simple, one-band pseudo-spin 1/2 model, subject to electron-electron interactions, on a square lattice, fostering analogies with cuprate superconductors, believed to be well described by a…

We report measurements of the specific heat and the thermal conductivity of the model Heisenberg spin-1/2 chain cuprate Sr$_{2}$CuO$_{3}$ at low temperatures. In addition to a nearly isotropic phonon heat transport, we find a quasi…

强关联电子 · 物理学 2009-10-31 A. V. Sologubenko , E. Felder , K. Gianno , H. R. Ott , A. Vietkine , A. Revcolevschi

Metamagnetism in antiferromagnets exhibits distinct critical behaviors and dynamics when invoking spin reversal and rotation. Here we show a 0.05% anisotropic strain suffices to in-situ modulate the metamagnetic critical field of the Mott…

强关联电子 · 物理学 2020-07-24 H. Zhang , L. Hao , J. Yang , J. Mutch , Z. Liu , Q. Huang , K. Noordhoek , A. F. May , J. -H. Chu , J. W. Kim , P. J. Ryan , H. D. Zhou , Jian Liu

We perform a time-resolved optical study of Sr$_2$IrO$_4$ to understand the influence of magnetic ordering on the low energy electronic structure of a strongly spin-orbit coupled $J_{eff}$=1/2 Mott insulator. By studying the recovery…

强关联电子 · 物理学 2012-03-21 D. Hsieh , F. Mahmood , D. H. Torchinsky , G. Cao , N. Gedik

We report a high-field electron spin resonance study in the sub-THz frequency domain of a single crystal of Sr$_2$IrO$_4$ that has been recently proposed as a prototypical spin-orbital Mott insulator. In the antiferromagnetically (AFM)…

强关联电子 · 物理学 2015-06-18 S. Bahr , A. Alfonsov , G. Jackeli , G. Khaliullin , A. Matsumoto , T. Takayama , H. Takagi , B. Büchner , V. Kataev

As a hallmark of electronic correlation, spin-charge interplay underlies many emergent phenomena in doped Mott insulators, such as high-temperature superconductivity, whereas the half-filled parent state is usually electronically frozen…

The antiferromagnetic structure of Sr3Ir2O7, the bilayer analogue of a spin-orbital Mott insulator Sr2IrO4, was revealed by resonant magnetic x-ray diffraction. Contrasting intensities of the magnetic diffraction at the Ir LIII and LII…

强关联电子 · 物理学 2015-06-05 Shigeki Fujiyama , K. Ohashi , H. Ohsumi , K. Sugimoto , T. Takayama , T. Komesu , M. Takata , T. Arima , H. Takagi

An intriguing idea of spin-orbit Mott insulator has been proposed to explain magnetic insulating behavior in various iridates. This scenario relies on the strength of the spin-orbit coupling being comparable to electronic correlations, and…

强关联电子 · 物理学 2013-05-30 Jean-Michel Carter , Hae-Young Kee

The temperature-dependent behavior of magnetic domains plays an essential role in the magnetic properties of materials, leading to widespread applications. However, experimental methods to access the three-dimensional (3D) magnetic domain…

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