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Innovative ways of harnessing sustainable energy are needed to meet the world's ever-increasing energy demands. Supercapacitors may contribute, as they can convert waste heat to electricity through cyclic charging and discharging at…

软凝聚态物质 · 物理学 2023-03-27 Mathijs Janssen , Taras Verkholyak , Andrij Kuzmak , Svyatoslav Kondrat

The energy efficiency and power of a three-terminal thermoelectric nanodevice are studied by considering elastic tunneling through a single quantum dot. Facilitated by the three-terminal geometry, the nanodevice is able to generate…

介观与纳米尺度物理 · 物理学 2017-08-22 Jincheng Lu , Rongqian Wang , Yefeng Liu , Jian-Hua Jiang

An atomistic effective Hamiltonian technique is used to investigate the finite-temperature energy storage properties of a ferroelectric nanocomposite consisting of an array of BaTiO$_{3}$ nanowires embedded in a SrTiO$_{3}$ matrix, for…

Photo-rechargeable (solar) battery can be considered as an energy harvesting cum storage system, where it can charge the conventional metal-ion battery using light instead of electricity, without having other parasitic reactions. Here we…

It is shown that continuously occurring electrolyte-reduction reaction on freshly-exposed electrode surfaces during lithiation/delithiation cycles causes the lowering of cycling efficiency, and hence, capacity fade in well-cycled silicon…

材料科学 · 物理学 2020-02-19 Vijay A. Sethuraman

The solid-state electrolyte is critical for achieving next-generation high energy density and high-safety batteries. Solid polymer electrolytes (SPEs) possess great potential for commercial application owing to their compatibility with the…

材料科学 · 物理学 2023-07-04 Xiong Xiong Liu , Shengfa Feng , Pengcheng Yuan , Yaping Wang , Long Pan , ZhengMing Sun

We use molecular dynamics simulations to explore the impact of a non-ionic solvent on the structural and capacitive properties of supercapacitors based on an ionic liquid electrolyte and carbon electrodes. The study is focused on two pure…

材料科学 · 物理学 2013-08-27 Céline Merlet , Mathieu Salanne , Benjamin Rotenberg , Paul A Madden

We measure gate-tuned thermoelectric power of mechanically exfoliated Bi2Se3 thin films in the topological insulator regime. The sign of the thermoelectric power changes across the charge neutrality point as the majority carrier type…

介观与纳米尺度物理 · 物理学 2015-03-12 Dohun Kim , Paul Syers , Nicholas P. Butch , Johnpierre Paglione , Michael S. Fuhrer

The conversion of heat into current can be obtained by a process with two stages. In the first one, the heat is used for distilling a solution and obtaining two flows with different concentrations. In the second stage, the two flows are…

化学物理 · 物理学 2014-03-18 M. Marino , L. Misuri , A. Carati , D. Brogioli

A nonequilibrium thermodynamic model is presented for the nonisothermal lithium-ion battery cell. Coupling coefficients, all significant for transport of heat, mass, charge and chemical reaction, were used to model profiles of temperature,…

化学物理 · 物理学 2024-11-25 Felix Schloms , Øystein Gullbrekken , Signe Kjelstrup

When plasmonic nanoparticles are coupled with semiconductors, highly energetic hot carriers can be extracted from the metal-semiconductor interface for various applications in light energy conversion. Hot charge-carrier extraction upon…

In situ electrochemical dilatometry was used to study, for the first time, the expansion behavior of a porous carbon electrode in a pure ionic liquid, 1-ethyl-3-methyl-imidazolium-tetrafluoroborate. For a single electrode, an applied…

化学物理 · 物理学 2013-06-11 F. Kaasik , T. Tamm , M. M. Hantel , E. Perre , A. Aabloo , E. Lust , M. Z. Bazant , V. Presser

Numerical simulations are a powerful tool for the development and improvement of Li-ion batteries. Modeling the mass transport of the involved electrolytic solutions requires precise determination of the corresponding electrolyte…

化学物理 · 物理学 2024-11-21 Lukas Lehnert , Maryam Nojabaee , Arnulf Latz , Birger Horstmann

Advanced supercapacitors have great potential to transform how we store and utilize energy, leading to more efficient and sustainable energy systems. This study reveals the structural features influencing the interfacial thermal transport…

应用物理 · 物理学 2024-02-20 Sobin Alosious , Shern R. Tee , Debra J. Searles

This work proposes a new variational, thermodynamically consistent model to predict thermal electrokinetics in electric double layer capacitors (EDLCs) by using an energetic variational approach. The least action principle and maximum…

化学物理 · 物理学 2022-08-15 Xiang Ji , Chun Liu , Pei Liu , Shenggao Zhou

Electrical and electrochemical processes in a bioactive soda-lime phosphosilicate glasses and in a bioabsorbable soda-lime phosphate glass during thermal poling were studied by means of thermally stimulated depolarization current…

材料科学 · 物理学 2007-09-04 C. R. Mariappan , B. Roling

An extremely efficient ethanol fuel cell electrode is produced by combining the large surface area of vertically oriented and highly conductive few-layer graphene sheets with electrochemically deposited palladium nanoparticles. The…

化学物理 · 物理学 2016-10-18 Michael Höltig , Charlotte Ruhmlieb , Tobias Kipp , Alf Mews

Interfacial thermal transport between electrodes and polymer electrolytes can play a crucial role in the thermal management of solid-state lithium-ion batteries (SLIBs). Modifying the electrode surface with functional molecules can…

介观与纳米尺度物理 · 物理学 2021-07-22 Siyu Tian , Dezhao Huang , Zhihao Xu , Shiwen Wu , Tengfei Luo , Guoping Xiong

Understanding charge storage in low-dimensional electrodes is crucial for developing novel ecologically friendly devices for capacitive energy storage and conversion, water desalination, etc. Exactly-solvable models allow in-depth analyses…

软凝聚态物质 · 物理学 2021-12-23 Taras Verkholyak , Andrij Kuzmak , Svyatoslav Kondrat

Electric capacitors are commonly used in electronic circuits for short-term storage of small amounts of energy. It is desirable however to use capacitors to store much larger energy amounts to replace rechargeable batteries. Unfortunately,…

介观与纳米尺度物理 · 物理学 2020-11-25 A. Bezryadin , A. Belkin , E. Ilin , M. Pak , Eugene V. Colla , A. Hubler