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The dynamics of the photoinduced commensurate to incommensurate charge density wave (CDW) phase transition in 4Hb-TaSe2 are investigated by femtosecond electron diffraction. In the perturbative regime the CDW reforms on a 150 ps timescale,…

强关联电子 · 物理学 2015-06-11 N. Erasmus , M. Eichberger , K. Haupt , I. Boshoff , G. Kassier , R. Birmurske , H. Berger , J. Demsar , H. Schwoerer

We report on a transient optical reflectivity study of the charge density wave (CDW) in CuxTiSe2 single crystals. Our measurements reveal that the system undergoes a quantum phase transition at x=0.04 from a strong commensurate CDW (x<0.04)…

强关联电子 · 物理学 2016-12-07 D. B. Lioi , R. D. Schaller , G. P. Wiederrecht , G. Karapetrov

Transport studies of atomically thin 1T-TaS2 have demonstrated the presence of intermediate resistance states across the nearly commensurate (NC) to commensurate (C) charge density wave (CDW) transition, which can be further switched…

Transitions between different charge density wave (CDW) states in quasi-two-dimensional materials may be accompanied also by changes in the inter-layer stacking of the CDW. Using MeV ultrafast electron diffraction, the out-of-plane stacking…

材料科学 · 物理学 2017-11-09 L. Le Guyader , T. Chase , A. Reid , R. K. Li , D. Svetin , X. Shen , T. Vecchione , X. J. Wang , D. Mihailovic , H. A. Dürr

In quasi-two-dimensional 1T-TaS2, a charge density wave (CDW) prototype, the transition occurs in two steps, from incommensurate (ICDW) and nearly commensurate (NCCDW) and from NCDW to commensurate (CCDW), locked in the resistivity…

强关联电子 · 物理学 2022-11-15 Sharon S. Philip , Despina Louca

We study the non-equilibrium structural dynamics of the incommensurate and nearly-commensurate charge-density wave phases in 1T-TaS$_2$. Employing ultrafast low-energy electron diffraction (ULEED) with 1 ps temporal resolution, we…

Transition metal dichalcogenides have been actively studied for their intriguing charge density wave (CDW) formations and their impacts on material properties. Among these, 1T-TiSe$_2$ is well-known to exhibit a 2$\times$2$\times$2 CDW…

材料科学 · 物理学 2025-09-09 Seungrok Mun , Woojin Choi , Hayoon Im , Sung-Kwan Mo , Choongyu Hwang , Jinwoong Hwang , Heung-Sik Kim

Charge density waves (CDWs), electronic crystals that form within a host solid, have long been speculated to melt into a spatially textured electronic liquid. Though they have not been previously detected, liquid CDWs may nonetheless be…

强关联电子 · 物理学 2025-05-09 Joshua S. H. Lee , Thomas M. Sutter , Goran Karapetrov , Pietro Musumeci , Anshul Kogar

Using temperature dependent Raman spectroscopy we address the question of how the transition from bulk to few atomic layers affects the charge density wave (CDW) phases in 1T-TaS2. We find that for crystals with thickness larger than approx…

介观与纳米尺度物理 · 物理学 2019-10-30 Adina Luican-Mayer , Jeffrey R. Guest , Saw-Wai Hla

Recent experiments suggest that excitonic degrees of freedom play an important role in precipitating the charge density wave (CDW) transition in $1T$-$\mathrm{TiSe}_2$. Through systematic calculations of the electronic and phonon spectrum…

介观与纳米尺度物理 · 物理学 2018-12-03 Chuan Chen , Bahadur Singh , Hsin Lin , Vitor M. Pereira

Transition metal dichalcogenides host a variety of charge density wave phases that couple lattice, charge, and correlation effects. In 1T-TaS2, the commensurate and nearly commensurate states are well characterized, yet the transition near…

Multiple charge density wave (CDW) phases in 2H-TaSe2 are investigated by high-resolution synchrotron x-ray diffraction. In a narrow temperature range immediately above the commensurate CDW transition, we observe a multi-q superstructure…

强关联电子 · 物理学 2015-03-17 Ph. Leininger , D. Chernyshov , A. Bosak , H. Berger , D. S. Inosov

Charge density waves (CDW) are states of broken symmetry with a periodic modulation of charge and lattice typically leading to the opening of a gap in the band structure. In the model CDW system 1T-TiSe$_2$ such a gap opens up between its…

We report a low-temperature scanning tunneling microscopy study of the charge density wave (CDW) order in 1$T$-TiSe$_2$ and Cu$_{0.08}$TiSe$_2$. In pristine 1$T$-TiSe$_2$ we observe a long-range coherent commensurate CDW (C-CDW) order. In…

超导电性 · 物理学 2017-03-14 Shichao Yan , Davide Iaia , Emilia Morosan , Eduardo Fradkin , Peter Abbamonte , Vidya Madhavan

In this work, we study the out-of-equilibrium dynamics of the paradigmatic quasi-one-dimensional material (TaSe$_4$)$_2$I, that exhibits a transition into an incommensurate CDW phase when cooled just below room temperature, namely at…

CuTe is a two-dimensional (2D) layered material, yet forming a quasi-one-dimensional (quasi-1D) charge-density-wave (CDW) along the a-axis in the ab-plane at high transition temperature $T_{CDW}=335$ K. However, the anisotropic properties…

强关联电子 · 物理学 2022-03-03 R. S. Li , L. Yue , Q. Wu , S. X. Xu , Q. M. Liu , Z. X. Wang , T. C. Hu , X. Y. Zhuo , L. Y. Shi , S. J. Zhang , D. Wu , T. Dong , N. L. Wang

Bulk 1T-TaSe2 exhibits unusually high charge density wave (CDW) transition temperatures of 600 K and 473 K below which the material exists in the incommensurate (I-CDW) and the commensurate (C-CDW) charge-density-wave phases, respectively.…

介观与纳米尺度物理 · 物理学 2015-08-19 R. Samnakay , D. Wickramaratne , T. R. Pope , R. K. Lake , T. T. Salguero , A. A. Balandin

The complex phase diagram of 1T-TiSe2 consists of a charge density wave (CDW) below 200 K, and CDW fluctuations of still unknown origin at higher temperatures. Here, we use time-resolved extreme ultraviolet momentum microscopy and density…

We report temperature-dependent transport and x-ray diffraction measurements of the influence of Ti hole doping on the charge density wave (CDW) in 1T-Ta(1-x)Ti(x)S(2). Confirming past studies, we find that even trace impurities eliminate…

Ultra-thin 2D materials have shown complete paradigm shift of understanding of physical and electronic properties because of confinement effects, symmetry breaking and novel phenomena at nanoscale. Bulk 2H-TaS2 undergoes an incommensurate…

介观与纳米尺度物理 · 物理学 2023-07-18 Divya Rawat , Aksa Thomas , Ajay Soni
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