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The high-pressure phases of FeO and MnO were studied by the first principles calculations. The present theoretical study predicts that the high-pressure phase of MnO is a metallic normal B8 structure (nB8), while that of FeO should take the…

材料科学 · 物理学 2009-10-30 Z. Fang , K. Terakura , H. Sawada , T. Miyazaki , I. Solovyev

The recent discovery of superconductivity in La$_3$Ni$_2$O$_7$ and La$_4$Ni$_3$O$_{10}$ under high pressure stimulates intensive research interests. These nickelates crystallize in an orthogonal/monoclinic structure with tilted NiO$_6$…

We investigate a range of possible materials containing the supermolecular form of hydrogen comprising 13 hydrogen molecules arranged in an icosahedral arrangement. This supermolecule consists of freely rotating 12 hydrogen molecules in an…

材料科学 · 物理学 2019-05-10 Graeme J. Ackland , Jack Binns , Ross Howie , Miguel Martinez-Canales

Pressure is a unique tuning parameter for probing the properties of materials and has been particularly useful for studies of electronic materials such as high-temperature cuprate superconductors. Here we report the effects of…

Magnetic properties of the conduction pi-electron system of kappa-BETS)2Mn[N(CN)2]3 have been probed using 13C NMR. At ambient pressure, the metal-insulator transition observed in the resistivity measurements below T~23K is shown to be…

强关联电子 · 物理学 2015-06-04 O. M. Vyaselev , M. V. Kartsovnik , N. D. Kushch , E. B. Yagubskii

Room-temperature superconductivity has been a long-standing goal for scientific progress and human development. Thermodynamic stability is a prerequisite for material synthesis and application. Here, we perform a combination of…

超导电性 · 物理学 2025-01-03 Decheng An , Defang Duan , Zihan Zhang , Qiwen Jiang , Hao Song , Tian Cui

We performed large-scale molecular dynamics simulations based on a machine-learning force field (MLFF) to investigate the Li-ion transport mechanism in cation-disordered Li$_3$TiCl$_6$ cathode at six different temperatures, ranging from…

材料科学 · 物理学 2024-06-19 Selva Chandrasekaran Selvaraj , Volodymyr Koverga , Anh T. Ngo

Small single crystals of Rb$_3$Ni$_2$(NO$_3$)$_7$ were obtained by crystallization from anhydrous nitric acid solution of rubidium nitrate and nickel nitrate hexahydrate. The basic elements of the crystal structure of this new compound are…

Binary metal sulfides are potential material family for exploring high Tc superconductors under high pressure. In this work, we study the crystal structures, electronic structures and superconducting properties of the Lu-S system in the…

超导电性 · 物理学 2023-12-25 Juefei Wu , Bangshuai Zhu , Chi Ding , Dexi Shao , Cuiying Pei , Qi Wang , Jian Sun , Yanpeng Qi

A new-type structural transition has been found in Li2RuO3 with honeycomb lattice of edge-sharing RuO6-octahedra. With decreasing temperature T, the electrical resistivity exhibits an anomalous increase at T=Tc~540 K, suggesting the (metal…

强关联电子 · 物理学 2015-06-25 Yoko Miura , Yukio Yasui , Masatoshi Sato , Naoki Igawa , Kazuhisa Kakurai

Results of a first-principles study of the Li impurity in GaN are presented. We find Li is a channel interstitial, with an onset for diffusion at T$\sim$ 600 K. Above this temperature, Li can transform to a Ga-substitutional acceptor by…

材料科学 · 物理学 2007-05-23 Fabio Bernardini , Vincenzo Fiorentini

Using ab initio evolutionary simulations, we explore all the possible stoichiometries for Mg-O system at pressures up to 850 GPa. In addition to MgO, our calculations find that two extraordinary compounds MgO2 and Mg3O2 become…

材料科学 · 物理学 2012-12-05 Qiang Zhu , Artem R. Oganov , Andriy O. Lyakhov

Lithium, a prototypical simple metal under ambient conditions, has a surprisingly rich phase diagram under pressure, taking up several structures with reduced symmetry, low coordination numbers, and even semiconducting character with…

材料科学 · 物理学 2019-04-26 Stephanie A. Mack , Sinéad M. Griffin , Jeffrey B. Neaton

The discovery of superconductivity under high pressure with $T_c$ exceeding 80 K in a bilayer nickelate La$_3$Ni$_2$O$_7$ has led to a strong desire to realize similar high $T_c$ phenomena at ambient pressure. As one possible path toward…

超导电性 · 物理学 2025-02-20 Masayuki Ochi , Hirofumi Sakakibara , Hidetomo Usui , Kazuhiko Kuroki

First-principles calculations within the density functional theory (DFT) with GGA-PBE exchange-correlation scheme have been employed to predict the structural, the elastic and the electronic properties of newly discovered lithium silicide…

The newest homologous series of superconducting As-pnictides, LiFeAs (Li111) and NaFeAs (Na111) have been synthesized and investigated. Both crystallize with the layered tetragonal anti-PbFCl-type structure in P4/nmm space group.…

超导电性 · 物理学 2015-05-13 C. W. Chu , F. Chen , M. Gooch , A. M. Guloy , B. Lorenz , B. Lv , K. Sasmal , Z. J. Tang , J. H. Tapp , Y. Y. Xue

Motivated by the recent discovery of superconductivity in La$_3$Ni$_2$O$_7$ under high pressure, we explore its potential charge and spin instabilities through combined model analysis and first-principles calculations. Taking into account…

超导电性 · 物理学 2025-01-24 Xuejiao Chen , Peiheng Jiang , Jie Li , Zhicheng Zhong , Yi Lu

Intermetallic compounds with sizable band gaps are attractive for their unusual properties but rare. Here, we present a new family of stable semiconducting quaternary Heusler compounds, designed and discovered by means of high-throughput…

材料科学 · 物理学 2018-02-15 Jiangang He , S. Shahab Naghavi , Vinay I. Hegde , Maximilian Amsler , Chris Wolverton

We perform a systematic \textit{ab initio} density functional study of the superconductivity, electronic and phononic band structures, electron-phonon coupling and elastic constants of all four possible structures of niobium nitride…

超导电性 · 物理学 2023-08-15 K. Ramesh Babu , Guang-Yu Guo

Li containing transition metal oxides are known as good ionic conductors. Performing classical molecular dynamics simulations, the diffusion behavior of Li ions is investigated in crystalline and amorphous phases with the stoichiometries…

材料科学 · 物理学 2025-01-29 Daniel Mutter , Diego A. Pantano , Christian Elsässer , Daniel F. Urban
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