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A neutron scattering investigation of the magnetoelectric coupling in PbFe_{1/2}Nb_{1/2}O_{3} (PFN) has been undertaken. Ferroelectric order occurs below 400 K, as evidenced by the softening with temperature and subsequent recovery of the…

材料科学 · 物理学 2018-07-20 C. Stock , S. R. Dunsiger , R. A. Mole , X. Li , H. Luo

We find unusual temperature dependence of the ferromagnetic resonance (FMR) frequency $f_{\rm R}$ for the spin-reorientation (SR) transition, in which the easy axis changes depending on temperature, observed in the Nd permanent magnet,…

统计力学 · 物理学 2020-09-21 Masamichi Nishino , Seiji Miyashita

Hexagonal YMnO$_{3}$ is a prototype antiferromagnet which exhibits multiferroic behavior with the ferroelectric and magnetic transitions occurring at different temperatures. We observe an out-of-plane canting of the Mn$^{3+}$ magnetic…

We have studied the temperature dependence of the photoemission spectra of Pr$_{1-x}$Ca$_x$MnO$_3$ (PCMO) with $x=0.25$, 0.3 and 0.5. For $x=0.3$ and 0.5, we observed a gap in the low-temperature CE-type charge-ordered (CO) phase and a…

强关联电子 · 物理学 2009-11-13 K. Ebata , M. Hashimoto , K. Tanaka , A. Fujimori , Y. Tomioka , Y. Tokura

We report on TmMnO3 far infrared emissivity and reflectivity spectra from 1910 K to 4 K. At the highest temperature the number of infrared bands is lower than that predicted for centrosymmetric P63/mmc (D6h4) (Z=2) space group due high…

Ferroelectricity is observed in orthorhombic $HoMnO_3$ and $YMnO_3$ at the magnetic lock-in transitions into an E-type structure or an incommensurate phase with a temperature independent wave vector, respectively. In $HoMnO_3$ the…

强关联电子 · 物理学 2011-11-09 B. Lorenz , Y. Q. Wang , C. W. Chu

The low-temperature thermal conductivity (\kappa) of GdFeO_3 single crystals is found to be strongly dependent on magnetic field. The low-field \kappa (H) curves show two "dips" for H \parallel a and only one "dip" for H \parallel c, with…

强关联电子 · 物理学 2011-01-25 Z. Y. Zhao , X. M. Wang , C. Fan , W. Tao , X. G. Liu , W. P. Ke , F. B. Zhang , X. Zhao , X. F. Sun

The ZFC and FC magnetization dependence on temperature was measured for BiFeO3 ceramics at the applied magnetic field up to H=10T in 2K-1000K range. The antiferromagnetic order was detected from the hysteresis loops below the Neel…

材料科学 · 物理学 2013-05-15 B. Andrzejewski , A. Molak , B. Hilczer , A. Budziak , R. Bujakiewicz-Koronska

We have found a remarkable increase (up to 60 %) of the dielectric constant with the onset of magnetic order at 42 K in the metastable orthorhombic structures of YMnO3 and HoMnO3 that proves the existence of a strong magneto-dielectric…

强关联电子 · 物理学 2009-11-10 B. Lorenz , Y. Q. Wang , Y. Y. Sun , C. W. Chu

(NH$_4$)$_2$[FeCl$_5$(H$_2$O)], a member of the family of antiferromagnetic $A_2$[Fe$X_5$(H$_2$O)] compounds ($X$ = halide ion, $A$ = alkali metal or ammonium ion) is classified as a new multiferroic material. We report the onset of…

强关联电子 · 物理学 2015-06-16 M. Ackermann , D. Brüning , T. Lorenz , P. Becker , L. Bohatý

We report an ultrasonic investigation of the elastic moduli on a single crystal of hexagonal YMnO_3 as a function of temperature. Stiffening anomalies in the antiferromagnetic N\'eel state below T_N = 72.4 K are observed on all the four…

强关联电子 · 物理学 2007-08-07 Mario Poirier , Francis Laliberte , Loreynne Pinsard , Alexandre Revcolevschi

Using first-principles calculations, we study theoretically the stable 2H hexagonal structure of BaMnO3. We show that from the stable high temperature P63/mmc structure, the compound should exhibit an improper ferroelectric structural phase…

材料科学 · 物理学 2015-06-15 Julien Varignon , Philippe Ghosez

The magnetic, dielectric and structural properties of type-I multiferroic KNiPO$_4$ have been investigated by neutron powder diffraction, magnetization, dielectric and high temperature synchrotron-XRD measurements. Below the N\'{e}el…

FeRh has a phase transition from an antiferromagnetic state (low temperature) to a ferromagnetic state (high temperature) at 360 K. Various explanations for this behavior have been proposed over the past 20 years. However, many of the…

材料科学 · 物理学 2020-02-05 Brianne McGrath , Robert Camley , Karen Livesey

The orthovanadate DyVO3 crystal, known to exhibit multiple structural, spin and orbital ordering transitions, is presently investigated on the basis of magnetization, heat capacity, resistivity, dielectric and polarization measurements. Our…

强关联电子 · 物理学 2014-07-24 Q. Zhang , K. Singh , C. Simon , L. D. Tung , G. Balakrishnan , V. Hardy

Resonant x-ray scattering at the Dy $M_5$ and Ni $L_3$ absorption edges was used to probe the temperature and magnetic field dependence of magnetic order in epitaxial LaNiO$_3$-DyScO$_3$ superlattices. For superlattices with 2 unit cell…

The optical conductivity of the undoped PrMnO$_3$ manganite has been investigated in details at various temperatures between 300 and 4 K. Its low energy spectrum exhibits an optical gap, and is characterized by a single broad peak centered…

强关联电子 · 物理学 2007-05-23 R. Sopracase , G. Gruener , C. Autret-Lambert , V. Ta Phuoc , V. Brize , J. C. Soret

We use high-resolution angle-resolved photoemission spectroscopy (ARPES) and density functional theory (DFT) calculations to study the electronic and magnetic properties of La2Ni7, an itinerant magnetic system with a series of three…

Thin films and heterostructures of hexagonal manganites as promising multiferroic materials have attracted a considerable interest recently. We report structural transformations of high quality epitaxial h-TMO/YSZ(111) films, analyzed by…

强关联电子 · 物理学 2020-09-23 R. Mandal , M. Hirsbrunner , V. Roddatis , L. Schüler , U. Roß , S. Merten , V. Moshnyaga

The sequence of phase transitions in PbHf0.83Sn0.17O3 has been studied by THz, far infrared and Raman spectroscopies, revealing the complementary behaviour of both, polar and non-polar phonons and their impact on the transition lattice…