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In-plane temperature dependent dielectric behavior of BiFeO3 (BFO) as-grown thin films show diffuse but prominent phase transitions near 450 (+/-10) K and 550 K with dielectric loss temperature dependences that suggest skin layer effects.…

材料科学 · 物理学 2015-06-04 Ashok Kumar , J. F. Scott , R. Martinez , G. Srinivasan , R. S. Katiyar

Temperature-dependent FAR-infrared reflectivity spectra of partially ordered magnetodielectric La2CoMnO6 is presented, from room temperature up to 675 K. A clear first-ordered structural phase transition (SPT) from a monoclinic structure…

材料科学 · 物理学 2018-02-22 R. X. Silva , A. Nonato , R. L. Moreira , R. M. Almeida , C. W. A. Paschoal

We have studied the influence of antiferromagnetic ordering on the local dielectric moments of the MnO_5 and LuO_7 polyhedra by measuring neutron powder diffraction patterns of LuMnO_3 at temperatures near T_N. We show that the coupling is…

强关联电子 · 物理学 2009-11-10 Bas B. Van Aken , Thomas T. M. Palstra

The lattice dynamics of the $\rm YMnO_3$ magneto-electric compound has been investigated using density functional calculations, both in the ferroelectric and the paraelectric phases. The coherence between the computed and experimental data…

材料科学 · 物理学 2012-03-09 Julien Varignon , Sébastien Petit , Marie-Bernadette Lepetit

Hexagonal HoMnO$_{3}$ is a frustrated antiferromagnet (T$_{N}$=72 K) ferroelectric (T$_{C}$=875 K) in which these two order parameters are coupled. Our neutron measurements of the spin wave dispersion for the S=2 Mn$^{3+}$ on the layered…

强关联电子 · 物理学 2009-11-11 O. P. Vajk , M. Kenzelmann , J. W. Lynn , S. B. Kim , S. -W. Cheong

Dielectric measurements on 0.65[Pb(Ni_1/3Nb_2/3)O_3]-0.35PbTiO_3 ceramic in the temperature range 90K to 470K shows a relaxor ferroelectric transition around 350K with a Vogel-Fulcher freezing temperature of 338K and appearance of a…

材料科学 · 物理学 2007-06-08 Satendra Pal Singh , Akhilesh Kumar Singh , Dhananjai Pandey , S. M. Yusuf

We have studied the thermodynamic properties of a multiferroic that couples ferromagnetic and ferroelectric order. Some of the results are independent of the form of the free energy. We calculate the temperature dependence of the electric,…

材料科学 · 物理学 2011-01-31 G. R. Boyd , P. Kumar , S. R. Phillpot

Temperature (5--250 K) and magnetic field (0--70 kOe) variations of the low-energy (1--10 meV) electrodynamics of spin excitations have been investigated for a complete set of light-polarization configurations for a ferroelectric magnet…

材料科学 · 物理学 2009-11-13 N. Kida , Y. Ikebe , Y. Takahashi , J. P. He , Y. Kaneko , Y. Yamasaki , R. Shimano , T. Arima , N. Nagaosa , Y. Tokura

We report complex dielectric and Raman spectroscopy measurements in four samples of $\alpha$- Fe$_2$O$_3$, consisting of crystallites which are either hexagonal shaped plates or cuboids. All four samples exhibit the spin reorientation…

强关联电子 · 物理学 2019-04-17 Namrata Pattanayak , Jitender Kumar , Partha Pratim Patra , G. V. Pavan Kumar , Ashna Bajpai

The temperature dependence of electronic and magnetic properties of the organic charge-transfer salt (DOEO)$_4$[HgBr$_4$]TCE was investigated using magnetometry. Electronic transport properties revealed three distinct phases which are…

We report results of the Raman measurements for SrRu$_2$O$_6$ having extraordinary high N$\acute{\textrm{e}}$el temperature for a layered material. No additional phonon modes were detected at the temperature of magnetic transition thus…

材料科学 · 物理学 2019-02-13 Yu. S. Ponosov , E. V. Komleva , D. A. Zamyatin , R. I. Walton , S. V. Streltsov

Epitaxial strain in thin films can yield surprising magnetic and electronic properties not accessible in bulk. One materials system destined to be explored in this direction are orthoferrites with two intertwined spin systems where strain…

We investigate the demagnetization dynamics of the cycloidal and sinusoidal phases of multiferroic TbMnO$_3$ by means of time-resolved resonant soft x-ray diffraction following excitation by an optical pump. Using orthogonal linear x-ray…

Low-energy magnon excitations in multiferroic BiFeO$_3$ were measured in detail as a function of temperature around several Brillouin zone centers by inelastic neutron scattering experiments on single crystals. Unique features around 1 meV…

The ferroelectric phase of the multiferroic hexagonal manganites (h-ReMnO3) has been reported to undergo a series of magnetic transitions involving long-range ordering/reorientation of 4fRe3+ and/or 3dMn3+ spins below room temperature.…

We have investigated magnetoelastic effects in multiferroic HoMnO$_3$ below the antiferromagnetic phase transition $T_N \approx 75$ K by neutron powder diffraction. The lattice parameter $a$ of the hexagonal unit cell of HoMnO$_3$ decrease…

强关联电子 · 物理学 2014-01-08 Tapan Chatterji , Thomas Hansen , Simon A. J. Kimber , Dipten Bhattacharya

We have recently reported that the Haldane spin-chain system, Er2BaNiO5, undergoing antiferromagnetic order below 32 K, is characterized by the onset of ferroelectricity near 60K due to magnetoelectric coupling induced by short-range…

强关联电子 · 物理学 2015-06-22 Tathamay Basu , Kiran Singh , N. Mohapatra , E. V. Sampathkumaran

The coupling between localized spins and phonons can lead to shifts in the dielectric constant of insulating materials at magnetic ordering transitions. Studies on isostructural SeCuO3 (ferromagnetic) and TeCuO3 (antiferromagnetic)…

材料科学 · 物理学 2009-04-14 G. Lawes , T. Kimura , C. M. Varma , M. A. Subramanian , R. J. Cava , A. P. Ramirez

The AFMR spectra of the NdFe$_3$(BO$_3$)$_4$ crystal are measured in a wide range of frequencies and temperatures. It is found that by the type of magnetic anisotropy the compound is an "easy-plane" antiferromagnet with a weak anisotropy in…

We report an infrared reflection spectroscopy study of La$_{1/2}$Ca$_{1/2}$MnO$_3$ over a broad frequency range and temperature interval which covers the transitions from the high temperature paramagnetic to ferromagnetic and, upon further…

强关联电子 · 物理学 2009-11-10 A. P. Litvinchuk , M. N. Iliev , M. Pissas , C. W. Chu