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In the pyrochlore compounds, Tb$_2$Ti$_2$O$_7$ and Tb$_2$Sn$_2$O$_7$, only the Tb$^{3+}$ ions are magnetic. They exhibit quite abnormal -- and, in view of their chemical similarity, strikingly different -- magnetic behaviour, as probed by…

强关联电子 · 物理学 2009-11-11 I. Mirebeau , A. Apetrei , I. N. Goncharenko , R. Moessner

We report the discovery of a spin one diamond lattice in NiRh2O4. This spinel undergoes a cubic to tetragonal phase transition at T = 440 K that leaves all nearest neighbor interactions equivalent. In the tetragonal phase, magnetization…

强关联电子 · 物理学 2018-03-30 J. R. Chamorro , L. Ge , J. Flynn , M. Subramanian , M. Mourigal , T. M. McQueen

Geometrical frustration among interacting spins combined with strong quantum fluctuations destabilize long-range magnetic order in favour of more exotic states such as spin liquids. By following this guiding principle, a number of spin…

Motivated by recent experiments on material Ba3NiSb2O9, we propose two novel spin liquid phases (A and B) for spin-1 systems on a triangular lattice. At the mean field level, both spin liquid phases have gapless fermionic spinon excitations…

强关联电子 · 物理学 2013-05-30 Cenke Xu , Fa Wang , Yang Qi , Leon Balents , Matthew P. A. Fisher

YbMgGaO$_{4}$, a structurally perfect two-dimensional triangular lattice with odd number of electrons per unit cell and spin-orbit entangled effective spin-1/2 local moments of Yb$^{3+}$ ions, is likely to experimentally realize the quantum…

强关联电子 · 物理学 2015-10-20 Yuesheng Li , Gang Chen , Wei Tong , Li Pi , Juanjuan Liu , Zhaorong Yang , Xiaoqun Wang , Qingming Zhang

Low-temperature states of polycrystalline samples of a frustrated pyrochlore oxide Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been investigated by specific heat, magnetic susceptibility, and neutron scattering experiments. We have found that this…

We present an interpretation of zero field diffuse neutron scattering and of high field magnetisation data at very low temperature in the frustrated pyrochlore system Tb2Ti2O7. This material has antiferromagnetic exchange interactions and…

强关联电子 · 物理学 2013-12-16 P. Bonville , A. Gukasov , I. Mirebeau , S. Petit

The XY pyrochlore Yb$_2$Ti$_2$O$_7$, with pseudo spin 1/2 at the Yb$^{3+}$ site, has been celebrated as potential host for the quantum spin ice state. The substitution of non-magnetic Ti with Pt gives Yb$_2$Pt$_2$O$_7$, a system with…

The Tb$_2$Ti$_2$O$_7$ pyrochlore magnetic material is attracting much attention for its {\em spin liquid} state, failing to develop long range order down to 50 mK despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K. In this paper…

统计力学 · 物理学 2007-05-23 Hamid R. Molavian , Michel J. P. Gingras , Benjamin Canals

Inelastic neutron scattering studies in single crystals of TbInO3 and TbIn0.95Mn0.05O3 with nearly-triangular antiferromagnetic lattice are reported. At low energies, a broad and apparently gapless continuum of magnetic excitations, located…

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

强关联电子 · 物理学 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

We present high-resolution single crystal time-of-flight neutron scattering measurements on the candidate quantum spin liquid pyrochlore Tb2Ti2O7 at low temperature and in a magnetic field. At ~70 mK and in zero field, Tb2Ti2O7 reveals…

强关联电子 · 物理学 2013-04-16 K. Fritsch , K. A. Ross , Y. Qiu , J. R. D. Copley , T. Guidi , R. I. Bewley , H. A. Dabkowska , B. D. Gaulin

Magnetic properties and magnetic structure of the Ba$_{2}$Mn(PO$_{4}$)$_{2}$ antiferromagnet featuring frustrated zigzag chains of $S=\frac{5}{2}$ Mn$^{2+}$ ions are reported based on neutron diffraction, density-functional band-structure…

强关联电子 · 物理学 2018-04-10 Arvind Yogi , A. K. Bera , Ashwin Mohan , Ruta Kulkarni , S. M. Yusuf , A. Hoser , A. A. Tsirlin , A. Thamizhavel

We use the projective symmetry group analysis to classify the quantum spin liquids on the $S=1/2$ pyrochlore magnet with a breathing anisotropy. We find 40 $\mathbb{Z}_2$ spin liquids and 16 $U(1)$ spin liquids that respect the $F\bar{4}3m$…

强关联电子 · 物理学 2022-11-17 Li Ern Chern , Yong Baek Kim , Claudio Castelnovo

We report the low temperature magnetic properties of Ce$_2$Sn$_2$O$_7$, a rare-earth pyrochlore. Our susceptibility and magnetization measurements show that due to the thermal isolation of a Kramers doublet ground state, Ce$_2$Sn$_2$O$_7$…

强关联电子 · 物理学 2016-08-15 Romain Sibille , Elsa Lhotel , Vladimir Pomjakushin , Chris Baines , Tom Fennell , Michel Kenzelmann

NMR studies have been carried out on a single crystal sample of TbBaCo2O5.5 with the oxygen-deficient perovskite structure. We have also carried out neutron diffraction studies and added new results to our previously published data. By…

强关联电子 · 物理学 2009-11-11 Minoru Soda , Yukio Yasui , Yoshiaki Kobayashi , Toshiaki Fujita , Masatoshi Sato , Kazuhisa Kakurai

Neutron scattering and magnetization measurements have been performed on the stuffed pyrochlore system Tb2+xTi2-2xNbxO7. We find that despite the introduction of chemical disorder and increasingly antiferromagnetic interactions, a spin…

Tb2Ti2O7 is a pyrochlore antiferromagnet that has dynamical spins and only short-range correlations even at 50 mK; the lowest temperature explored so far, which is much smaller than the scale set by the Curie-Weiss temperature T_{CW}~14 K.…

统计力学 · 物理学 2009-12-16 Hamid R. Molavian , Paul A. McClarty , Michel J. P. Gingras

Here we have experimentally demonstrated spin-correlation-driven ferroelectric quantum criticality in a prototype quantum spin-liquid system, Ba3CuSb2O9, a quantum phenomenon rarely observed. The dielectric constant follows a clear T2…

强关联电子 · 物理学 2026-04-01 Sayan Ghosh , Gourab Roy , Ekta Kushwaha , Mohit Kumar , Tathamay Basu

Motivated by the recent proposal of the spinon Fermi surface spin liquids for several candidate materials such as YbMgGaO4, we explore the experimental consequences of the external magnetic fields on this exotic state. Specifically, we…

强关联电子 · 物理学 2017-08-22 Yao Dong Li , Gang Chen