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Evolution of composite spin-orbital order and coupled spin-orbital excitations is studied in a variety of $d^4$ systems with $n$=$4$ electrons in the $t_{2g}$ orbital sector using the generalised self-consistent + fluctuations approach for…

强关联电子 · 物理学 2025-04-30 Shahid Ahmad , Harshvardhan Parmar , Shubhajyoti Mohapatra , Avinash Singh

Given that energy scales associated with crystal field splitting, spin orbit coupling and coulomb correlations in iridates are comparable, hence leading to exotic properties, we investigate the physical properties of orthorhombic SrIrO3…

材料科学 · 物理学 2015-07-23 Vijeta Singh , J. J. Pulikkotil

Resonant inelastic X-ray scattering (RIXS) is a powerful probe of elementary excitations in solids. It is now widely applied to study magnetic excitations. However, its complex cross-section means that RIXS has been more difficult to…

强关联电子 · 物理学 2021-06-30 H. C. Robarts , M. Garcia-Fernandez , J. Li , A. Nag , A. C. Walters , N. E. Headings , S. M. Hayden , Ke-Jin Zhou

Tailoring spin-orbit interactions and Coulomb repulsion are the key features to observe exotic physical phenomena such as magnetic anisotropy and topological spin texture at oxide interfaces. Our study proposes a novel platform for…

Based on the microscopic model including strong spin-orbit coupling, on-site Coulomb and Hund's interactions, as well as crystal field effects, we have investigated magnetic and optical properties of Sr2IrO4. Taking into account all…

强关联电子 · 物理学 2012-12-11 Beom Hyun Kim , G. Khaliullin , B. I. Min

Strongly correlated ground states and exotic quasiparticle excitations in low-dimensional systems are central research topics in the solid state research community. The present work develops a new layered material and explores the physical…

强关联电子 · 物理学 2023-02-09 Xianghan Xu , Guangming Cheng , Danrui Ni , Xin Gui , Weiwei Xie , Nan Yao , R. J. Cava

The electronic structure and magnetism of Sr$_2$CeIrO$_6$, an Ir-based double perovskite system has been investigated using first-principles calculations. We found that a strong spin-orbit coupling dictate the electronic and magnetic…

强关联电子 · 物理学 2013-01-29 S. K. Panda , I. Dasgupta

Neutron powder diffraction and inelastic measurements were performed examining the 5d pyrochlore Y$_2$Ir$_2$O$_7$. Temperature dependent measurements were performed between 3.4 K and 290 K, spanning the magnetic transition at 155 K. No sign…

强关联电子 · 物理学 2014-05-30 M. C. Shapiro , S. C. Riggs , M. B. Stone , C. R. de la Cruz , S. Chi , A. A. Podlesnyak , I. R. Fisher

Spin orbit coupling provides a mechanism to lock the momentum of electron to its spin degree, recent years was revealed to be essential in arousing many novel physical behaviors. SrIrO3 is a typical metallic member of the strong spin orbit…

材料科学 · 物理学 2018-08-10 Lunyong Zhang , Bin Pang , Y. B. Chen , Yanfeng Chen

We report on thermodynamic, magnetization, and muon spin relaxation measurements of the strong spin-orbit coupled iridate Ba$_3$IrTi$_2$O$_9$, which constitutes a new frustration motif made up a mixture of edge- and corner-sharing…

强关联电子 · 物理学 2017-09-13 W. -J. Lee , S. -H. Do , Sungwon Yoon , S. Lee , Y. S. Choi , D. J. Jang , M. Brando , M. Lee , E. S. Choi , S. Ji , Z. H. Jang , B. J. Suh , K. -Y. Choi

We report on the spin structure of the pyrochlore iridate Nd$_2$Ir$_2$O$_7$ that could be directly determined by means of powder neutron diffraction. Our magnetic structure refinement unravels a so-called all-in/all-out magnetic structure…

强关联电子 · 物理学 2016-10-14 H. Guo , C. Ritter , A. C. Komarek

The electronic and magnetic properties of Ba$_5$AlIr$_2$O$_{11}$ containing Ir-Ir dimers are investigated using the GGA and GGA+SOC calculations. We found that strong suppression of the magnetic moment in this compound recently found in [J.…

强关联电子 · 物理学 2017-08-02 S. V. Streltsov , G. Cao , D. I. Khomskii

The magnetoelectric (ME) effects are investigated in a cubic compound SrCuTe2O6, in which uniform Cu2+ (S=1/2) spin chains with considerable spin frustration exhibit a concomitant antiferromagnetic transition and dielectric constant peak at…

材料科学 · 物理学 2016-03-16 B. Koteswararao , Kyongjun Yoo , F. C. Chou , Kee Hoon Kim

Resonant inelastic X-ray scattering measurements reveal robust magnetic excitations in the perovskite iridates SrIr$_{1-x}$Sn$_x$O$_3$. We analyzed the dispersions of the magnetic excitation with spin-dilution ratio $x$ = 0, 0.03, 0.06,…

强关联电子 · 物理学 2026-04-14 Xiang Li , Yifan Jiang , Yuan Wan , Xuerong Liu

Transition metal oxides with 4d or 5d metals are of great interest due to the competing interactions, of the Coulomb repulsion and the itineracy of the d-electrons, opening a possibility of building new quantum ground states. Particularly…

强关联电子 · 物理学 2016-10-19 Katharina Rolfs , Ekaterina Pomjakushina , Denis Sheptyakov , Kazimierz Conder

We have systematically investigated substrate-strain effects on the electronic structures of two representative Sr-iridates, a correlated-insulator Sr$_2$IrO$_4$ and a metal SrIrO$_3$. Optical conductivities obtained by the \emph{ab initio}…

材料科学 · 物理学 2016-06-07 Bongjae Kim , Beom Hyun Kim , Kyoo Kim , B. I. Min

The single crystalline form of an insulator, Sr$_3$CuIrO$_{6+\delta}$, is shown to exhibit unexpectedly more than one magnetic transition (at 5 and 19 K) with spin-glass-like magnetic susceptibility behaviour. On the basis of this finding,…

强关联电子 · 物理学 2009-11-07 Asad Niazi , P. L. Paulose , E. V. Sampathkumaran

We study the magnetic excitations in 5d transition-metal oxide Sr$_2$IrO$_4$ on the basis of the Heisenberg model with small anisotropic terms on a square lattice. We calculate the correlation functions by using the Green's functions in the…

强关联电子 · 物理学 2015-06-18 Jun-ichi Igarashi , Tatsuya Nagao

Iridium oxides have provided a playground to study novel phases originating from spin-orbit coupling and electron-electron interactions. Among them, the d-wave singlet superconductor was proposed for electron-doped Sr$_2$IrO$_4$, containing…

超导电性 · 物理学 2019-08-21 Austin W. Lindquist , Hae-Young Kee

An intriguing idea of spin-orbit Mott insulator has been proposed to explain magnetic insulating behavior in various iridates. This scenario relies on the strength of the spin-orbit coupling being comparable to electronic correlations, and…

强关联电子 · 物理学 2013-05-30 Jean-Michel Carter , Hae-Young Kee