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We present measurements of the dielectric response of quasi one-dimensional (TMTTF)2AsF6 in a wide temperature and frequency range. We provide a thorough characterization of the relaxational dynamics observed close to the ferroelectric-like…

强关联电子 · 物理学 2009-11-11 D. Staresinic , K. Biljakovic , P. Lunkenheimer , A. Loidl

We present experimental evidences for a ferro-electric transition in the family of quasi one- dimensional conductors (TMTTF)2X. We interpret this new transition in the frame of the combined Mott-Hubbard state taking into account the double…

强关联电子 · 物理学 2009-10-31 P. Monceau , F. Ya. Nad , S. Brazovskii

Conductivity and permittivity of the quasi-one-dimensionsional organic transfer salt (TMTTF)2PF6 have been measured at low frequencies (10^3-10^7 Hz) between room temperature down to below the temperature of transition into the spin-Peierls…

强关联电子 · 物理学 2009-10-31 F. Nad , P. Monceau , C. Carcel , J. M. Fabre

The correlation-driven Mott transition is commonly characterized by a drop in resistivity across the insulator-metal phase boundary; yet, the complex permittivity provides a deeper insight into the microscopic nature. We investigate the…

The family of molecular conductors TMTTF/TMTSF-X demonstrates almost all known electronic phases in parallel with a set of weak structural modifications of anion ordering and mysterious structureless transitions. Only in early 2000's their…

强关联电子 · 物理学 2007-05-23 Serguei Brazovskii

The phase diagram of the organic superconductor $\kappa$-(BEDT-TTF)$_2$Cu[N(CN)$_2$Cl has been investigated by ultrasonic velocity measurements under helium gas pressure. Different phase transitions were identified trough several elastic…

强关联电子 · 物理学 2009-11-07 D. Fournier , M. Poirier , M. Castonguay , K. Truong

The two-dimensional organic conductor $\alpha$-(BEDT-TTF)$_2$I$_3$ undergoes a metal-insulator transition at $T_{\rm CO}=135$ K due to electronic charge ordering. We have conducted time-resolved investigations of its electronic properties…

强关联电子 · 物理学 2016-06-15 Tobias Peterseim , Tomislav Ivek , Dieter Schweitzer , Martin Dressel

(TMTTF)2AsF6 undergoes two phase transitions upon cooling from 300 K. At Tco=103 K a charge-ordering (CO) occurs, and at Tsp(B=9 T)=11 K the material undergoes a spin-Peierls (SP) transition. Within the intermediate, CO phase, the charge…

强关联电子 · 物理学 2009-11-07 F. Zamborszky , W. Yu , W. Raas , S. E. Brown , B. Alavi , C. A. Merlic , A. Baur

We present key issues of related phenomenons of the Ferroelectricity and the Charge Disproportionation in organic metals. In (TMTTF_2X the dielectric susceptibility demonstrates clear cases of the ferroelectric and anti-ferroelectric phase…

强关联电子 · 物理学 2007-05-23 S. Brazovskii , P. Monceau , F. Nad

We report on dc and microwave experiments of the low-dimensional organic conductors (TMTSF)$_2$PF$_6$ and (TMTSF)$_2$ClO$_4$ along the $a$, $b^{\prime}$, and $c^*$ directions. In the normal state of (TMTSF)$_2$PF$_6$ below T=70 K, the dc…

强关联电子 · 物理学 2009-11-10 M. Dressel , K. Petukhov , B. Salameh , P. Zornoza , T. Giamarchi

We study the differential resistivity transition of two-dimensional superconducting arrays induced by an external driving current, in the presence of thermal fluctuations and a magnetic field corresponding to $f$ flux quantum per plaquette.…

超导电性 · 物理学 2018-09-26 Enzo Granato

We report the first comprehensive investigation of the organic superconductor (TMTSF)2PF6 in the vicinity of the endpoint of the spin density wave - metal phase transition where phase coexistence occurs. At low temperature, the transition…

Mysterious high temperature structureless transitions in (TMTTF)2X compounds have been discovered in mid 80's (Coulon, Lawersanne,vet al), but left unexplained and abandoned, together with other warnings from structural effects (Moret,…

强关联电子 · 物理学 2007-05-23 Serguei Brazovskii

High-resolution thermal expansion measurements have been performed for exploring the mysterious "structureless transition" in (TMTTF)$_{2}$X (X = PF$_{6}$ and AsF$_{6}$), where charge ordering at $T_{CO}$ coincides with the onset of…

强关联电子 · 物理学 2008-11-24 M. de Souza , P. Foury-Leylekian , A. Moradpour , J. -P. Pouget , M. Lang

By applying measurements of the dielectric constants and relative length changes to the dimerized molecular conductor $\kappa$-(BEDT-TTF)$_2$Hg(SCN)$_2$Cl, we provide evidence for order-disorder type electronic ferroelectricity which is…

We investigate the metallic transport in the organic superconductor (TMTSF)2PF6 under pressure within the framework of the spin density wave theory in the proximity of a Peierls quantum critical point (QCP). We use a simple transport model…

强关联电子 · 物理学 2013-03-28 H. Meier , P. Auban-Senzier , C. Pépin , D. Jérome

Magnetic properties in the quasi-one-dimensional organic salt (TMTTF)2SbF6 are investigated by 13C NMR under pressures. Antiferromagnetic phase transition at ambient pressure (AFI) is confirmed. Charge-ordering is suppressed by pressure and…

强关联电子 · 物理学 2015-05-30 F. Iwase , K. Sugiura , K. Furukawa , T. Nakamura

The switching dynamics of ferroelectric materials is a crucial intrinsic property which directly affects the operation and performance of ferroelectric devices. In conventional ferroelectric materials, the typical ferroelectric switching…

材料科学 · 物理学 2023-08-02 Ri He , Hua Wang , Fucai Liu , Shi Liu , Houfang Liu , Zhicheng Zhong

An organic Mott insulator, $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Cl, was investigated by resistance measurements under continuously controllable He gas pressure. The first-order Mott transition was demonstrated by observation of clear…

强关联电子 · 物理学 2009-11-10 F. Kagawa , T. Itou , K. Miyagawa , K. Kanoda

The electrical resistivity of the quasi-1D organic superconductor (TMTSF)2PF6 was recently measured at low temperature from the critical pressure needed to suppress the spin-density-wave state up to a pressure where superconductivity has…

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