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The oxygen adsorption and dissociation on pristine silicene surface are studied by use of first-principles in this letter. The oxygen adsorption and dissociation on pristine silicene surface are studied by use of first-principles in this…

介观与纳米尺度物理 · 物理学 2016-11-27 G. Liu , X. L. Lei , M. S. Wu , B. Xu , C. Y. OuYang

The oxygen dissociation and the oxidized structure on the pristine C3N monolayer in exposure to air are the inevitably critical issues for the C3N engineering and surface functionalization yet have not been revealed in detail. Using the…

材料科学 · 物理学 2022-12-28 Liang Zhao , Wenjin Luo , Zhijing Huang , Zihan Yan , Hui Jia , Wei Pei , Yusong Tu

We present a first-principles and tight-binding model study of silicane and germanane, the hydrogenated derivatives of two-dimensional silicene and germanene. We find that the materials are stable in freestanding form, analyse the orbital…

材料科学 · 物理学 2014-04-16 V. Zólyomi , J. R. Wallbank , V. I. Fal'ko

We present and discuss the results of ab initio DFT plane-wave supercell calculations of the atomic and molecular oxygen adsorption and diffusion on the LaMnO3 (001) surface which serves as a model material for a cathode of solid oxide fuel…

材料科学 · 物理学 2008-02-04 Eugene A. Kotomin , Yuri A. Mastrikov , Eugene Heifets , Joachim Maier

We study the interaction of H$_2$, O$_2$, CO, H$_2$O and OH molecules with the vacancy defects of graphene and silicene. Atoms around the bare vacancy reconstruct and specific chemically active sites are created. While H$_2$, O$_2$ and CO…

化学物理 · 物理学 2014-11-27 H. Hakan Gurel , V. Ongun Ozcelik , S. Ciraci

By performing first-principles molecular dynamics calculations, we systematically simulate the adsorption behavior of oxygen molecules on the clean and strained Pb(111) surfaces. The obtained molecular adsorption precursor state, and the…

材料科学 · 物理学 2011-10-28 Yu Yang , Ping Zhang

Using first-principles calculations within density functional theory we demonstrate that the adsorption of single oxygen atom results in significant electron transfer from graphene to oxygen. This strongly disturbs the charge landscape of…

材料科学 · 物理学 2015-06-11 M. Topsakal , S. Ciraci

The interstitial oxygen centers in silicon and germanium are reconsidered and compared in an analysis based on the first-principles total-energy determination of the potential-energy surface of the centers, and a calculation of their…

凝聚态物理 · 物理学 2007-05-23 Emilio Artacho , Felix Yndurain

Two dimensional allotropes of group IV substrates including silicene, germanene and stanene have recently attracted considerable attention in nanodevice fabrication industry. These materials involving the buckled structure have been…

材料科学 · 物理学 2017-04-17 B Mortazavi , O Rahaman , M Makaremi , A Dianat , G Cuniberti , T Rabczuk

The adsorption of atomic oxygen and its inclusion into subsurface sites on Ag(210) and Ag(410) surfaces have been investigated using density functional theory. We find that--in the absence of adatoms on the first metal layer--subsurface…

凝聚态物理 · 物理学 2009-11-10 A. Kokalj , N. Bonini , A. Dal Corso , S. de Gironcoli , S. Baroni

Using density-functional theory in combination with a thermodynamic formalism we calculate the relative stability of various structural models of the polar O-terminated (000-1)-O surface of ZnO. Model surfaces with different concentrations…

材料科学 · 物理学 2009-11-10 B. Meyer

Using first-principles Density Functional Theory calculations, we showed that electronic and magnetic properties of bare and Ti adatom adsorbed single-layer silicene and germanene, which are charged or exerted by a perpendicular electric…

介观与纳米尺度物理 · 物理学 2013-07-12 H. Hakan Gürel , V. Ongun Özçelik , S. Ciraci

We report a study of structural and electronic properties of a germanium layer on Al(111) using scanning tunneling microscopy (STM), low energy electron diffraction and core-level photoelectron spectroscopy. Experimental results show that a…

材料科学 · 物理学 2017-12-08 W. Wang , R. I. G. Uhrberg

The dissociation of a hydrogen molecule on MgO(001) films deposited on Mo(001) surface is investigated systematically using periodic density-functional theory method. The unusual adsorption behavior of heterolytic dissociative hydrogen…

化学物理 · 物理学 2016-04-29 Zhenjun Song , Hu Xu

The energy to desorb atomic oxygen from an interstellar dust grain surface, $E_{\rm des}$, is an important controlling parameter in gas-grain models; its value impacts the temperature range over which oxygen resides on a dust grain.…

星系天体物理 · 物理学 2015-06-23 Jiao He , Jianming Shi , Tyler Hopkins , Gianfranco Vidali , Michael J. Kaufman

Classical molecular dynamics simulations are used to study the structure of densified germanium dioxide ($GeO_2$). It is found that the coordination number of germanium changes with increasing density (pressure) while pressure released…

材料科学 · 物理学 2007-05-23 Matthieu Micoulaut

The structural, electronic and dynamical properties of a group of 2D germanium-based compounds, including GeC, GeN, GeO, GeSi, GeS, GeSe, and germanene, are investigated by employing first-principles calculations. The most stable structure…

We report static and dynamic first-principles calculations that provide atomistic pictures of the initial stage of the oxidation processes occurring at the ($11\bar20$) surface of 4H-SiC. Our results unveil reaction pathways and their…

材料科学 · 物理学 2017-02-15 Han Li , Yu-ichiro Matsushita , Mauro Boero , Atsushi Oshiyama

Silicene, germanene and stanene likely to graphene are atomic thick material with interesting properties. We employed first-principles density functional theory (DFT) calculations to investigate and compare the interaction of Na or Li ions…

材料科学 · 物理学 2017-04-17 B Mortazavi , A Dianat , G Cuniberti , T Rabczuk

First-principles DFT levels of calculations have been carried out in order to study the structural stability and electronic properties of hydrogen passivated graphene (H-graphene) clusters. Two different shaped clusters, rectangular and…

材料科学 · 物理学 2014-05-02 Deepak B Karki , Narayan P Adhikari
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