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Antiferromagnetic insulators on the diamond lattice are candidate materials to host exotic magnetic phenomena ranging from spin-orbital entanglement to degenerate spiral ground-states and topological paramagnetism. Compared to other…

强关联电子 · 物理学 2017-08-16 L. Ge , J. Flynn , J. A. M. Paddison , M. B. Stone , S. Calder , M. A. Subramanian , A. P. Ramirez , M. Mourigal

We report muSR experiments on Mg{x}Cu{4-x}(OH)6Cl2 with x \sim 1, a new material isostructural to Herbertsmithite exhibiting regular kagome planes of spin 1/2 (Cu^{2+}), and therefore a candidate for a spin liquid ground state. We evidence…

强关联电子 · 物理学 2014-10-06 E. Kermarrec , P. Mendels , F. Bert , R. H. Colman , A. S. Wills , P. Strobel , P. Bonville , A. Hillier , A. Amato

The magnetic subsystem of nabokoite, KCu$_7$(TeO$_4$)(SO$_4$)$_5$Cl, is constituted by copper ions forming a buckled square kagom\'e lattice decorated by quasi-isolated ions. This combination determines peculiar physical properties of this…

The structural and magnetic properties of a spin-$\frac{1}{2}$ averievite (CsBr)Cu$_5$V$_2$O$_{10}$ are investigated by means of temperature-dependent x-ray diffraction, magnetization, heat capacity, and $^{51}$V nuclear magnetic resonance…

材料科学 · 物理学 2024-11-12 S. Guchhait , D. V. Ambika , S. Mohanty , Y. Furukawa , R. Nath

Anisotropic magnetic properties of a layered kagome-like system Cu3Bi(SeO3)2O2Br have been studied by bulk magnetization and magnetic susceptibility measurements as well as powder and single-crystal neutron diffraction. At T_N = 27.4 K the…

强关联电子 · 物理学 2012-10-16 M. Pregelj , O. Zaharko , A. Günther , A. Loidl , V. Tsurkan , S. Guerrero

Quantum antiferromagnets based on the square-kagome lattice are proving to be a fertile platform for realizing nontrivial phenomena in frustrated magnetism. Recently, several decorated square-kagome compounds of the nabokoite family have…

强关联电子 · 物理学 2025-05-19 Matías G. Gonzalez , Yasir Iqbal , Johannes Reuther , Harald O. Jeschke

The spin wave excitations of the ideal S=5/2 Kagome lattice antiferromagnet KFe3(OH)6(SO4)2 have been measured using high-resolution inelastic neutron scattering. We directly observe a flat mode which corresponds to a lifted "zero energy…

强关联电子 · 物理学 2008-10-31 K. Matan , D. Grohol , D. G. Nocera , T. Yildirim , A. B. Harris , S. H. Lee , S. E. Nagler , Y. S. Lee

Metal-organic frameworks (MOFs), which are self-assemblies of metal ions and organic ligands, provide a tunable platform to search a new state of matter. A two-dimensional (2D) perfect kagome lattice, whose geometrical frustration is a key…

Cu(1,3-benzenedicarboxylate) [Cu(1,3-bdc)] contains structurally perfect kagom\'{e} planes formed by Cu$^{2+}$ ions without the presence of diamagnetic defects. This organometallic compound should have served as a precious platform to…

强关联电子 · 物理学 2015-10-07 Zheng Liu , Jia-Wei Mei , Feng Liu

We report a comprehensive muon spectroscopy study of the Zn-barlowite series of $S={\frac{1}{2}}$ kagom\'e antiferromagnets, Zn$_x$Cu$_{4-x}$(OH)$_{6}$FBr, for $x=0.00$ to $0.99(1)$. By combining muon spin relaxation and rotation…

强关联电子 · 物理学 2020-10-28 K. Tustain , B. Ward-O'Brien , F. Bert , T. -H. Han , H. Luetkens , T. Lancaster , B. M. Huddart , P. J. Baker , L. Clark

We report a single-crystal neutron diffraction and inelastic neutron scattering study on the spin 1/2 cuprate Cu$_3$Bi(SeO$_3$)$_2$O$_2$Cl, complemented by dielectric and electric polarization measurements. The study clarifies a number of…

We synthesized single crystals of the new hexagonal compounds A$_2$Cu$_3$SnF$_{12}$ with A=Cs and Rb, and investigated their magnetic properties. These compounds are composed of Kagom\'{e} layers of corner-sharing CuF$_6$-octahedra.…

强关联电子 · 物理学 2009-11-13 T. Ono , K. Morita , M. Yano , H. Tanaka , K. Fujii , H. Uekusa , Y. Narumi , K. Kindo

Hexagonal antiferromagnets Cs$_2$Cu$_3$MF$_{12}$ (M = Zr, Hf and Sn) have uniform Kagome lattices of Cu$^{2+}$ with S = 1/2, whereas Rb$_2$Cu$_3$SnF$_{12}$ has a 2a by 2a enlarged cell as compared with the uniform Kagome lattice. The…

强关联电子 · 物理学 2013-05-29 T. Ono , K. Morita , M. Yano , H. Tanaka , K. Fujii , H. Uekusa , Y. Narumi , K. Kindo

The mineral haydeeite, alpha-MgCu3(OD)6Cl2, is a S=1/2 kagome ferromagnet that displays long-range magnetic order below TC=4.2 K with a strongly reduced moment. Our inelastic neutron scattering data show clear spin-wave excitations that are…

强关联电子 · 物理学 2015-06-26 D. Boldrin , B. Fak , M. Enderle , S. Bieri , J. Ollivier , S. Rols , P. Manuel , A. S. Wills

Magnetic and crystallographic properties of the mineral langite Cu$_4$(OH)$_6$SO$_4\cdot 2$H$_2$O are reported. Its layered crystal structure features a peculiar spatial arrangement of spin-$\frac12$ Cu$^{2+}$ ions that arises from a…

强关联电子 · 物理学 2017-02-10 Stefan Lebernegg , Alexander A. Tsirlin , Oleg Janson , Günther J. Redhammer , Helge Rosner

The layered compound with distorted Kagome nets, Dy3Ru4Al12, was previously reported to undergo antiferromagnetic ordering below (TN=) 7 K, based on investigations on single crystals. Here, we report the results of our investigation of ac…

强关联电子 · 物理学 2016-05-05 Venkatesh Chandragiri , Kartik K Iyer , E. V. Sampathkumaran

We investigated the crystal structure of Rb$_2$Cu$_3$SnF$_{12}$ and its magnetic properties using single crystals. This compound is composed of Kagome layers of corner-sharing CuF$_{6}$ octahedra with a 2a x 2a enlarged cell as compared…

强关联电子 · 物理学 2009-11-13 K. Morita , M. Yano , T. Ono , H. Tanaka , K. Fujii , H. Uekusa , Y. Narumi , K. Kindo

Two kagome compounds, volborthite Cu3V2O7(OH)2-2H2O and herbertsmithite ZnCu3(OH)6Cl2, are compared in order to derive information about the intrinsic properties of the spin-1/2 kagome antiferromagnet. Volborthite shows a broad maximum at T…

强关联电子 · 物理学 2009-11-13 Z Hiroi , H Yoshida , Y Okamoto , M Takigawa

Cubic crystal structure and regular octahedral environment of Ir$^{4+}$ render antifluorite-type K$_2$IrCl$_6$ a model fcc antiferromagnet with a combination of Heisenberg and Kitaev exchange interactions. High-resolution synchrotron powder…

Kagome lattice Heisenberg antiferromagnets are known to be highly sensitive to perturbations caused by structural disorder. NMR is a local probe ideally suited for investigating such disorder-induced effects, but in practice large…

强关联电子 · 物理学 2023-01-09 Weishi Yuan , Jiaming Wang , Philip M. Singer , Rebecca W. Smaha , Jiajia Wen , Young S. Lee , Takashi Imai