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We performed Raman spectroscopy measurements under temperature changes from 10 K up to 850 K to probe the phonon-spin coupling in Y$_2$NiMnO$_6$. The spin-phonon coupling was observed as a softening of the stretching mode, indicating this…

In this paper, we present the spin-phonon coupling and dielectric response of nano-crystalline Pr$_2$CoMnO$_6$ employing Raman and dielectric spectroscopic study. Pr$_2$CoMnO$_6$ is a manganite compound , it undergoes a paramagnetic to…

强关联电子 · 物理学 2021-04-13 Ilyas Noor Bhatti , Imtiaz Noor Bhatti

Weak antiferromagnetic (AF) interaction in the ferromagnetic (FM) partially ordered La2CoMnO6 (LCMO) was detected by Raman spectroscopy by monitoring spin-phonon coupling. Because of the sensibility to probe short-range disorder and lattice…

材料科学 · 物理学 2022-05-17 R. X. Silva , C. C. Santos , H. Reichlova , X. Marti , R. Paniago , C. W. A. Paschoal

The temperature dependence of phonon excitations and the presence of spin phonon coupling in polycrystalline Pr2NiMnO6 samples were studied using micro-Raman spectroscopy and magnetometry. Magnetic properties show a single…

材料科学 · 物理学 2011-01-17 K. D. Truong , M. P. Singh , S. Jandl , P. Fournier

Raman study on a select few orthochromites, RCrO$_3$ (R = Y, Lu, Gd, Eu and Sm) shows that the phonon behavior at TN in compounds with magnetic R-ion (Gd and Sm) is remarkably different from that of non-magnetic R-ion (Y, Lu and Eu). While…

材料科学 · 物理学 2013-06-11 Venkata Srinu Bhadram , B. Rajeswaran , A. Sundaresan , Chandrabhas Narayana

We report the influence of Ni/Mn ordering on the spin-phonon coupling in multifunctional La2NiMnO6. Three types of films with different levels of structural order, including long-range Ni/Mn cation order, cation disorder, and an admixture…

材料科学 · 物理学 2015-05-14 K. D. Truong , M. P. Singh , S. Jandl , P. Fournier

We have investigated the temperature-dependent Raman-active phonons and the magnetic properties of Gd(Co1/2Mn1/2)O3 perovskite ceramics in the temperature range from 40 K to 300 K. The samples crystallized in an orthorhombic distorted…

Electronic structure near Fermi level of Pr2CoFeO6 (at 300 K) was investigated by X-ray photoemission spectroscopy (XPS) technique. All three cations, i.e., Pr, Co and Fe were found to be trivalent in nature. XPS analysis also suggested the…

Using first-principles density functional calculations, we study the electronic and magnetic properties of ferromagnetic insulating double-perovskite compound La2NiMnO6, which has been reported to exhibit interesting magnetic field…

材料科学 · 物理学 2008-05-09 Hena Das , Umesh V. Waghmare , T. Saha-Dasgupta , D. D. Sarma

Multifunctional properties in quantum systems require the interaction between different degrees of freedom. As such, spin-phonon coupling emerges as an ideal mechanism to tune multiferroicity, magnetism, and magnetoelectric response. In…

The effect of rare-earth ions (R = Er^{3+}, Tb^{3+}) with strong spin-orbit coupling on the dielectric properties and the electric polarization induced by local polar phase separation domains in RMn_2O_5 multiferroics has been studied.…

材料科学 · 物理学 2020-02-14 B. Kh. Khannanov , E. I. Golovenchits , V. A. Sanina

We demonstrate the coupling of rare-earth ions locally implanted in a substrate (Gd$^{3+}$ in Al$_{2}$O$_{3}$) to a superconducting NbN lumped-element micro-resonator. The hybrid device is fabricated by a controlled ion implantation of…

介观与纳米尺度物理 · 物理学 2015-06-22 I. Wisby , S. E. de Graaf , R. Gwilliam , A. Adamyan , S. Kubatkin , P. J. Meeson , A. Ya. Tzalenchuk , T. Lindström

The Griffiths phase-like features and the spin-phonon coupling effects observed in Tb$_2$NiMnO$_6$ are reported. The double perovskite compound crystallizes in monoclinic $P2_1/n$ space group and exhibits a magnetic phase transition at $T_c…

First-principles electronic structure calculations have been performed for the double perovskite Bi$_2$CoMnO$_6$ in its non-centrosymmetric polar state using generalized gradient approximation plus Hubbard U approach. We find that while Co…

材料科学 · 物理学 2010-10-25 Satadeep Bhattacharjee , Olle Eriksson , Biplab Sanyal

Infrared reflectivity spectra of cubic SrMnO$_{3}$ ceramics reveal 18 % stiffening of the lowest-frequency phonon below the antiferromagnetic phase transition occurring at T$_{N}$ = 233 K. Such a large temperature change of the polar phonon…

Temperature dependent Raman scattering measurements have been performed to explore unusual coupling between magnetism and crystal structure in doped pyrochlore iridate Y$_2$(Ir$_{1-x}$Ru$_x$)$_2$O$_7$ with $x$ = 0.0, 0.05 and 0.2. The…

强关联电子 · 物理学 2019-02-20 Harish Kumar , V. G. Sathe , A. K. Pramanik

Magnetoelectric phase diagrams of the rare-earth (R) Mn perovskites RMnO3 are theoretically studied by focusing on crucial roles of the symmetric magnetostriction or the Peierls-type spin-phonon coupling through extending our previous work…

强关联电子 · 物理学 2011-10-07 Masahito Mochizuki , Nobuo Furukawa , Naoto Nagaosa

Cr2Ge2Te6 has been of interest for decades, as it is one of only a few naturally forming ferromagnetic semiconductors. Recently, this material has been revisited due to its potential as a 2 dimensional semiconducting ferromagnet and a…

材料科学 · 物理学 2016-05-02 Yao Tian , Mason J. Gray , Huiwen Ji , R. J. Cava , Kenneth S. Burch

Two-dimensional metal-halide perovskites are highly versatile for light-driven applications due to their exceptional variety in material composition, which can be exploited for tunability of mechanical and optoelectronic properties. The…

The rise of high-entropy oxides as a major functional materials design principle in recent years has prompted us to investigate how compositional disorder affects long-range magnetic ordering in double perovskite oxides. Since ferromagnetic…

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