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Hybrid transition metal oxides continue to attract attention due to their multiple degrees of freedom ($e.g.$, lattice, charge, spin, and orbital) and versatile properties. Here we investigate the magnetic and electronic properties of the…

强关联电子 · 物理学 2022-05-17 Ke Yang , Wenjing Xu , Di Lu , Yuxuan Zhou , Lu Liu , Yaozhenghang Ma , Guangyu Wang , Hua Wu

We investigate the electronic and magnetic properties of the newly synthesized double perovskites Y$_{2}$NiIrO$_{6}$ and La$_{2}$NiIrO$_{6}$, using density functional calculations, crystal field theory, superexchange pictures, and Monte…

材料科学 · 物理学 2023-11-20 Lu Liu , Ke Yang , Di Lu , Yaozhenghang Ma , Yuxuan Zhou , Hua Wu

Double-perovskite oxides that contain both 3d and 5d transition metal elements have attracted growing interest as they provide a model system to study the interplay of strong electron interaction and large spin-orbit coupling (SOC). Here,…

Neutron diffraction on the double perovskite Sr2YRuO6 with a quasi-face-centered cubic (FCC) lattice of Ru moments reveals planar magnetic correlations that condense into a partial long-range ordered state with coupled alternate…

强关联电子 · 物理学 2015-06-11 E. Granado , J. W. Lynn , R. F. Jardim , M. S. Torikachvili

The double-perovskite A$_2$BB'O$_6$ with heavy transition metal ions on the ordered B' sites is an important family of compounds to study the interplay between electron correlation and spin-orbit coupling (SOC). Here we prepared…

强关联电子 · 物理学 2020-07-01 Shang Gao , Daigorou Hirai , Hajime Sagayama , Hiroyuki Ohsumi , Zenji Hiroi , Taka-hisa Arima

We studied structural and magnetic properties of a series of insulating double perovskite compounds, La$_{2-x}$Sr$_{x}$CuRuO$_{6}$ (0 $\le$ x $\le$ 1), representing doping via \textit{A}-site substitution. The end members…

Using density-functional theory calculations, we investigated the electronic structure and magnetic exchange interactions of the ordered 3d-5d double perovskite Sr2FeOsO6, which has recently drawn attention for interesting antiferromagnetic…

材料科学 · 物理学 2014-07-24 Sudipta Kanungo , Binghai Yan , Martin Jansen , Claudia Felser

We carry out a first-principles investigation on magnetism, electronic structure, magneto-optical effects and topological property of newly grown cubic double perovskite Ba2NiOsO6 and its (111) (Ba2NiOsO6)/(BaTiO3)10 superlattice, based on…

强关联电子 · 物理学 2019-10-02 Hai-Shuang Lu , Guang-Yu Guo

We report an experimental investigation of the two-dimensional ${J}_{\rm eff}$ = 1/2 antiferromagnetic Mott insulator by varying the interlayer exchange coupling in [(SrIrO$_3$)$_1$, (SrTiO$_3$)$_m$] ($m$ = 1, 2 and 3) superlattices.…

Coupling between different interactions allows to control physical aspects in multifunctional materials by perturbing any of the degrees of freedom. Here, we aim to probe the correlation among structural, electronic and magnetic observables…

We perform a comparative magnetic study on two series of rare-earth (RE) based double perovskite iridates RE2BIrO6 (RE=Pr,Nd,Sm-Gd;B=Zn,Mg), which show Mott insulating state with tunable charge energy gap from ~330 meV to ~560 meV by…

We have deployed density functional theory, Wannier function analysis and mean-field calculations to investigate the double-double perovskite compound CaMnCrSbO_{6}. The crystallographically non-equivalent Mn atoms in the unit cell have…

材料科学 · 物理学 2022-06-14 Rakshanda Dhawan , Padmanabhan Balasubramanian , Tashi Nautiyal

Magnetic double perovskite compounds provide a fertile playground to explore interesting electronic and magnetic properties. By complementary macroscopic characterizations, neutron powder diffraction measurements and first-principles…

强关联电子 · 物理学 2024-04-03 Cheng Su , Xu-Tao Zeng , Kaitong Sun , Denis Sheptyakov , Ziyu Chen , Xian-Lei Sheng , Haifeng Li , Wentao Jin

In this work, we report on the synthesis and magnetic properties of a series of double perovskites Ln$_2$ZnIrO$_6$ with Ln = Nd, Sm, Eu & Gd. These compounds present new examples of the rare case of double perovskites (general formula…

The structural, electronic and magnetic properties of anti-site disordered Sm$ _{2} $NiMnO$ _{6} $ double perovskite has been studied. RE$_{2}$NiMnO$_{6}$ (RE: rare-earth) ordered double perovskite is commonly believed to show two distinct…

材料科学 · 物理学 2025-07-28 S. Majumder , M. Tripathi , P. Rajput , S. N. Jha , R. J. Choudhary , D. M. Phase

Oxide double perovskites wherein octahedra formed by both 3d elements and sp-based heavy elements give rise to unconventional magnetic ordering and correlated quantum phenomena crucial for futuristic applications. Here, by carrying out…

We report electron spin resonance (ESR) spectroscopy results on the double perovskite Ba$_2$YIrO$_6$. On general grounds, this material is expected to be nonmagnetic due to the strong coupling of the spin and orbital momenta of Ir$^{5+}$…

强关联电子 · 物理学 2018-06-12 S. Fuchs , T. Dey , G. Aslan-Cansever , A. Maljuk , S. Wurmehl , B. Büchner , V. Kataev

The strong exchange interaction between 3$d$-4$f$ magnetic sublattice in rare-earth perovskites introduces a variety of complex magnetic states hosting fascinating electronic ground states with exotic properties. Especially when it comes to…

We study experimentally and theoretically the electronic and magnetic properties of two insulating double perovskites that show similar atomic and electronic structure, but different magnetic properties. In magnetization measurements,…

Insulating ferromagnets with high TC are required for many new magnetic devices. More complexity arises when strongly correlated 3d ions coexist with strongly spin-orbit coupled 5d ones in a double perovskite. Here, we perform the…

强关联电子 · 物理学 2019-07-30 Xingyu Zhang , Bin Li , Jie Cheng , Xu Chen , Lining Wang , Zilong Miu , Ziwan Song , Shengli Liu , Z. H. Wang
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