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We consider the reduced dynamics of a molecular chain weakly coupled to a phonon bath. With a small and constant inhomogeneity in the coupling, the excitation relaxation rates are obtained in closed form. They are dominated by transitions…
We present a theoretical study showing that an optically driven excitonic two-level system in a solid state environment acts as a heat pump by means of repeated phonon emission or absorption events. We derive a master equation for the…
The non-classical spectral and temporal features of entangled photons offer new possibilities to investigate the interactions of excitons in photosynthetic complexes, and to target the excitation of specific states. Simulations of…
Spontaneous vibrational Raman scattering is a ubiquitous form of light-matter interaction whose description necessitates quantization of the electromagnetic field. It is usually considered as an incoherent process because the scattered…
Coherence and de-coherence are the most fundamental steps that follow the initial photo-excitation occurring in typical Pump&Probe experiments. Indeed, the initial external laser pulse transfers coherence to the system in terms of creation…
The dissociation of excited electron-hole pairs is a microscopic process that is fundamental to the performance of photovoltaic systems. For this process to be successful, the oppositely charged electron and hole must overcome an…
We show that the phase difference of two overlapping ground state Bose-Einstein condensates can effect the optical spontaneous emission rate of excited atoms. Depending on the phase difference the atom stimulated spontaneous emission rate…
High-harmonic generation is a light up-conversion process occurring in a strong laser field, leading to coherent bursts of extreme ultrashort broadband radiation [1]. As a new perspective, we propose that ultrafast strong-field electronic…
The spectral and spatiotemporal dynamics of photoluminescence in monolayers of transition metal dichalcogenide WSe$_2$ obtained by mechanical exfoliation on a Si/SiO$_2$ substrate is studied over a wide range of temperatures and excitation…
We show that a pulsed stimulus can be used to generate many-body quantum coherences in light-matter systems of general size. Specifically, we calculate the exact real-time evolution of a driven, generic out-of-equilibrium system comprising…
The sequential resonant excitation of a 2-level quantum system results in the emission of a state of light showing time-entanglement encoded in the photon-number-basis - notions that can be extended to 3-level quantum systems as discussed…
The bound electron-hole pairs known as excitons govern the optical properties of insulating solids. While their behavior in equilibrium is well-understood theoretically, the nonequilibrium regime at high excitation densities-where phenomena…
The manipulation of molecular excited state processes through strong coupling has attracted significant interest for its potential to provide precise control of photochemical phenomena. However, the key limiting factor for achieving this…
We have developed a model accounting for the photo-excitation dynamics and the photoluminescence of strongly coupled J-aggregate microcavities. Our model is based on a description of the J-aggregate film as a disordered Frenkel exciton…
Photosynthetic light harvesting provides a natural blueprint for bioengineered and biomimetic solar energy and light detection technologies. Recent evidence suggests some individual light harvesting protein complexes (LHCs) and LHC subunits…
Extension of coherent response time is a desired goal in the field of all-optical information processing implemented in classical and quantum ways. Here we demonstrate how spin-dependent stimulated photon echo can be used to extend decay…
An excitonic insulator phase is expected to arise from the spontaneous formation of electron-hole pairs (excitons) in semiconductors where the exciton binding energy exceeds the size of the electronic band gap. At low temperature, these…
The dynamics of exciton and electron-hole plasma populations is studied via time-resolved photoluminescence after nonresonant excitation. By comparing the peak emission at the exciton resonance with the emission of the continuum, it is…
Periodically driven systems are a common topic in modern physics. In optical lattices specifically, driving is at the origin of many interesting phenomena. However, energy is not conserved in driven systems, and under periodic driving,…
We study the dynamics of an atomic two-level system decaying by spontaneous emission of light. Subject to continuous detection of the radiated field, the system tends with certainty to the ground state in the long time limit, but at initial…