相关论文: Emergence of molecular chirality due to chiral int…
We study the problem of stability of chiral states, also known as problem of chirality, within the framework of a two-dimensional approximation of a symmetric double-well potential. We show how the symmetry breaking of the potential due to…
In this work, we develop a system {\it plus} environment approach for interacting chiral molecules under a quantum-classical description of the spin-spin model using a Caldeira-Leggett-like coupling. After presenting the interacting model,…
We examine the effect of decoherence and intermolecular interactions (chiral discrimination energies) on the chiral stability and the distinguishability of initially pure versus mixed states in an open chiral system. Under a two-level…
We study the effective chiral interaction between molecules arising from quantum dispersion interactions within a model in which a) the dominant excited states of a molecule form a band whose width is small compared to the average…
We study in the framework of the Schrodinger equation the effect of intermolecular interactions on the tunneling racemization of the active molecule. The active molecule is assumed as a two-level system and the left-right isomerism is…
It has been long recognized that the spatial polarization of the electronic clouds in molecules, and the spatial arrangements of atoms into chiral molecular structures, play crucial roles in physics, chemistry and biology. However, these…
The presence of chirality in the main molecules of life may well be not just a structural artifact, but of pure biological advantage. The possibility of the existence of a phenomenon of a special mode of interaction, labeled as "chiral…
In plasmonic chirality, the phenomenon of circular dichroism for achiral nanoparitcles caused by Coulomb interaction between metal nanoparticles (NPs) and chiral molecules have been studied. At the same time, under the resonance condition,…
To understand the relationship between the chirality of individual cells and that of tissues and organisms, we have developed a chiral polarized particle model to investigate the movement of cell populations on substrates. Our model…
The superposition of chiral states of chiral molecules, as delocalized quantum states of a many-particle system, can be used for the experimental investigations of decoherence theory. In this regard, a great challenge is the precise…
We investigate the interplay between chirality and confinement in harmonically trapped active particles. The circular character of chiral motion combines with the radial symmetry of the potential to create distinctive non-equilibrium…
Strong-field ionization by counter-rotating two-color laser fields produces quantum interference between photoelectrons emitted on the leading and trailing edges of the laser field oscillations. We show that in chiral molecules, this…
Conceptualizing planetary habitability depends on understanding how living organisms originated and what features of environments are essential to foster abiogenesis. Estimates of the abundance of life's building blocks are confounded by…
Living organisms exhibit consistent homochirality. It is argued that the specific, binary choice made is not an accident but is a consequence of parity violation in the weak interaction expressed by cosmic irradiation. The secondary muons…
We examine the dynamics of chiral states of chiral molecules with high tunneling rates in dilute and condensed phases in the context of time-dependent perturbation theory. The chiral molecule is effectively described by an asymmetric…
Chiral active matter is a variant of active matter systems in which the motion of the constituent particles violates mirror symmetry. In this letter, we simulate two-dimensional chiral Active Brownian Particles, the simplest chiral model in…
We consider a simple model for the assembly of chiral molecules in two dimensions driven by maximization of the contact area. We derive a macroscopic model described by a parameter taking nine possible values corresponding to the possible…
We studied a collection of chiral active particles (CAP) on a two dimensional substrate using extensive numerical study. Particles interact through soft repulsive interaction. The activity and chirality of particles is tuned by varying…
The decoherence of a two-state tunneling molecule, such as a chiral molecule or ammonia, due to collisions with a buffer gas is analyzed in terms of a succession of quantum states of the molecule satisfying the conditions for a consistent…
Biological systems exhibit marked molecular asymmetry, with proteins based predominantly on L-amino acids and nucleic acids and carbohydrates largely composed of D-sugars. Explanations for homochirality include asymmetric photochemistry,…