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Strong spin-orbit coupled 5d transition metal based ABO3 oxides, especially iridates, allow tuning parameters in the phase diagram and may demonstrate important functionalities, for example, by means of strain effects and symmetry-breaking,…

强关联电子 · 物理学 2015-05-22 Abhijit Biswas , Yoon Hee Jeong

The large spin-orbit coupling in iridium oxides plays a significant role in driving novel physical behaviors, including emergent phenomena in the films and heterostructures of perovskite and Ruddlesden-Popper iridates. In this work, we…

TbMnO$_{3}$ films have been grown under compressive strain on (001)-oriented SrTiO$_{3}$ crystals. They have an orthorhombic structure and display the (001) orientation. With increasing thickness, the structure evolves from a more symmetric…

The 5d iridium-based transition metal oxides have gained broad interest because of their strong spin-orbit coupling which favors new or exotic quantum electronic states. On the other hand, they rarely exhibit more mainstream orders like…

强关联电子 · 物理学 2022-01-26 Arun Kumar Jaiswal , Di Wang , Vanessa Wollersen , Rudolf Schneider , Matthieu Le Tacon , Dirk Fuchs

SrIrO3, the three-dimensional member of the Ruddlesden-Popper iridates, is a paramagnetic semimetal characterised by a the delicate interplay between spin-orbit coupling and Coulomb repulsion. In this work, we study the anisotropic…

The spin-orbit coupling and electron correlation in perovskite SrIrO3 (SIO) strongly favor new quantum states and make SIO very attractive for next generation quantum information technology. In addition, the small electronic band-width…

材料科学 · 物理学 2019-07-18 A. K. Jaiswal , R. Schneider , R. Singh , D. Fuchs

Electronic transport has been investigated for strong spin-orbit coupled perovskite SrIrO3 thin films grown at various substrate temperatures. The electronic transport of the SrIrO3 films is found to be very sensitive to the growth…

强关联电子 · 物理学 2015-03-17 Abhijit Biswas , Yoon Hee Jeong

We report a magnetotransport study of spin relaxation in 1.4-21.2 nm epitaxial SrIrO$_3$ thin films coherently strained on SrTiO$_3$ substrates. Fully charge compensated semimetallic transport has been observed in SrIrO$_3$ films thicker…

强关联电子 · 物理学 2020-06-16 L. Zhang , X. Jiang , X. Xu , X. Hong

We report on the synthesis and transport properties of perovskite (Pv) CaIrO3 thin films. The Pv phase of CaIrO3 was stabilized by epitaxial growth on SrTiO3, (LaAlO3)0.3(Sr2AlTaO6)0.7, and LaAlO3 substrates with strong tensile, weak…

超导电性 · 物理学 2015-07-23 Daigorou Hirai , Jobu Matsuno , Hidenori Takagi

We investigate the thickness-dependent electronic structure of ultrathin SrIrO$_3$ and discover a transition from a semimetallic to a correlated insulating state below 4 unit cells. Low-temperature magnetoconductance measurements show that…

Epitaxial strain in transition-metal oxides can induce dramatic changes in electronic and magnetic properties. A recent study on the epitaxially strained SrCoO$_3$ thin films revealed persistent ferromagnetism even across a metal-insulator…

In this work, we report observation of strain effect on physical properties of Sr2IrO4 thin films grown on SrTiO3 (001) and LaAlO3 (001) substrates. It is found that the film on LaAlO3 with compressive strain has a lower antiferromagnetic…

强关联电子 · 物理学 2023-09-19 N. Hu , Y. K. Weng , K. Chen , B. You , Y. Liu , Y. T. Chang , R. Xiong , S. Dong , C. L. Lu

The burgeoning fields of spintronics and topological electronics require materials possessing a unique combination of properties: ferromagnetism, metallicity, and chemical stability. SrRuO3 (SRO) stands out as a compelling candidate due to…

Electrical transport in oxide thin films under high pressure remains largely unexplored due to the lack of a universal experimental strategy. Here we develop an approach that enables high-pressure transport measurements in freestanding…

The semi-metallic behavior of the perovskite iridate SrIrO3 shifts the end-member of the strongly spin-orbit (SO) coupled Ruddlesden-Popper series Srn+1IrnO3n+1 away from the Mott insulating regime and the half-filled pseudospin Jeff=1/2…

强关联电子 · 物理学 2025-02-06 Dirk Fuchs , Arun Kumar Jaiswal , Fabrice Wilhelm , Di Wang , Andre Rogalev , Matthieu Le Tacon

We observed a hump-like feature in Hall effects of SrRuO$_3$ ultrathin films, and systematically investigated it with controlling thicknesses, temperatures and magnetic fields. The hump-like feature is extremely stable, even surviving as a…

We investigated the nature of transport and magnetic properties in SrIr0.5Ru0.5O3, (SIRO) which has characteristics intermediate between a correlated non-Fermi liquid state and an itinerant Fermi liquid state, by growing perovskite thin…

强关联电子 · 物理学 2015-09-11 Abhijit Biswas , Yong Woo Lee , Sang Woo Kim , Yoon Hee Jeong

SrRuO3 is an itinerant ferromagnet and in its thin film form when grown on miscut SrTiO3 it has Tc of ~ 150 K and strong uniaxial anisotropy. We measured both the Hall effect and the magnetoresistance (MR) of the films as a function of the…

材料科学 · 物理学 2011-06-15 Isaschar Genish , Yevgeny Kats , Lior Klein , James W. Reiner , M. R. Beasley

Spin orbit coupling plays a non-perturbation effect in many recently developed novel fields including topological insulators and spin-orbit assistant Mott insulators. In this paper, strongly temperature-dependent spin orbit coupling,…

材料科学 · 物理学 2014-06-17 Lunyong Zhang , Y. B. Chen , Jian Zhou , Shan-Tao Zhang , Zheng-bin Gu , Shu-Hua Yao , Yan-Feng Chen

We investigated the electronic properties of epitaxially stabilized perovskite SrIrO3 and demonstrated the effective strain-control on its electronic structure. Comprehensive transport measurements showed that the strong spin-orbit coupling…