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The thermoelectric properties of nanostructured silicon are not fully understood despite their initial promise. While the anomalously low thermal conductivity has attracted much work, the impact of nanostructuring on the power factor has…

材料科学 · 物理学 2020-10-06 Jun Ma , Dhruv Gelda , Krishna V. Valavala , Sanjiv Sinha

We report on the elaboration of germanium manganese nanostructured thin films and the measurement of their thermoelectric properties. We investigate the growth of Ge:Mn layers along with a thorough structural characterization of this…

The thermal conductivity of a crystal is sensitive to the presence of surfaces and nanoscale defects. While this opens tremendous opportunities to tailor thermal conductivity, a true "phonon engineering" of nanocrystals for a specific…

材料科学 · 物理学 2012-07-16 Xiaowang Zhou , Reese E. Jones

Silicon nanoparticles have the promise to surpass the theoretical efficiency limit of single-junction silicon photovoltaics by the creation of a "phonon bottleneck", a theorized slowing of the cooling rate of hot optical phonons that in…

介观与纳米尺度物理 · 物理学 2021-04-14 Ilana J. Porter , Angela Lee , Scott K. Cushing , Hung-Tzu Chang , Justin C. Ondry , A. Paul Alivisatos , Stephen R. Leone

We study the size dependence of thermal conductivity in nanoscale semiconducting systems. An analytical formula including the surface scattering and the size confinement effects of phonon transport is derived. The theoretical formula gives…

材料科学 · 物理学 2009-11-11 L. -H Liang , Baowen Li

Nanostructured materials enable high thermal transport tunability, holding promises for thermal management and heat harvesting applications. Predicting the effect that nanostructuring has on thermal conductivity requires models, such as the…

材料科学 · 物理学 2021-10-19 S. Aria Hosseini , Sarah Khanniche , P. Alex Greaney , Giuseppe Romano

A correlation is observed between the diameter (d) distribution of single walled carbon nanotubes and the percentages of metallic and semiconducting tubes in materials synthesized at low temperature (600 C) by plasma-assisted chemical vapor…

介观与纳米尺度物理 · 物理学 2007-05-23 Yiming Li , Shu Peng , David Mann , Jien Cao , Ryan Tu , K. J. Cho , Hongjie Dai

Controlling thermal transport at the nanoscale is vital for many applications. Previously, it has been shown that this control can be achieved with periodically nanostructured two-dimensional phononic crystals, for the case of suspended…

介观与纳米尺度物理 · 物理学 2024-06-12 Samuli Heiskanen , Tuomas Puurtinen , Ilari J. Maasilta

We theoretically compute the thermal conductivity of SiGe alloy nanowires as a function of nanowire diameter, alloy concentration, and temperature, obtaining a satisfactory quantitative agreement with experimental results. Our results…

材料科学 · 物理学 2015-05-27 Zhao Wang , N. Mingo

Thermal conductivity measurements over variable lengths on nanostructures such as nanowires provide important information about the mean free paths (MFPs) of the phonons responsible for heat conduction. However, nearly all of these…

介观与纳米尺度物理 · 物理学 2015-02-23 Hang Zhang , Chengyun Hua , Ding Ding , Austin J. Minnich

Heat transfer between two surfaces separated by a nanometre gap is important for a number of applications ranging from spaced head disk systems, scanning thermal microscopy and thermal transport in aerogels. At these separation distances,…

材料科学 · 物理学 2020-01-07 A. Alkurdi , C. Adessi , F. Tabatabaei , S. Li , K. Termentzidis , S. Merabia

Hyperpolarized nanoparticles (NPs) offer high polarization levels with room temperature relaxation times exceeding half an hour. In this work, we demonstrate that the achievable hyperpolarization enhancement and relaxation (decay) time at…

In-plane thermal conduction and phonon transport in both single-crystalline and polycrystalline Si two-dimensional phononic crystal (PnC) nanostructures were investigated at room temperature. The impact of phononic patterning on thermal…

介观与纳米尺度物理 · 物理学 2015-02-11 M. Nomura , Y. Kage , J. Nakagawa , T. Hori , J. Maire J. Shiomi , D. Moser , O. Paul

Engineering materials to include nanoscale porosity or other nanoscale structures has become a well-established strategy for enhancing the thermoelectric performance of dielectrics. However, the approach is only considered beneficial for…

材料科学 · 物理学 2021-10-14 Hosseini , S. Aria , Romano , Giuseppe , Greaney , P. Alex

By using molecular dynamics simulations, we study thermal conductivity of silicon nanowires (SiNWs) with different cross sectional geometries. It is found that thermal conductivity decreases monotonically with the increase of…

介观与纳米尺度物理 · 物理学 2015-06-03 Jie Chen , Gang Zhang , Baowen Li

We have shown theoretically that a combination of cross-section modulation and acoustic mismatch in the core-shell Si/Ge nanowires can lead to a drastic reduction of the thermal conductivity. Our calculations, which utilized two different…

介观与纳米尺度物理 · 物理学 2015-06-16 Denis L. Nika , Alexandr I. Cocemasov , Dmitrii V. Crismari , Alexander A. Balandin

The short diffusion lengths in insertion battery nanoparticles render the capacitive behavior of bounded diffusion, which is rarely observable with conventional larger particles, now accessible to impedance measurements. Coupled with…

化学物理 · 物理学 2012-05-31 J. Song , M. Z. Bazant

Prevailing nanostructuring strategies focus on increasing phonon scattering and reducing the mean-free-path of phonons across the spectrum. In nanoporous Si materials, for example, boundary scattering reduces thermal conductivity…

介观与纳米尺度物理 · 物理学 2020-12-02 Laura de Sousa Oliveira , S. Aria Hosseini , Alex Greaney , Neophytos Neophytou

Nanofluids are suspensions of nanoparticles and fibers which have recently attracted much attention due to their superior thermal properties. Here, nanofluids are studied in the sense of nanofins transversally attached to a surface, so that…

介观与纳米尺度物理 · 物理学 2010-11-23 Eliodoro Chiavazzo , Pietro Asinari

Recent advances in our understanding of thermal transport in nanocrystalline systems are responsible for the integration of new technologies into advanced energy systems, including thermoelectric refrigeration systems and renewable energy…

介观与纳米尺度物理 · 物理学 2019-08-12 Brian F. Donovan , Ronald J. Warzoha , R. Bharath Venkatesh , Nicholas T. Vu , Jay Wallen , Daeyeon Lee