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The quest for Kitaev quantum spin liquids has led to great interest in honeycomb quantum magnets with strong spin-orbit coupling. It has been recently proposed that even Mott insulators with $3d$ transition metal ions, having nominally weak…

强关联电子 · 物理学 2021-11-25 Shreya Das , Sreekar Voleti , Tanusri Saha-Dasgupta , Arun Paramekanti

The honeycomb Mott insulator $\alpha$-RuCl$_3$ loses its low-temperature magnetic order by pressure. We report clear evidence for a dimerized structure at $P>1$ GPa and observe the breakdown of the relativistic $j_{\rm eff}$ picture in this…

The weak Mott insulating regime of the triangular lattice Hubbard model exhibits a rich magnetic phase diagram as a result of the ring exchange interaction in the spin Hamiltonian. These phases include the Kalmeyer-Laughlin type chiral spin…

强关联电子 · 物理学 2025-12-23 Asimpunya Mitra , Daniel J. Schultz , Yong Baek Kim

The Kitaev-Heisenberg (KH) model has been proposed to capture magnetic interactions in iridate Mott insulators on the honeycomb lattice. We show that analogous interactions arise in many other geometries built from edge-sharing IrO_6…

强关联电子 · 物理学 2014-02-28 Itamar Kimchi , Ashvin Vishwanath

The Kitaev spin model offers an exact quantum spin liquid in the ground state, which has stimulated exploration of its material realization over the last decade. Thus far, most of the candidates are found in $4d$- and $5d$-electron…

强关联电子 · 物理学 2020-11-03 Seong-Hoon Jang , Ryoya Sano , Yasuyuki Kato , Yukitoshi Motome

We study the quantum many-body instabilities of the $t -J_{\mathrm{K}} - J_{\mathrm{H}}$ Kitaev-Heisenberg Hamiltonian on the honeycomb lattice as a minimal model for a doped spin-orbit Mott insulator. This spin-$1/2$ model is believed to…

We explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr$_{0.5}$Ru$_{0.5}$Cl$_3$, where spin-1/2 and spin-3/2 ions occupy distinct sublattices of a honeycomb lattice. By developing a…

强关联电子 · 物理学 2025-05-09 Willian Natori , Yang Yang , Hui-Ke Jin , Johannes Knolle , Natalia B. Perkins

We discuss the ground state of the spin-orbital model for spin-one ions with partially filled $t_{2g}$ levels on a honeycomb lattice. We find that the orbital degrees of freedom induce a spontaneous dimerization of spins and drive them into…

强关联电子 · 物理学 2008-04-12 G. Jackeli , D. I. Khomskii

The quest for entangled spin excitations has stimulated intense research on frustrated magnetic systems. For almost two decades, the triangular-lattice Mott insulator $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ has been the hottest candidate for…

强关联电子 · 物理学 2023-06-06 A. Pustogow , Y. Kawasugi , H. Sakurakoji , N. Tajima

We present a theory of spin and orbital states in Mott insulator $LaTiO_3$. The spin-orbital superexchange interaction between $d^1(t_{2g})$ ions in cubic crystal suffers from a pathological degeneracy of orbital states at classical level.…

强关联电子 · 物理学 2009-10-31 G. Khaliullin , S. Maekawa

The mineral malachite, Cu2(OD)2CO3, has a quantum spin-liquid ground state and no long-range magnetic order down to at least T=0.4 K. Inelastic neutron scattering measurements show that the excitation spectrum consists of dispersive gapped…

We present a theoretical study of the static and dynamical properties of the Kitaev magnet $\beta$-Li$_2$IrO$_3$ based on the minimal $J$-$K$-$\Gamma$ model. We argue that the incommensurate magnetic order of $\beta$-Li$_2$IrO$_3$ can be…

强关联电子 · 物理学 2018-03-20 Samuel Ducatman , Ioannis Rousochatzakis , Natalia B. Perkins

We study the general phase diagram of correlated electrons for iridium-based (Ir) compounds on the hyperhoneycomb lattice---a crystal structure where the Ir$^{4+}$ ions form a three-dimensional network with three-fold coordination recently…

强关联电子 · 物理学 2014-06-11 Eric Kin-Ho Lee , Subhro Bhattacharjee , Kyusung Hwang , Heung-Sik Kim , Hosub Jin , Yong Baek Kim

Very recently a quantum liquid was reported to form in H$_3$LiIr$_2$O$_6$, an iridate proposed to be a close realization of the Kitaev honeycomb model. To test this assertion we perform detailed quantum chemistry calculations to determine…

Intensive studies of the interplay between spin-orbit coupling (SOC) and electronic correlations in transition metal compounds have recently been undertaken. In particular, $j_{\rm eff}$ = 1/2 bands on a honeycomb lattice provide a pathway…

强关联电子 · 物理学 2015-06-24 Heung-Sik Kim , V. Vijay Shankar , Andrei Catuneanu , Hae-Young Kee

The emergence of quasiparticles in quantum many-body systems underlies the rich phenomenology in many strongly interacting materials. In the context of doped Mott insulators, magnetic polarons are quasiparticles that usually arise from an…

量子气体 · 物理学 2025-02-12 Max L. Prichard , Benjamin M. Spar , Ivan Morera , Eugene Demler , Zoe Z. Yan , Waseem S. Bakr

We report a detailed study of a model Hamiltonian which exhibits a rich interplay of geometrical spin frustration, strong electronic correlations, and charge ordering. The character of the insulating phase depends on the magnitude of…

强关联电子 · 物理学 2013-05-29 J. Merino , R. H. McKenzie , B. J. Powell

There have been constant efforts to find exotic quantum spin-liquid (QSL) materials. Some of the transition metal insulators dominated by the direction dependent anisotropic exchange interaction (Kitaev model for honeycomb network of…

强关联电子 · 物理学 2023-05-17 S. Rayaprol , K. K. Iyer , A. Hoser , M. Reehuis , A. V. Morozkin , V. Siruguri , K. Maiti , E. V. Sampathkumaran

Geometric frustration among competing spin exchanges can give rise to novel quantum phases by enhancing fluctuations that drive magnetic systems beyond the classical regime. We investigate the frustrated array of strongly correlated spin…

The study of non-s-wave unconventional superconductivities in strongly correlated-electron systems has been a central issue in condensed matter physics for more than 30 years. In such unconventional superconductivities, d-wave Cooper…