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We report strong coupling of a monolayer of J-aggregated dye molecules to the whispering gallery modes of a dielectric microsphere at room temperature. We systematically studied the evolution of strong coupling as the number of layers of…

光学 · 物理学 2020-02-27 Adarsh B Vasista , William L Barnes

Colloidal semiconductor nanoplatelets exhibit quantum size effects due to their thickness of only few monolayers, together with strong optical band-edge transitions facilitated by large lateral extensions. In this article we demonstrate…

Strong light-matter coupling has shown great potential for modifying the electro-optical properties of semiconducting materials in recent years. In the strong coupling regime, excitons and cavity photons form new states named…

应用物理 · 物理学 2023-11-23 Yahui Tang , Alexandra Stuart , Timothy van der Laan , Girish Lakhwani

Semiconductor microcavities operating in the polaritonic regime are highly non-linear, high speed systems due to the unique half-light, half-matter nature of polaritons. Here, we report for the first time the observation of propagating…

We report on strong coupling between surface plasmon polaritons (SPP) and Rhodamine 6G (R6G) molecules, with double vacuum Rabi splitting energies up to 230 and 110 meV. In addition, we demonstrate the emission of all three energy branches…

光学 · 物理学 2010-08-30 T. K. Hakala , J. J. Toppari , A. Kuzyk , M. Pettersson , H. Tikkanen , H. Kunttu , P. Törmä

Coupling excitons with quantized radiation has been shown to enable coherent ballistic transport at room temperature inside optical cavities. Previous theoretical works employ a simple description of the material, depicting it as a…

量子物理 · 物理学 2026-05-14 Saeed Rahmanian Koshkaki , Arshath Manjalingal , Logan Blackham , Arkajit Mandal

Guided 2D exciton-polaritons, resulting from the strong coupling of excitons in semiconductors with non-radiating waveguide modes, provide an attractive approach towards developing novel on-chip optical devices. These quasiparticles are…

Strong interactions between surface plasmons in ultra-compact nanocavities and excitons in two dimensional materials have attracted wide interests for its prospective realization of polariton devices at room temperature. Here, we propose a…

Carrier dynamics at energy level anticrossings in biased semiconductor superlattices, was studied in the time domain by solving the time-dependent Schroedinger equation. The resonant nature of interminiband Rabi oscillations has been…

介观与纳米尺度物理 · 物理学 2009-11-13 Pavel Abumov , D. W. L. Sprung

We embedded an all-hydrocarbon-based carbocation in a metallic microcavity that was tuned to resonance with an electronic transition of the carbocation. The measured Rabi splitting was 41% of the excitation energy, putting the system well…

量子物理 · 物理学 2022-04-11 Mao Wang , Suman Mallick , Anton Frisk Kockum , Karl Börjesson

Organic semiconductors are a promising platform for ambient polaritonics. Several applications, such as polariton routers, and many-body condensed matter phenomena are currently hindered due to the ultra-short polariton lifetimes in…

We present a study of the strong coupling between radiation and matter, considering a system of two quantum dots, which are in mutual interaction and interacting with a single mode of light confined in a semiconductor nanocavity. We take…

强关联电子 · 物理学 2015-05-27 Paulo C. Cárdenas , Nicolás Quesada , Herbert Vinck-Posada , Boris A. Rodríguez

We calculate the intensity of the polariton mediated inelastic light scattering in semiconductor microcavities. We treat the exciton-photon coupling nonperturbatively and incorporate lifetime effects in both excitons and photons, and a…

强关联电子 · 物理学 2008-05-04 L. M. Leon Hilario , A. Bruchhausen , A. M. Lobos , A. A. Aligia

Hybridization of excitons with photons to form hybrid quasiparticles, exciton-polaritons (EPs), has been widely investigated in a range of semiconductor material systems coupled to photonic cavities. Self-hybridization occurs when the…

We present novel experimental results demonstrating the coherence properties of the nonlinear emission from semiconductor microcavities in the strong coupling regime, recently interpreted by parametric polariton four-wave mixing. We use a…

We extend the model of exciton-plasmon materials to include a ro-vibrational structure of molecules using wave-packet propagations on electronic potential energy surfaces. The new model replaces conventional two-level emitters with more…

介观与纳米尺度物理 · 物理学 2017-08-18 Maxim Sukharev , Eric Charron

The strong coupling of molecules with surface plasmons results in hybrid states which are part molecule, part surface-bound light. Since molecular resonances may acquire the spatial coherence of plasmons, which have mm-scale propagation…

光学 · 物理学 2022-05-26 Marie S Rider , Rakesh Arul , Jeremy J Baumberg , William L Barnes

Strongly-coupled quantum fields, such as multi-component atomic condensates, optical fields and polaritons, are remarkable systems where the simple dynamics of coupled oscillators can meet the intricate phenomenology of quantum fluids. When…

Modal coupling between frequency-degenerate resonances of an optical ring resonator is a commonly observed phenomenon that results in adverse mode splitting. Traditionally, this coupling is attributed to Rayleigh scattering of a propagating…

光学 · 物理学 2018-06-27 Kathleen McGarvey-Lechable , Pablo Bianucci

It is demonstrated that the effect of coexistence of bulk and surface polaritons within the same frequency band and wavevector space can be achieved in a magnetic-semiconductor superlattice providing a conscious choice of characteristic…

材料科学 · 物理学 2017-03-10 Vladimir R. Tuz , Volodymyr I. Fesenko , Illia V. Fedorin , Hong-Bo Sun , Wei Han