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We develop a theory of the electronic structure and photophysics of interacting chains of \pi- conjugated polymers to understand the differences between solutions and films. While photoexcitation generates only the intrachain exciton in…

材料科学 · 物理学 2009-11-13 Zhendong Wang , Sumit Mazumdar , Alok Shukla

The elementary optical excitations in two dimensional semiconductors hosting itinerant electrons are attractive and repulsive polarons -- excitons that are dynamically screened by electrons. Exciton-polarons have hitherto been studied in…

The exciton spin dynamics are investigated both experimentally and theoretically in two-monolayer-thick GaAs/AlAs quantum wells with an indirect band gap and a type-II band alignment. The magnetic-field-induced circular polarization of…

介观与纳米尺度物理 · 物理学 2017-07-14 T. S. Shamirzaev , J. Rautert , D. R. Yakovlev , J. Debus , A. Yu. Gornov , M. M. Glazov , E. L. Ivchenko , M. Bayer

Electrically conducting polymers with mechanical adaptability are essential for flexible electronics, yet most suffer structural degradation under rapid deformation. In this study, multiscale coarse-grained (MSCG) simulations are used to…

软凝聚态物质 · 物理学 2025-11-03 Jingchen Wang , Tianqi Hu , Jingjie Yeo

We report on a strong dependence of the phonon-induced damping of Rabi dynamics in an optically driven exciton-biexciton quantum dot system on the polarization of the exciting pulse. While for a fixed pulse intensity the damping is maximal…

介观与纳米尺度物理 · 物理学 2013-03-15 M. Glässl , V. M. Axt

Large exciton-polariton optical nonlinearities present a key mechanism for photonics-based communication, ultimately in the quantum regime. Enhanced nonlinear response from various materials hosting excitons and allowing for their strong…

介观与纳米尺度物理 · 物理学 2024-08-05 Anna M. Grudinina , Nina S. Voronova

Herein, the dynamics of excitons coupled with optical phonons in a triangular system is numerically studied. By representing the excitons by quasi-spin states, the similarity between the chiral spin states and the exciton chiral states is…

介观与纳米尺度物理 · 物理学 2023-05-30 Noriyuki Aoyagi , Hiroaki Matsueda , Kunio Ishida

Charge transport in polymers, such as polyacrylonitrile (PAN), is crucial for electronics and energy storage. For instance, PAN can transport cations e.g., Li+, by facilitating dynamic cation-nitrile coordination in batteries. However,…

The scattering of lattice excitations (phonons) with the photoexcited charge carriers is of a major concern in optoelectronic devices. Here, the resonant Raman scattering will be utilized to study an exciton-phonon interaction in GaN…

Exciton dynamics can be strongly affected by lattice vibrations through electron-phonon coupling. This is rarely explored in two-dimensional magnetic semiconductors. Focusing on bilayer CrI3, we first show the presence of strong…

Strong light-matter coupling in optical waveguides provides a versatile platform for engineering hybrid polaritonic modes and their dispersion. Here we investigate multimode exciton-photon coupling in visible semiconductor waveguides…

We study the relaxation dynamics of driven, two-dimensional semiconductors, where itinerant electrons dress optically pumped excitons to form two Fermi-polaron branches. Repulsive polarons excited around zero momentum quickly decay to the…

介观与纳米尺度物理 · 物理学 2022-04-21 Tomasz Wasak , Falko Pientka , Francesco Piazza

In this work we attempt to elucidate the nature of conductivity in polymers by taking the acid-base doped polyaniline (PAni) polymer. We evaluate the PAni conductance by using realistic ab initio parameters and including decoherent…

无序系统与神经网络 · 物理学 2010-10-06 Carlos J. Cattena , Raúl A. Bustos-Marún , Horacio M. Pastawski

Optical orientation of carrier spins by circularly polarized light is the basis of spin physics in semiconductors. Here, we demonstrate strong optical orientation of 85\%, approaching the ultimate limit of unity, for excitons in…

Polymer nanofibers are one-dimensional organic hydrocarbon systems containing conducting polymers where the non-linear local excitations such as solitons, polarons and bipolarons formed by the electron-phonon interaction were predicted.…

介观与纳米尺度物理 · 物理学 2012-10-18 A. Choi , K. H. Kim , S. J. Hong , M. Goh , K. Akagi , R. B. Kaner , N. N. Kirova , S. A. Brazovskii , A. T. Johnson , D. A. Bonnell , E. J. Mele , Y. W. Park

We study the dynamics of the spin system that consist of a positively charged II-VI semiconductor quantum dot doped with a single Cr$^+$ ion. The resonant photoluminescence (PL) of the positively charged exciton coupled with the Cr$^+$ spin…

介观与纳米尺度物理 · 物理学 2022-08-17 V. Tiwari , M. Morita T. Inoue , S. Ando S. Kuroda , H. Boukari , L. Besombes

The exciton spin dynamics and polarization properties of the related emission are investigated in colloidal CdSe/CdS dot-in-rod (DiR) and spherical core/shell nanocrystal (NC) ensembles by magneto-optical photoluminescence (PL) spectroscopy…

介观与纳米尺度物理 · 物理学 2015-06-23 B. Siebers , L. Biadala , D. R. Yakovlev , A. V. Rodina , T. Aubert , Z. Hens , M. Bayer

Optically controlled coherent dynamics of charge (excitonic) degrees of freedom in a semiconductor quantum dot under the influence of lattice dynamics (phonons) is discussed theoretically. We show that the dynamics of the lattice response…

介观与纳米尺度物理 · 物理学 2007-05-23 Pawel Machnikowski , Lucjan Jacak

The exciton relaxation dynamics of photoexcited electronic states in poly($p$-phenylenevinylene) (PPV) are theoretically investigated within a coarse-grained model, in which both the exciton and nuclear degrees of freedom are treated…

化学物理 · 物理学 2018-02-14 Jonathan R. Mannouch , William Barford , Sarah Al-Assam

Exciton plasmon polaritons have gained increasing interests over recent years due to their versatile properties emerging by the underlying light-matter coupling and making them potential candidates for new photonic applications. We have…

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