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An experimental study of the dispersion cancellation occurring in frequency-entangled photon pairs is presented. The approach uses time-resolved up conversion of the pairs, which has temporal resolution at the fs level, and group-delay…

量子物理 · 物理学 2011-03-03 Kevin A. O'Donnell

Entangled two-photon absorption (eTPA) has been recognized as a potentially powerful tool for the implementation of ultra-sensitive spectroscopy. Unfortunately, there exists a general agreement in the quantum optics community that…

量子物理 · 物理学 2025-01-31 Áulide Martínez-Tapia , Roberto de J. León-Montiel

We theoretically investigate the generation of two entangled beams of light in the process of single-pass type-I noncollinear frequency degenerate parametric downconversion with an ultrashort pulsed pump. We find the spatio-temporal…

量子物理 · 物理学 2021-03-09 L. La Volpe , S. De , M. I. Kolobov , V. Parigi , C. Fabre , N. Treps , D. B. Horoshko

Encoding quantum information in photonic time-bin states is typically considered impractical for moving free-space quantum communication due to the difficulties with phase stabilization of distant quantum time-bin interferometers and…

As relative systematic frequency uncertainties in trapped-ion spectroscopy are approaching the low $10^{-18}$ range, motional frequency shifts account for a considerable fraction of the uncertainty budget. Micromotion, a driven motion…

原子物理 · 物理学 2015-11-18 J. Keller , H. L. Partner , T. Burgermeister , T. E. Mehlstäubler

The possibility of soliton self-compression of ultrashort laser pulses down to the few-cycle regime in photonic crystal fibers is numerically investigated. We show that efficient sub-two-cycle temporal compression of nanojoule-level 800 nm…

光学 · 物理学 2009-11-13 Marco V. Tognetti , Helder M. Crespo

Frequency-bin entangled photons can be efficiently produced on-chip which offers a scalable, robust and low-footprint platform for quantum communication, particularly well-suited for resource-constrained settings such as mobile or…

We experimentally demonstrate two-photon absorption (TPA) with broadband down-converted light (squeezed vacuum). Although incoherent and exhibiting the statistics of a thermal noise, broadband down-converted light can induce TPA with the…

量子物理 · 物理学 2011-12-06 Barak Dayan , Avi Pe'er , Asher A. Friesem , Yaron Silberberg

We present a study of the effects of dispersion on the properties of photon pairs generated by type-II, collinear spontaneous parametric downconversion. Specifically, we take into consideration the effects of a chirped pump, as well as of…

量子物理 · 物理学 2009-04-27 Yasser Jeronimo-Moreno , Alfred B. U'Ren

We study the probability distribution of an atomic ion being laser-cooled in a periodically-driven Paul trap using a Floquet approach to the semiclassical photon scattering dynamics. We show that despite the microscopic nonequilibrium…

原子物理 · 物理学 2019-07-24 H. Landa

Entangled two-photon absorption (ETPA) has recently become a topic of lively debate, mainly due to the apparent inconsistencies in the experimentally-reported ETPA cross sections of organic molecules. In this work, we provide a thorough…

A natural choice for quantum communication is to use the relative phase between two paths of a single-photon for information encoding. This method was nevertheless quickly identified as impractical over long distances and thus a…

量子物理 · 物理学 2021-10-06 A. Alarcón , J. Argillander , G. Lima , G. B. Xavier

A pair of optical pulses traveling through two dispersive media will become broadened and, as a result, the degree of coincidence between the optical pulses will be reduced. For a pair of entangled photons, however, nonlocal dispersion…

量子物理 · 物理学 2015-05-13 So-Young Baek , Young-Wook Cho , Yoon-Ho Kim

The pursuit of ever-shorter time scales is a frontier in modern physics, exemplified by the synthesis of attosecond light pulses -- an achievement made possible by coherently superimposing a broad range of photon energies, as required by…

介观与纳米尺度物理 · 物理学 2025-04-25 Xin Jin , Cruz I. Velasco , F. Javier García de Abajo

We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by…

量子物理 · 物理学 2024-04-26 Tiemo Landes , Brian J. Smith , Michael G. Raymer

We demonstrate sub-shot-noise photon-number correlations in a (temporal) multimode mesoscopic ($\sim 10^3$ detected photons) twin-beam produced by ps-pulsed spontaneous non-degenerate parametric downconversion. We have separately detected…

量子物理 · 物理学 2009-11-13 Maria Bondani , Alessia Allevi , Guido Zambra , Matteo G. A. Paris , Alessandra Andreoni

Frequency-entangled photons can be readily produced using parametric down-conversion. We have recently shown how such entanglement could be manipulated and measured using electro-optic phase modulators and narrow-band frequency filters,…

In virtual-state spectroscopy, information about the energy-level structure of an arbitrary sample is retrieved by Fourier transforming sets of measured two-photon absorption probabilities of entangled photon pairs where the degree of…

量子物理 · 物理学 2021-08-04 Lutz Mertenskötter , Kurt Busch , Roberto de J. León-Montiel

Entangled two-photon absorption (ETPA) could form the basis of nonlinear quantum spectroscopy at very low photon fluxes, since, at sufficiently low photon fluxes, ETPA scales linearly with the photon flux. When different pairs start to…

量子物理 · 物理学 2023-12-04 Frank Schlawin

Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and has become a highly successful method for experiments in chemical physics. Current quantum optical experiments…

量子物理 · 物理学 2016-10-19 Frank Schlawin , Manuel Gessner , Shaul Mukamel , Andreas Buchleitner