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We demonstrate strong coupling between molecular excited states and surface plasmon modes of a slit array in a thin metal film. The coupling manifests itself as an anti-crossing behavior of the two newly formed polaritons. As the coupling…

介观与纳米尺度物理 · 物理学 2012-08-17 Adi Salomon , Robert J. Gordon , Yehiam Prior , Tamar Seideman , Maxim Sukharev

The manipulation of molecular excited state processes through strong coupling has attracted significant interest for its potential to provide precise control of photochemical phenomena. However, the key limiting factor for achieving this…

Using random matrices, we study the reduced dynamics of a two level system interacting with a generic environment. In the weak coupling limit, the result can be obtained directly from known results for purity decay, and result in Markovian…

量子物理 · 物理学 2016-02-01 Nephtalí Garrido , Thomas Gorin , Carlos Pineda

Multi-particle correlations of exciton-polaritons and reservoir-excitons in the strong light-matter coupling regime dictate the quantum dynamics of optical microcavities. In this letter, we examine the many-body exciton-polariton dynamics…

In this work we investigate the late-time stationary states of open quantum systems coupled to a thermal reservoir in the strong coupling regime. In general such systems do not necessarily relax to a Boltzmann distribution if the coupling…

统计力学 · 物理学 2013-01-15 Y. Subasi , C. H. Fleming , J. M. Taylor , B. L. Hu

Polaritons, in particular microcavity exciton-polaritons, have attracted much attention in recent years, as the phenomena of Bose-Einstein condensation and superfluidity have been observed for these quasiparticles. While the basic physics…

量子气体 · 物理学 2015-09-07 David Snoke

We report on the strong coupling between the Bloch surface wave supported by an inorganic multilayer structure and $J$-aggregate excitons in an organic semiconductor. The dispersion curves of the resulting polariton modes are investigated…

The notion of strong light-matter coupling is typically associated with the observation of Rabi splitting, corresponding to the formation of the hybrid light-matter states known as polaritons. However, this relationship is derived based on…

化学物理 · 物理学 2025-12-03 Wei-Kuo Li , Hsing-Ta Chen

It is shown analytically that there exists a natural basis in terms of which the nonperturbative time evolution of an important class of driven four-level systems in the strong-coupling regime decouples and essentially reduces to the…

量子物理 · 物理学 2010-07-01 Vicente Delgado , J. M. Gomez Llorente

We study the dynamics of a dressed qubit implemented by a spinless fermion hopping between two lattice sites with each site strongly coupled to a bath of phonons. We employ Lang-Firsov transformation to make the problem tractable…

量子物理 · 物理学 2026-02-10 Saima Bashir , Muzaffar Qadir Lone , Prince A Ganai

Strong coupling of molecular vibrations with light creates polariton states, enabling control over many optical and chemical properties. However, the near-field signatures of strong coupling are difficult to map as most cavities are closed…

A quantum two-level system immersed in a sub-Ohmic bath experiences enhanced low-frequency quantum statistical fluctuations which render the nonequilibrium quantum dynamics highly non-Markovian. Upon using the numerically exact…

统计力学 · 物理学 2022-09-20 Florian Otterpohl , Peter Nalbach , Michael Thorwart

The collective dynamics of two non-interacting two-level emitters, which are coupled to a structured wave guide that supports two-photon bound states, is investigated. Tuning the energy of the two emitters such that they are in resonance…

量子气体 · 物理学 2023-01-25 J. Talukdar , D. Blume

We show that non-Markovian open quantum systems can exhibit exact Markovian dynamics up to an arbitrarily long time; the non-Markovianity of such systems is thus perfectly "hidden", i.e. not experimentally detectable by looking at the…

量子物理 · 物理学 2021-01-08 Daniel Burgarth , Paolo Facchi , Marilena Ligabò , Davide Lonigro

Phonon interactions are inevitable in cavity quantum electrodynamical systems based on solid-state emitters or fluorescent molecules, where vibrations of the lattice or chemical bonds couple to the electronic degrees of freedom. Due to the…

量子物理 · 物理学 2021-06-16 Matias Bundgaard-Nielsen , Jesper Mørk , Emil Vosmar Denning

The dynamics of two interacting spins coupled to separate bosonic baths is studied. An analytical solution in Born approximation for arbitrary spectral density functions of the bosonic environments is found. It is shown that in the…

量子物理 · 物理学 2018-09-05 I. Sinayskiy , E. Ferraro , A. Napoli , A. Messina , F. Petruccione

Quantum information processing relies on how dynamics unfold in open quantum systems. In this work, we study the non-Markovian dynamics in the single mode spin-boson model at strong couplings. In order to apply perturbation theory, we…

量子物理 · 物理学 2025-01-03 Rayees A Mala , Mehboob Rashid , Muzaffar Qadir Lone

The strong coupling of an IR-active molecular transition with an optical mode of the cavity results in vibrational polaritons, which opens a new way to control chemical reactivity via confined electromagnetic fields of the cavity. In this…

We investigate second harmonic generation (SHG) from hexagonal periodic arrays of triangular nano-holes of aluminum using a self-consistent methodology based on the hydrodynamics-Maxwell-Bloch approach. It is shown that angular polarization…

光学 · 物理学 2021-07-07 Maxim Sukharev , Adi Salomon , Joseph Zyss

We report on strong coupling between surface plasmon polaritons (SPP) and Rhodamine 6G (R6G) molecules, with double vacuum Rabi splitting energies up to 230 and 110 meV. In addition, we demonstrate the emission of all three energy branches…

光学 · 物理学 2010-08-30 T. K. Hakala , J. J. Toppari , A. Kuzyk , M. Pettersson , H. Tikkanen , H. Kunttu , P. Törmä