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We explain the concept of superadiabatic approximations and show how in the context of the Born- Oppenheimer approximation they lead to an explicit formula that can be used to predict transitions at avoided crossings. Based on this formula,…

化学物理 · 物理学 2016-06-29 Volker Betz , Benjamin D. Goddard , Uwe Manthe

Adiabatic passage employs a slowly varying time-dependent Hamiltonian to control the evolution of a quantum system along the Hamiltonian eigenstates. For processes of finite duration, the exact time evolving state may deviate from the…

量子物理 · 物理学 2021-06-18 Albert Benseny , Klaus Mølmer

Real-time time-dependent density functional theory, in conjunction with the Ehrenfest molecular dynamics scheme, is becoming a popular methodology to investigate ultrafast phenomena on the nanoscale. Thanks to recent developments, it is…

材料科学 · 物理学 2020-08-18 Jannis Krumland , Ana M. Valencia , Stefano Pittalis , Carlo A. Rozzi , Caterina Cocchi

We demonstrate how dynamic Stark control (DSC) can be achieved on molecular photodissociation in the dipole limit, using single-cycle (FWHM) laser pulses in the terahertz (THz) regime. As the laser-molecule interaction follows the…

化学物理 · 物理学 2020-03-25 A. Tóth , A. Csehi , G. J. Halász , Á. Vibók

We propose a scheme for sensing of an oscillating field in systems with large inhomogeneous broadening and driving field variation by applying sequences of phased, adiabatic, chirped pulses. The latter act as a double filter for dynamical…

量子物理 · 物理学 2020-08-12 Genko T. Genov , Yachel Ben-Shalom , Fedor Jelezko , Alex Retzker , Nir Bar-Gill

We use microwave induced adiabatic passages for selective spin flips within a string of optically trapped individual neutral Cs atoms. We position-dependently shift the atomic transition frequency with a magnetic field gradient. To flip the…

We investigate the influence of dissipation on one- and two-qubit rotations in coupled semiconductor quantum dots, using a (pseudo) spin-boson model with adiabatically varying parameters. For weak dissipation, we solve a master equation,…

介观与纳米尺度物理 · 物理学 2009-11-07 T. Brandes , T. Vorrath

In a recent work we have developed a robust chainwise atom-molecule adiabatic passage scheme to produce ultracold ground-state molecules via photo-associating free atoms [J. Qian {\it et.al.} Phys. Rev. A 81 013632 (2010)]. With the help of…

原子物理 · 物理学 2015-10-28 Jingjing Zhai , Lu Zhang , Keye Zhang , Jing Qian , Weiping Zhang

We theoretically explore photoassociation by Adiabatic Passage of two colliding cold ^{85}Rb atoms in an atomic trap to form an ultracold Rb_2 molecule. We consider the incoherent thermal nature of the scattering process in a trap and show…

量子物理 · 物理学 2009-11-13 Evgeny A. Shapiro , Moshe Shapiro , Avi Pe'er , Jun Ye

The standard model of femtosecond filamentation is based on phenomenological assumptions which suggest that the ionization-induced carriers can be treated as free according to the Drude model, while the nonlinear response of the bound…

原子物理 · 物理学 2016-11-03 Michael Hofmann , Carsten Brée

The use of the nuclear spins surrounding electron spin qubits as quantum registers and long-lived memories opens the way to new applications in quantum information and biological sensing. Hence, there is a need for generic and robust forms…

量子物理 · 物理学 2021-07-06 O. T. Whaites , J. Randall , T. H. Taminiau , T. S. Monteiro

We investigate the geometrical phase associated to the Schr\"odinger equation in a three level system in Stimulated Raman Adiabatic Passage (STIRAP). We solve explicitly a dual model, in which the pulses are applied in the counterintuitive…

量子物理 · 物理学 2020-04-15 Timo Aukusti Laine

We analyze the optical selection rules of the microwave-assisted transitions in a flux qubit superconducting quantum circuit (SQC). We show that the parities of the states relevant to the superconducting phase in the SQC are well-defined…

量子物理 · 物理学 2009-11-11 Yu-xi Liu , J. Q. You , L. F. Wei , C. P. Sun , Franco Nori

The light propagation of a probe field pulse in a four-level double-lambda type system driven by laser fields that form a closed interaction loop is studied. Due to the finite frequency width of the probe pulse, a time-independent analysis…

量子物理 · 物理学 2009-11-13 Mohammad Mahmoudi , Joerg Evers

An adiabatic-connection fluctuation-dissipation theorem approach based on a range separation of electron-electron interactions is proposed. It involves a rigorous combination of short-range density functional and long-range random phase…

材料科学 · 物理学 2009-03-03 Julien Toulouse , Iann C. Gerber , Georg Jansen , Andreas Savin , János G. Ángyán

We study the dissociation of H$_2$$^+$ in uv laser pulses by solving the non-Born-Oppenheimer time-dependent Schr\"{o}dinger equation as a function of the photon energy $\omega$ of the pulse. Significant enhancements of the dissociation…

原子与分子团簇 · 物理学 2014-07-22 Kunlong Liu , Qianguang Li , Pengfei Lan , Peixiang Lu

We study the dynamics of a molecule's nuclear wave-function near an avoided crossing of two electronic energy levels, for one nuclear degree of freedom. We derive the general form of the Schroedinger equation in the n-th superadiabatic…

数学物理 · 物理学 2015-05-13 Volker Betz , Benjamin D. Goddard , Stefan Teufel

A simple technique for robust generation of vibrational Fock states in a chain of trapped ions is proposed. The method is fast and easy to implement, since only a single chirped laser pulse, simultaneously addressing all of the ions, is…

量子物理 · 物理学 2009-11-13 I. E. Linington , P. A. Ivanov , N. V. Vitanov , M. B. Plenio

We investigate the relationship between stability, adiabaticity and transfer efficiency in a \Lambda-type atom-molecule coupling system via a nonlinear stimulated Raman adiabatic passage. We find that only when the pump and control lasers…

量子物理 · 物理学 2011-12-19 Ning Jia , Jing Qian , Guangjiong Dong , Weiping Zhang

It is showed on the basis of the multiple-quantum operator algebra space formalism that ultra-broadband heteronuclear Hartmann-Hahn polarization transfer could be achieved by the amplitude- and frequency-modulation quasi-adiabatic…

量子物理 · 物理学 2007-05-23 Xijia Miao