相关论文: Discussion of the adiabatic hypothesis in control …

Light-induced conical intersections (LICIs) can be formed both by standing or by running laser waves. The position of a LICI is determined by the laser frequency while the laser intensity controls the strength of the nonadiabatic coupling.…

We consider an adiabatic population transfer process that resembles the well established stimulated Raman adiabatic passage (STIRAP). In our system, the states have nonzero angular momentums $J$, therefore, the coupling laser fields induce…

We demonstrate theoretically the possibility of optimal control of light propagation and exciton transfer in arrays constructed of subnanometer sized noble-metal clusters by using phase-shaped laser pulses and analyze the mechanism…

A three-level atom in a $\Lambda$ configuration trapped in an optical cavity forms a basic unit in a number of proposed protocols for quantum information processing. Through control with an appropriate laser, this system allows for…

The chirped-pulse interaction in the adiabatic coupling regime induces cyclic permutations of the energy states of a three-level system in the $V$-type configuration, which process is known as the three-level chirped rapid adiabatic…

When a molecule is exposed to a laser field, all field-free vibrational states become resonances, with complex quasi energies calculated using Floquet theory. There are many ways to produce the coalescences of pairs of such quasi energies,…

Energy transfer during molecular collisions on metal surfaces plays a pivotal role in a host of critical interfacial processes. Despite significant efforts, our understanding of relevant energy transfer mechanisms, even in an…

A new perspective on how to manipulate molecules by means of very strong laser pulses is emerging with insights from the so-called light-induced potentials, which are the adiabatic potential energy surfaces of molecules severely distorted…

The superadiabatic quantum driving, producing a perfect adiabatic transfer on a given Hamitonian by introducing an additional Hamiltonian, is theoretically analysed for transfers within a three-level system. Our starting point is the…

Real-time simulations of laser-driven electron dynamics contain information about molecular optical properties through all orders in response theory. These properties can be extracted by assuming convergence of the power series expansion of…

We present an algebraic method for treating molecular vibrations in the Morse potential perturbed by an external laser field. By the help of a complete and normalizable basis we transform the Schr\"{o}dinger equation into a system of…

We investigate two well-known approaches for extending the fewest switches surface hopping (FSSH) algorithm to periodic time-dependent couplings. The first formalism acts as if the instantaneous adiabatic electronic states were standard…

We show here that due to non-adiabatic couplings in decaying systems applying the same time-dependent protocol in the forward and reverse direction to the same mixed initial state leads to different final pure states. In particular, in…

We demonstrate a method of adiabatic population transfer from a single quantum state into a coherent superposition of states. The transfer is executed with femtosecond pulses, spectrally shaped in simple and intuitive manner, which does not…

A novel laser cooling mechanism was recently demonstrated using a narrow-linewidth optical transition. Counter-propagating laser beams are swept in frequency to cause adiabatic transfer between a ground state and excited state, and Doppler…

Laser excitation pulses that lead to perfect adiabatic state transfer in an ensemble of three-level ladder atoms lead to highly entangled states of many atoms if their highest excited state is subject to Rydberg blockade. Solution of the…

The influence of photon-momentum recoil on adiabatic population transfer in an atomic three-level lambda system is studied. It is shown that the Doppler frequency shifts, due to atomic motion can play an important role in adiabatic…

Resonant dissipation-enabled adiabatic quantum state transfer processes between the polarization degrees of freedom of a single photon wave packet and quantum emitters are discussed. These investigations generalize previous work [N.…

Floquet engineering offers a path to optically-controlled materials, but experimental implementations have frequently relied on femtosecond pulses to achieve the high peak fields required to maximise interactions and obtain a measurable…

Questions are raised about certain experimental and theoretical claims that atoms may be stabilized into their bound states, and prevented from achieving full ionization, by the application of adiabatic, ultraintense, high-frequency laser…