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With a specific choice of laser parameters resulting into a so-called exceptional point in the wavelength-intensity plane, it is possible to produce the coalescence of two Floquet resonances describing the photodissociation of the molecule…

量子物理 · 物理学 2010-11-12 Osman Atabek , Roland Lefebvre , M. Lepers , Amine Jaouadi , Olivier Dulieu , V. Kokoouline

We have experimentally and theoretically investigated the mixed-field orientation of rotational-state-selected OCS molecules and we achieve strong degrees of alignment and orientation. The applied moderately intense nanosecond laser pulses…

Using numerical simulations of two-photon electronic absorption with femtosecond pulses in Na$_2$ we show that: i) it is possible to avoid the characteristic saturation or dumped Rabi oscillations in the yield of absorption by time-delaying…

原子物理 · 物理学 2016-05-25 Pablo Sampedro , Bo Y. Chang , Ignacio R. Sola

We propose and demonstrate a novel laser cooling mechanism applicable to particles with narrow-linewidth optical transitions. By sweeping the frequency of counter-propagating laser beams in a sawtooth manner, we cause adiabatic transfer…

In molecular photodissociation, some specific combinations of laser parameters (wavelength and intensity) lead to unexpected Zero-Width Resonances (ZWR), with in principle infinite lifetimes. Their interest in inducing basic quenching…

量子物理 · 物理学 2016-10-19 Arnaud Leclerc , David Viennot , Georges Jolicard , Roland Lefebvre , Osman Atabek

We present a theoretical study of the impact of an electrostatic field combined with non-resonant linearly polarized laser pulses on the rotational dynamics of linear molecules. Within the rigid rotor approximation, we solve the…

原子物理 · 物理学 2015-06-05 Juan J. Omiste , Rosario González-Férez

We have developed a theory of three-pulse coherent control of photochemical processes. It is based on adiabatic passage and quantum coherence and interference attributed to the lower-lying dissociation continuum and excited upper discrete…

量子物理 · 物理学 2009-11-10 A. K. Popov , V. V. Kimberg , Thomas F. George

We show how one can perform arbitrary rotation of any qubit, using delayed laser pulses through nonadiabatic evolution, i.e., via transitions among the adiabatic states. We use a double-Lambda scheme and use a set of control parameters such…

量子物理 · 物理学 2007-05-23 Asoka Biswas , G. S. Agarwal

We evaluate the shifts imparted to vibrational and rotational levels of a linear molecule by a nonresonant laser field at intensities of up to 10^12 W/cm^2. Both types of shift are found to be either positive or negative, depending on the…

化学物理 · 物理学 2015-03-14 Mikhail Lemeshko , Bretislav Friedrich

We present a theoretical study of recent laser-alignment and mixed-field-orientation experiments of asymmetric top molecules. In these experiments, pendular states were created using linearly polarized strong ac electric fields from pulsed…

Accurate description of nonadiabatic dynamics of molecules at metal surfaces involving electron transfer has been a longstanding challenge for theory. Here, we tackle this problem by first constructing high-dimensional neural network…

材料科学 · 物理学 2024-01-05 Gang Meng , James Gardner , Wenjie Dou , Reinhard J. Maurer , Bin Jiang

We propose a method for slowing particles by laser fields that potentially has the ability to generate large forces without the associated momentum diffusion that results from the random directions of spontaneously scattered photons. In…

原子物理 · 物理学 2020-10-21 John P. Bartolotta , Jarrod T. Reilly , Murray J. Holland

The adiabatic theorem, a corollary of the Schr\"odinger equation, manifests itself in a profoundly different way in non-Hermitian arrangements, resulting in counterintuitive state transfer schemes that have no counterpart in closed quantum…

We present a theoretical study of the rotational dynamics of asymmetry top molecules in an electric field and a parallel non-resonant linearly polarized laser pulse. The time-dependent Schr\"odinger equation is solved within the rigid rotor…

量子物理 · 物理学 2015-06-16 Juan J. Omiste , Rosario González-Férez

High-fidelity Bragg pulses are an indispensable tool for state-of-the-art atom interferometry experiments. In this paper, we introduce an analytic theory for such pulses. Our theory is based on the pivotal insight that the physics of Bragg…

Dispersion management of few-cycle pulses is crucial for ultrafast optics and photonics. Often, nontrivial dispersion is compensated using complex optical systems or minimized through careful design of waveguides. Here, we present…

We present a magnetically enhanced laser cooling scheme applicable to multi-level type-II transitions and further diatomic molecules with adiabatic transfer. An angled magnetic field is introduced to not only remix the dark states, but also…

原子物理 · 物理学 2019-05-07 Qian Liang , Tao Chen , Wenhao Bu , Yuhe Zhang , Bo Yan

We show that a counter-intuitive pulse sequence leads to adiabatic passage between the vibrational levels of three harmonic potentials through parallel dark states in adiabatic approximation. However, the adiabatic assumptions break down…

化学物理 · 物理学 2007-05-23 Ignacio R. Solá , Vladimir S. Malinovsky

We propose a method to transfer the population and control the state of two-level and three-level atoms speeding-up Adiabatic Passage techniques while keeping their robustness versus parameter variations. The method is based on…

量子物理 · 物理学 2010-09-20 Xi Chen , I. Lizuain , A. Ruschhaupt , D. Guery-Odelin , J. G. Muga

We present a detailed semiclassical study on the propagation of a pair of optical fields in resonant media with and without adiabatic approximation. In the case of near and on resonance excitation, we show detailed calculation, both…

量子物理 · 物理学 2009-11-07 M. G. Payne , L. Deng , Chris Schmitt , Shannon Anderson
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