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By performing accurate ab-initio density functional theory calculations, we study the role of $4f$ electrons in stabilizing the magnetic-field-induced ferroelectric state of DyFeO$_{3}$. We confirm that the ferroelectric polarization is…

材料科学 · 物理学 2015-05-14 Alessandro Stroppa , Martijn Marsman , Georg Kresse , Silvia Picozzi

The electric polarization hysteresis loops and remanent polarization were revealed in multiferroics RMn$_2$O$_5$ with $R = Gd$ and $Bi$ at wide temperature interval from 5 K up to 330 K. Until recently, the long-range ferroelectric order…

材料科学 · 物理学 2016-10-21 B. Kh. Khannanov , V. A. Sanina , E. I. Golovenchits , M. P. Scheglov

The magnetic properties of RMn2O5 multiferrroics as obtained by unpolarized and polarized neutron diffraction experiments are reviewed. We discuss the qualitative features of the magnetic phase diagram both in zero magnetic field and in…

材料科学 · 物理学 2009-11-13 P. G. Radaelli , L. C. Chapon

From magnetic susceptibility, dielectric permittivity, electric polarization and specific heat measurements, we discover spin-induced ferroelectricity and magnetoelectric coupling in Mn3TeO6 and observe two successive magnetic transitions…

材料科学 · 物理学 2015-12-01 L. Zhao , Z. Hu , C. Y. Kuo , T. -W. Pi , M. -K. Wu , L. H. Tjeng , A. C. Komarek

Multiferroics, where two or more ferroic order parameters coexist, is one of the hottest fields in condensed matter physics and materials science[1-9]. However, the coexistence of magnetism and conventional ferroelectricity is physically…

材料科学 · 物理学 2016-03-11 Xiangang Wan , Hang-Chen Ding , Sergey Y. Savrasov , Chun-Gang Duan

Magnetoelectric multiferroics are highly sought after for applications in low-power electronics and for advancing fundamental research, including axion insulators and dark matter detection. However, achieving a combination of ferroic spin…

材料科学 · 物理学 2024-12-02 Libor Šmejkal

We report that the spin-chain compound Dy2BaNiO5 recently proven to exhibit magnetoelectric coupling below its Neel temperature (T_N) of 58 K, exhibits strong frequency-dependent behavior in ac magnetic susceptibility and complex dielectric…

Three independent contributions to the magnetically induced spontaneous polarization of multiferroic TbMn2O5 are uniquely separated by optical second harmonic generation and an analysis in terms of Landau theory. Two of them are related to…

强关联电子 · 物理学 2012-03-07 N. Leo , D. Meier , R. V. Pisarev , N. Lee , S. -W. Cheong , M. Fiebig

We report the results of various measurements, namely magnetization, complex dielectric permittivity and electric polarization (P) on Dy2BaNiO5 as a function of temperature (T) and magnetic-field (H), apart from heat-capacity (C), with the…

材料科学 · 物理学 2015-06-15 Kiran Singh , Tathamay Basu , S. Chowki , N. Mahapotra , K. Iyer , P. L. Paulose , E. V. Sampathkumaran

The precise crystal symmetry and hence the emergence of the electric polarization still remains an open question in the multiferroic materials $R$Mn$_2$O$_5$ ($R$ = rare-earth, Bi, Y). While previous diffraction studies have indicated that…

The orthovanadate DyVO3 crystal, known to exhibit multiple structural, spin and orbital ordering transitions, is presently investigated on the basis of magnetization, heat capacity, resistivity, dielectric and polarization measurements. Our…

强关联电子 · 物理学 2014-07-24 Q. Zhang , K. Singh , C. Simon , L. D. Tung , G. Balakrishnan , V. Hardy

A dielectric anomaly has been found near the incommensurate to commensurate antiferromagnetic phase transition (TN2=230 K) in YBaCuFeO5 ceramics, a compound which crystallizes in an ordered perovskite structure. The existence of electric…

材料科学 · 物理学 2009-03-13 B. Kundys , A. Maignan , Ch. Simon

We uncover a new pathway towards multiferroicity, showing how magnetism can drive ferroelectricity without relying on inversion symmetry breaking of the magnetic ordering. Our free-energy analysis demonstrates that any commensurate…

材料科学 · 物理学 2009-11-11 Joseph J. Betouras , Gianluca Giovannetti , Jeroen van den Brink

Resonant magnetic x-ray scattering has been used to investigate the magnetic structure of the magnetoelectric multiferroic DyMn2O5. We have studied the magnetic structure in the ferroelectric phase of this material, which displays the…

强关联电子 · 物理学 2012-06-08 G. E. Johnstone , R. A. Ewings , R. D. Johnson , C. Mazzoli , H. C. Walker , A. T. Boothroyd

It was recently observed that materials showing most striking multiferroic phenomena are frustrated spin-density-wave magnets. We present a simple phenomenological theory, which describes the orientation of the induced electric polarization…

强关联电子 · 物理学 2009-11-11 Maxim Mostovoy

The structural, electronic and lattice dielectric properties of multiferroic TbMn$_2$O$_5$ are investigated using density functional theory within the generalized gradient approximation (GGA). We use collinear spin approximations and ignore…

材料科学 · 物理学 2009-11-13 Chenjie Wang , Guang-Can Guo , Lixin He

The commensurate and incommensurate magnetic structures of the magnetoelectric system YMn$_{2}$O$_{5}$, as determined from neutron diffraction, were found to be spin-density waves lacking a global center of symmetry. We propose a model,…

材料科学 · 物理学 2009-11-11 L. C. Chapon , P. G. Radaelli , G. R. Blake , S. Park , S-W. Cheong

The magnetic properties of GdBaMn_{2}O_{5.0}, which exhibits charge ordering, are studied from 2 to 400 K using single crystals. In a small magnetic field applied along the easy axis, the magnetization M shows a temperature-induced reversal…

材料科学 · 物理学 2009-11-13 A. A. Taskin , Yoichi Ando

We present the rare existence of d5 off-centering, weak ferroelectric polarization and demonstrate its correlation with observed magnetoelectric (ME) properties in the G type (TN~210 K) antiferromagnet Fe2TeO6 (FTO) compound. The origin of…

We have studied the thermodynamic properties of a multiferroic that couples ferromagnetic and ferroelectric order. Some of the results are independent of the form of the free energy. We calculate the temperature dependence of the electric,…

材料科学 · 物理学 2011-01-31 G. R. Boyd , P. Kumar , S. R. Phillpot