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High-order harmonic generation (HHG) is investigated theoretically in the over-the-barrier ionization (OBI) regime revealing the strong signature of interference between two separately ionized and separately propagating free wave packets of…

We study high-order harmonic generation in aligned molecules close to the ionization threshold. Two distinct contributions to the harmonic signal are observed, which show very different responses to molecular alignment and ellipticity of…

原子物理 · 物理学 2011-09-16 H. Soifer , P. Botheron , D. Shafir , A. Diner , O. Raz , B. D. Bruner , Y. Mairesse , B. Pons , N. Dudovich

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

原子物理 · 物理学 2018-05-18 Peter Mulholland , Daniel Dundas

High harmonic generation (HHG) from semiconductors and insulators has become a very active area of research due to its great potential for developing compact HHG devices. Here we show that by growing monolayers (ML) of insulators on…

原子物理 · 物理学 2016-12-28 Néstor F. Aguirre , Fernando Martín

Electron quantum path interferences in strongly laser-driven aligned molecules and their dependence on the molecular alignment is an essential open problem in strong-field molecular physics. Here, we demonstrate an approach which provides…

We investigate the effect on high-order harmonic generation of the distortion of molecular orbitals by the driving laser field. Calculations for high-order harmonic generation including orbital distortion are performed for N2. Our results…

原子物理 · 物理学 2015-06-15 Maciej Dominik Śpiewanowski , Adam Etches , Lars Bojer Madsen

The generation of high harmonics (HHG) in atomic systems by the highly non-linear response to an intense laser field is a prominent pathway to the synthesis of ever shorter laser pulses at increasingly higher photon energies. Extensions of…

原子物理 · 物理学 2022-11-23 Mohammad Monfared , Elnaz Irani , Christoph Lemell , Joachim Burgdörfer

We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the…

材料科学 · 物理学 2022-08-31 David Freeman , Shunsuke Yamada , Atsushi Yamada , Kazuhiro Yabana , Anatoli Kheifets

We numerically solved the full-dimensional electronic time-dependent Schr\"{o}dinger equation for H$_2^+$ with Born-Oppenheimer approximation under different sin$^2$-shaped and trapezoidal laser pulses at some different wavelengths, with…

原子物理 · 物理学 2018-08-30 Sajad Taghipour , Mohsen Vafaee

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

We develop a numerical scheme to investigate the high-order harmonic generation (HHG) in intense laser-matter interactions. Tracing the time evolution of every electronic laser-field-free state, we "observe" the HHG in a time-integrated…

原子物理 · 物理学 2008-11-14 Y. J. Chen , J. Liu , Bambi Hu

We theoretically investigate photo-excitation of electron-hole pairs and high harmonic generation in the bulk of zinc oxide (ZnO) subjected to intense femto-second laser pulses with mid-infrared wavelength. The main microscopic mechanism of…

光学 · 物理学 2025-07-15 Boyan Obreshkov , Tzveta Apostolova

We theoretically and experimentally investigate orientation-dependent high-harmonic generation (HHG) in zinc oxide subjected to intense femtosecond mid-infrared (MIR) laser pulses. In agreement with past measurements from literature, we…

The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

原子物理 · 物理学 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

We investigate the connection of recently identified fine-scale oscillations in the dependence of the yield of the high-harmonic generation (HHG) on wavelength lambda of a few-cycle laser pulse [K. Schiessl, K.L. Ishikawa, E. Persson, and…

原子物理 · 物理学 2009-01-14 K. L. Ishikawa , K. Schiessl , E. Persson , J. Burgdörfer

The long standing issue of separating resonant from non-resonant processes in extreme nonlinear optics is resolved. The theoretical formalism is applied to high harmonic generation (HHG) in solids and reveals a deeper view into the dominant…

光学 · 物理学 2022-06-03 A. Thorpe , N. Boroumand , A. M. Parks , E. Goulielmakis , T. Brabec

We apply the time-dependent R-matrix method to investigate harmonic generation from Ne(+) at a wavelength of 390 nm and intensities up to 10(15) Wcm(-2). The 1s(2)2s(2)2p(4) (3)P(e), (1)D(e), and (1)S(e) states of Ne(2+) are included as…

原子物理 · 物理学 2014-05-14 O. Hassouneh , A. C. Brown , H. W. van der Hart

We investigate high-order harmonic spectra from aligned diatomic molecules in intense driving fields whose components have orthogonal polarizations. We focus on how the driving-field ellipticity influences structural interference patterns…

The cut-off regime of high-order harmonic generation (HHG) by atoms in an intense laser field is studied numerically and analytically. We find that the cut-off regime is characterized by equal dephasing between the successive harmonics. The…

原子物理 · 物理学 2016-04-27 M. A. Khokhlova , V. V. Strelkov

High-order harmonic generation (HHG) is a powerful tool for probing electronic structure and ultrafast dynamics in matter. Traditionally studied in atomic and molecular gases, HHG has recently been extended to condensed matter, enabling…