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We sympathetically cool a trapped 112Cd+ ion by directly Doppler-cooling a 114Cd+ ion in the same trap. This is the first demonstration of optically addressing a single trapped ion being sympathetically cooled by a different species ion.…

量子物理 · 物理学 2009-11-07 B. B. Blinov , L. Deslauriers , P. Lee , M. J. Madsen , R. Miller , C. Monroe

A mixed system of cooled and trapped, ions and atoms, paves the way for ion assisted cold chemistry and novel many body studies. Due to the different individual trapping mechanisms, trapped atoms are significantly colder than trapped ions,…

原子物理 · 物理学 2012-11-01 K. Ravi , Seunghyun Lee , Arijit Sharma , G. Werth , S. A. Rangwala

We have produced ultracold, polar RbCs* molecules via photoassociation in a laser-cooled mixture of Rb and Cs atoms. Using a model of the RbCs* molecular interaction which reproduces the observed rovibrational structure, we infer decay…

原子物理 · 物理学 2009-11-10 Andrew J. Kerman , Jeremy M. Sage , Sunil Sainis , David DeMille , Thomas Bergeman

We demonstrate broadband laser cooling of atomic ions in an rf trap using ultrafast pulses from a modelocked laser. The temperature of a single ion is measured by observing the size of a time-averaged image of the ion in the known harmonic…

量子物理 · 物理学 2009-11-11 B. B. Blinov , R. N. Kohn , M. J. Madsen , P. Maunz , D. L. Moehring , C. Monroe

We suggest a protocol for the sympathetic cooling of a molecular asymmetric top rotor co-trapped with laser-cooled atomic ions, based on resonant coupling between the molecular ion's electric dipole moment and a common normal mode of the…

量子物理 · 物理学 2026-02-04 Monika Leibscher , Alexander Blech , Christiane P. Koch

We demonstrate optical cycling and sub-Doppler laser cooling of a cryogenic buffer-gas beam of calcium monohydride (CaH) molecules. We measure vibrational branching ratios for laser cooling transitions for both excited electronic states A…

原子物理 · 物理学 2022-08-24 S. F. Vázquez-Carson , Q. Sun , J. Dai , D. Mitra , T. Zelevinsky

We report the generation, trapping and sympathetic cooling of individual conformers of molecular ions with the example of cis- and trans-meta-aminostyrene. Following conformationally selective photoionization, the incorporation of the…

化学物理 · 物理学 2023-08-09 Lei Xu , Jutta Toscano , Stefan Willitsch

State-of-the-art {\em ab initio} techniques have been applied to compute the potential energy curves of the (BaRb)$^+$ molecular ion in the Born-Oppenheimer approximation. The long-range coefficients describing the electrostatic, induction,…

Cooling the rotation and the vibration of molecules by broadband light sources was possible for trapped molecular ions or ultracold molecules. Because of a low power spectral density, the cooling timescale has never fell below than a few…

原子物理 · 物理学 2018-06-06 A. Cournol , P. Pillet , H. Lignier , D. Comparat

We demonstrate the ability to load, cool and detect singly-charged calcium ions in a surface electrode trap using only visible and infrared lasers for the trapped-ion control. As opposed to the standard methods of cooling using…

原子物理 · 物理学 2017-07-27 F. Lindenfelser , M. Marinelli , V. Negnevitsky , S. Ragg , J. P. Home

We report on a cycling scheme for Doppler cooling of trapped OH$^+$ ions using transitions between the electronic ground state $X^3\Sigma^-$ and the first excited triplet state $A^3\Pi$. We have identified relevant transitions for photon…

原子物理 · 物理学 2023-11-20 Niccolò Bigagli , Daniel W. Savin , Sebastian Will

Ultracold LiCs molecules in the absolute ground state X$^1\Sigma^+$, v"=0, J"=0 are formed via a single photo-association step starting from laser-cooled atoms. The selective production of v"=0, J"=2 molecules with a 50-fold higher rate is…

量子物理 · 物理学 2010-08-09 J. Deiglmayr , A. Grochola , M. Repp , K. Mörtlbauer , C. Glück , J. Lange , O. Dulieu , R. Wester , M. Weidemüller

We report direct laser cooling of a symmetric top molecule, reducing the transverse temperature of a beam of calcium monomethoxide (CaOCH$_3$) to $1.8\pm0.7$ mK while addressing two distinct nuclear spin isomers. These results open a path…

Employing a two-stage cryogenic buffer gas cell, we produce a cold, hydrodynamically extracted beam of calcium monohydride molecules with a near effusive velocity distribution. Beam dynamics, thermalization and slowing are studied using…

原子物理 · 物理学 2017-09-13 Hsin-I Lu , Julia Rasmussen , Matthew J. Wright , Dave Patterson , John M. Doyle

The trapped-ion quantum charge-coupled device (QCCD) architecture is a leading candidate for advanced quantum information processing. In current QCCD implementations, imperfect ion transport and anomalous heating can excite ion motion…

Aluminum monochloride (AlCl) has been proposed as a promising candidate for laser cooling to ultracold temperatures, and recent spectroscopy results support this prediction. It is challenging to produce large numbers of AlCl molecules…

While laser excitation of the nuclear isomeric transition in $^{229}$Th has been recently achieved for thorium atoms embedded in large-bandgap crystals, laser excitation and characterization of the nuclear transition in trapped…

We use electromagnetically induced transparency (EIT) laser cooling to cool motional modes of a linear ion chain. As a demonstration, we apply EIT cooling on $^{24}Mg^+$ ions to cool the axial modes of a $^9Be^+$ - $^{24}Mg^+$ ion pair and…

原子物理 · 物理学 2014-01-27 Y. Lin , J. P. Gaebler , T. R. Tan , R. Bowler , J. D. Jost , D. Leibfried , D. J. Wineland

Cold molecular ions are promising candidates in various fields ranging from precision spectroscopy and test of fundamental physics to ultra-cold chemistry. Control of internal and external degrees of freedom is a prerequisite for many of…

量子物理 · 物理学 2015-05-06 Yong Wan , Florian Gebert , Fabian Wolf , Piet O. Schmidt

We present a rigorous theoretical study of low-temperature collisions of polyatomic molecular radicals with ^1S_0 atoms in the presence of an external magnetic field. Accurate quantum scattering calculations based on ab initio and scaled…

原子物理 · 物理学 2011-03-07 T. V. Tscherbul , H-G. Yu , A. Dalgarno