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The molecular triangular lattice system, beta'-EtMe3Sb[Pd(dmit)2]2, is considered as a candidate material for the quantum spin liquid (QSL) state, although ongoing debates arise from recent controversial results. Here, the results of…

Magnetic structures of organic Mott insulators X[Pd(dmit)2]2 (X=Me4P, Me4Sb), of which electronic states are located near quantum spin liquid (X=EtMe3Sb), are demonstrated by 13C NMR. Antiferromagnetic spectra and nuclear relaxations show…

强关联电子 · 物理学 2019-05-01 Shigeki Fujiyama , Reizo Kato

Mott insulators with localized magnetic moments will exhibit a quantum spin liquid (QSL) state when the quantum fluctuations are strong enough to suppress the ordering of the spins. Such an entangled state will give rise to collective…

Organic charge transfer salts based on the molecule Pd(dmit)2 display strong electronic correlations and geometrical frustration, leading to spin liquid, valence bond solid, and superconducting states, amongst other interesting phases. The…

强关联电子 · 物理学 2013-11-15 A. C. Jacko , Luca F. Tocchio , Harald O. Jeschke , Roser Valenti

The electrodynamic response of organic spin liquids with highly-frustrated triangular lattices has been measured in a wide energy range. While the overall optical spectra of these Mott insulators are governed by transitions between the…

强关联电子 · 物理学 2018-08-09 A. Pustogow , Y. Saito , E. Zhukova , B. Gorshunov , R. Kato , T. -H. Lee , S. Fratini , V. Dobrosavljević , M. Dressel

Quantum spin liquids attract great interest due to their exceptional magnetic properties characterized by the absence of long-range order down to low temperatures despite the strong magnetic interaction. Commonly, these compounds are…

强关联电子 · 物理学 2018-05-01 Martin Dressel , Andrej Pustogow

Organic solids host various electronic phases. Especially, a milestone compound of organic solid, $\beta'$-$X$[Pd(dmit)$_2$]$_2$ with $X$=EtMe$_3$Sb shows quantum spin-liquid (QSL) properties suggesting a novel state of matter. However,…

强关联电子 · 物理学 2022-04-29 Kota Ido , Kazuyoshi Yoshimi , Takahiro Misawa , Masatoshi Imada

A molecular Mott insulator $\beta$'-EtMe$_3$Sb[Pd(dmit)$_2$]$_2$ is a quantum spin liquid candidate. In 2010, it was reported that thermal conductivity of $\beta$'-EtMe$_3$Sb[Pd(dmit)$_2$]$_2$ is characterized by its large value and gapless…

强关联电子 · 物理学 2022-01-19 Reizo Kato , Masashi Uebe , Shigeki Fujiyama , Hengbo Cui

For certain crystalline systems, most notably the organic compound EtMe3Sb[Pd(dmit)2]2, experimental evidence has accumulated of an insulating state with a high density of gapless neutral excitations that produce Fermi-liquid-like power…

强关联电子 · 物理学 2013-04-09 Maissam Barkeshli , Hong Yao , Steven A. Kivelson

EtMe$_3$Sb[Pd(dmit)$_2$]$_2$, an organic Mott insulator with nearly isotropic triangular lattice, is a candidate material for a quantum spin liquid, in which the zero-point fluctuations do not allow the spins to order. The itinerant gapless…

强关联电子 · 物理学 2020-04-29 M. Yamashita , Y. Sato , T. Tominaga , Y. Kasahara , S. Kasahara , H. Cui , R. Kato , T. Shibauchi , Y. Matsuda

Novel phases of two dimensional electron systems resulting from new surface or interface modified electronic structures have generated significant interest in material science. We utilize photoemission spectroscopy to show that the…

Experimental quest for the hypothetical "quantum spin liquid" state has recently met a few promising candidate materials including organic salts \kappa-(ET)2Cu2(CN)3 and EtMe3Sb[Pd(dmit)2]2, S=1/2 triangular-lattice Heisenberg…

强关联电子 · 物理学 2015-06-17 Ken Watanabe , Hikaru Kawamura , Hiroki Nakano , Toru Sakai

We consider an electronic model for realizing the Spin Bose-metal (SBM) phase on a 2-leg triangular strip --a spin liquid phase found by D. N. Sheng et al [Phys. Rev. B {\bf 79}, 205112 (2009)] in a spin-1/2 model with ring exchanges. The…

强关联电子 · 物理学 2010-06-09 Hsin-Hua Lai , Olexei I. Motrunich

Recently, $\alpha$-$\textrm{RuCl}_3$ has attracted much attention as a possible material realization of the honeycomb Kitaev model, which may stabilize a quantum-spin-liquid state. Compared to extensive studies on its magnetic properties,…

Recently, there has been a growing interest in altermagnetism, a novel form of magnetism, characterized by unique spin-splitting even in the absence of both net magnetic moments and spin-orbit coupling. Despite numerous theoretical…

The mixed-valent iridate Ba3InIr2O9 has been discussed as a promising candidate for quantum spin-liquid behavior. The compound exhibits Ir$^{4.5+}$ ions in face-sharing IrO6 octahedra forming Ir2O9 dimers with three t2g holes per dimer. Our…

We report electronic band structure calculations for Sr$_{4}$Ru$_{3}$O$_{10}$ that displays both ferromagnetic and metamagnetic behavior. The density functional calculations find the ground state to be ferromagnetic in agreement with the…

The compound UTe2 has recently been shown to realize spin triplet superconductivity from a non-magnetic normal state. This has sparked intense research activity, including theoretical analyses that suggest the superconducting order…

Systematic pressure- and temperature-dependent infrared studies on the two-dimensional organic quantum spin-liquid $\beta^{\prime}$-EtMe$_3$Sb[Pd(dmit)$_2$]$_2$ disclose the electronic and lattice evolution across the Mott insulator-metal…

强关联电子 · 物理学 2019-03-27 Weiwu Li , Andrej Pustogow , Reizo Kato , Martin Dressel

Two-dimensional triangular-lattice antiferromagnets are predicted under some conditions to exhibit a quantum spin liquid ground state whose low-energy behavior is described by a spinon Fermi surface. Directly imaging the resulting spinons,…

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