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Continuous hydrothermal flow synthesis (CHFS) is a facile, upscalable and cost-efficient synthetic method enabling the nanostructuring of advanced functional materials in steady conditions, i.e. not in batch synthesis. In this paper, we use…

The effect of Fe and Ni catalysts on the synthesis of carbon nanotubes (CNTs) using atmospheric pressure chemical vapor deposition (APCVD) was investigated. Field emission scanning electron microscopy (FESEM) analysis suggests that the…

材料科学 · 物理学 2019-08-02 J. Sengupta , C. Jacob

The assembly of aligned carbon nanotubes (CNT) into fibers (CNTF) is a convenient approach to exploit and apply the unique physico-chemical properties of CNTs in many fields. CNT functionalization has been extensively used for their…

The ability to efficiently evolve hydrogen via electrocatalysis at low overpotentials holds tremendous promise for clean energy. Hydrogen evolution reaction (HER) can be easily achieved from water if a voltage above the thermodynamic…

The interactions of charged particles with carbon nanotubes may excite electromagnetic modes in the electron gas produced in the cylindrical graphene shell constituting the nanotube wall. This wake effect has recently been proposed as a…

加速器物理 · 物理学 2023-12-18 P. Martín-Luna , A. Bonatto , C. Bontoiu , G. Xia , J. Resta-López

Two-dimensional (2D) heterostructuring is a versatile methodology for designing nanoarchitecture catalytic systems that allow for reconstruction and modulation of interfaces and electronic structures. However, catalysts with such structures…

The oxygen reduction (ORR) and oxygen evolution reactions (OER) in Zn-air batteries (ZABs) require highly efficient, cost-effective and stable electrocatalysts as replacements to traditionally high cost, inconsistently stable and low poison…

应用物理 · 物理学 2018-02-07 Wenhan Niu , Srimanta Pakhira , Kyle Marcus , Zhao Li , Jose L. Mendoza-Cortes , Yang Yang

A parametric study of so-called "super growth" of single-walled carbon nanotubes(SWNTs) was done by using combinatorial libraries of iron/aluminum oxide catalysts. Millimeter-thick forests of nanotubes grew within 10 min, and those grown by…

材料科学 · 物理学 2009-11-13 S. Noda , K. Hasegawa , H. Sugime , K. Kakehi , Z. Zhang , S. Maruyama , Y. Yamaguchi

In this work we describe the synthesis and electrochemical properties of nitridated hierarchical TiO$_2$ nanotubes as an electrode for supercapacitors. The hierarchical TiO$_2$ nanostructures are formed by a controlled layer-by-layer TiO2…

化学物理 · 物理学 2020-04-28 Nhat Truong Nguyen , Selda Ozkan , Imgon Hwang , Xuemei Zhou , Patrik Schmuki

Water electrolysis is promising for industrial hydrogen production to achieve a sustainable and green hydrogen economy, but the high cost of the technology limits its market share. Developing efficient yet economic electrocatalysts is…

This study introduces the high yield, electrolytic synthesis of carbon nanofibers, CNFs, directly from carbon dioxide. Production of a precious commodity such as CNFs from atmospheric carbon dioxide provides impetus to limit this greenhouse…

化学物理 · 物理学 2015-10-28 Stuart Licht

Finding proper electrocatalysts capable of efficient catalyzing both ORR and OER is of great importance for metal-air batteries. With increasing inclination towards structural and flexible devices, developing a high-performance…

材料科学 · 物理学 2019-02-01 Afshin Pendashteh , Jesus Palma , Marc Anderson , Juan J. Vilatela , Rebeca Marcilla

Electrocatalytic hydrogenation of nitrobenzene (Ph-NO2) reaction (EHNR) has been considered as a potential alternative to the traditional thermocatalytic process in the production of high-value aniline (Ph-NH2). However, due to the absence…

化学物理 · 物理学 2024-03-26 Yuchen Wang , Yaoyu Liu , Zhiyue Zhao , Zhikeng Zheng , Alina M. Balu , Rafael Luque , Kai Yan

Downsizing well-established materials to the nanoscale is a key route to novel functionalities, in particular if different functionalities are merged in hybrid nanomaterials. Hybrid carbon-based hierarchical nanostructures are particularly…

As renewable energy is becoming a critical energy source to meet the global demand, electrochemical energy storage devices become indispensable for the efficient energy storage and reliable supply. The electrode material is the key factor…

However, their electrocatalytic activity is still poorly understood. This work deciphers the origin of the catalytic activity of counter-electrodes (CEs)/current collectors made of self-standing carbon nanotubes fibers (CNTfs) using…

应用物理 · 物理学 2021-07-28 Alba Martínez-Muíño , Moumita Rana , Juan J. Vilatela , Rubén D. Costa

Nanoporous carbon materials containing small domains of sp2-carbon with highly disordered structures are promising for supercapacitor applications. Herein, we synthesize amorphous carbon nanofoam with 98% volumetric void fraction and low…

In the present work we grow self-organized Ta2O5 nanotube layers in a H2SO4/NH4F electrolyte at various elevated temperatures. Under optimized conditions we obtain 4 {\mu}m long nanotubes that are well adherent to the substrate and can be…

材料科学 · 物理学 2016-10-18 Sabina Grigorescu , Seulgi So , Jeong Eun Yoo , Anca Mazare , Robert Hahn , Patrik Schmuki

Many ligands commonly used to prepare nanoparticle catalysts with precise nanoscale features contain nitrogen (e.g., oleylamine); here, we found that the use of nitrogen-containing ligands during the synthesis of metal oxide nanoparticle…

Surfaces of metal oxides at working conditions are usually electrified due to the acid-base chemistry. The charged interface compensated with counterions forms the so-called electric double layer. The coupling of surface chemistry and…

软凝聚态物质 · 物理学 2019-07-02 Chao Zhang , Jürg Hutter , Michiel Sprik