相关论文: Vibrational spectroscopy of polar molecules with s…
When atoms are coupled to a common electromagnetic environment, the exchange of photons through dipole-dipole interactions leads to the emergence of cooperative effects. As a particular example, superradiance arises from spontaneous…
We have produced ultracold, polar RbCs* molecules via photoassociation in a laser-cooled mixture of Rb and Cs atoms. Using a model of the RbCs* molecular interaction which reproduces the observed rovibrational structure, we infer decay…
We study the collective behavior of molecules placed in an infrared (IR) microcavity, incorporating the local fluctuations, i.e., dynamical disorder. The cooperative feature in vibrational polaritons is shown to be dynamically eroded, due…
We calculate the microwave spectra of ultracold KRb alkali metal dimers, including hyperfine interactions and in the presence of electric and magnetic fields. We show that microwave transitions may be used to transfer molecules between…
We present theoretical results for superradiance, i.e. the collective coherent decay of a radiating system, in semiconductor structures. An optically active region can become superradiant if a strong magnetic field is applied. Pumping of…
In the present work, we analyze the influence of the polarization effects taking place during the course of a 2DIR spectroscopy experiment performed on a molecular system undergoing an intermolecular vibrational energy transfer process.…
We describe the theoretical advances that influenced the experimental creation of vibrationally and translationally cold polar $^{40}$K$^{87}$Rb molecules \cite{nphys08,science08}. Cold molecules were created from very-weakly bound…
We present a rigorous study of vibrational relaxation in p-H2 + p-H2 collisions at cold and ultracold temperatures and identify an efficient mechanism of ro-vibrational energy transfer. If the colliding molecules are in different rotational…
We have developed a novel method to describe superradiance and related cooperative and collective effects in a closed form. Using the method we derive a two-atom master equation in which any complexity of atomic levels, semiclassical…
We study the influence of cooperative effects such as superradiance and subradiance, on the scattering properties of dilute atomic gases. We show that cooperative effects lead to an effective potential between pairs of atoms that decays…
The Dicke superradiance on vibronic transitions of impurity crystals is considered. It is shown that parameters of the superradiance (duration and intensity of the superradiance pulse and delay times) on each vibronic transition depend on…
Microscopic control over polar molecules with tunable interactions would enable realization of novel quantum phenomena. Using an applied electric field gradient, we demonstrate layer-resolved state preparation and imaging of ultracold…
We present a method to design a finite decay rate for excited rotational states in polar molecules. The setup is based on a hybrid system of polar molecules with atoms driven into a Rydberg state. The atoms and molecules are coupled via the…
We show that the electric dipole-dipole interaction between a pair of polar molecules undergoes an all-out transformation when superimposed by a far-off resonant optical field. The combined interaction potential becomes tunable by variation…
Vibrational polaritons are formed by strong coupling of molecular vibrations and photon modes in an optical cavity. Experiments have demonstrated that vibrational strong coupling can change molecular properties and even affect chemical…
Dipole-coupled subwavelength quantum emitter arrays respond cooperatively to external light fields as they may host collective delocalized excitations (a form of excitons) with super- or subradiant character. Deeply subwavelength…
Atomic ensembles strongly interacting with light constitute rich quantum-optical many-body systems, with the potential for observing cooperative effects and dissipative nonequilibrium phase transitions. We theoretically analyze the…
We theoretically study collisions between ultracold polar molecules that are polarized by microwave or static electric fields. We systematically study the dependence on field strength, microwave polarization, and detuning from rotational…
The dipolar collision between ultracold polar molecules is an important topic both by its own right from the fundamental point of view and for the successful exploration of many-body physics with strong and long-range dipolar interactions.…
We study the superradiance dynamics in a dense system of atoms each of which can be generally a spin-$j$ particle with $j$ an arbitrary half-integer. We generalize Dicke's superradiance point of view to multiple-level systems, and compare…