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We develop a theoretical framework for probing moir\'e phonon modes using Raman spectroscopy, and illustrate it with the example of twisted bilayer graphene (TBG). These moir\'e phonons arise from interlayer sliding motion in twisted 2D…

强关联电子 · 物理学 2025-06-24 Vitor Dantas , Héctor Ochoa , Rafael M. Fernandes , Natalia B. Perkins

Twisted bilayer graphene (tBLG) provides us with a large rotational freedom to explore new physics and novel device applications, but many of its basic properties remain unresolved. Here we report the synthesis and systematic Raman study of…

We theoretically investigated phonon dispersion in AA-stacked, AB-stacked and twisted bilayer graphene with various rotation angles. The calculations were performed using the Born-von-Karman model for the intra-layer atomic interactions and…

介观与纳米尺度物理 · 物理学 2013-07-19 Alexandr I. Cocemasov , Denis L. Nika , Alexander A. Balandin

Twisted 2D layered materials have garnered a lot of attention recently as a class of 2D materials whose interlayer interactions and electronic properties are dictated by the relative rotation / twist angle between the adjacent layers. In…

We present an analysis of deep-UV Raman measurements of graphite, graphene and carbon nanotubes. For excitation energies above the strong optical absorption peak at the $M$ point in the Brillouin zone ($\approx 4.7\,\text{eV}$), we…

材料科学 · 物理学 2015-08-03 Christoph Tyborski , Felix Herziger , Roland Gillen , Janina Maultzsch

Twisted bilayer graphene (tBLG) devices with ion gel gate dielectrics are studied using Raman spectroscopy in the twist angle regime where a resonantly enhanced G band can be observed. We observe prominent splitting and intensity quenching…

介观与纳米尺度物理 · 物理学 2015-02-18 Ting-Fung Chung , Rui He , Tai-Lung Wu , Yong P. Chen

Twisted bilayer graphene (tBLG) has recently emerged as a platform for hosting correlated phenomena, owing to the exceptionally flat band dispersion that results near interlayer twist angle $\theta\approx1.1^\circ$. At low temperature a…

强关联电子 · 物理学 2019-10-03 H. Polshyn , M. Yankowitz , S. Chen , Y. Zhang , K. Watanabe , T. Taniguchi , C. R. Dean , A. F. Young

We study electronic contribution to the Raman scattering signals of two-, three- and four-layer graphene with layers at one of the interfaces twisted by a small angle with respect to each other. We find that the Raman spectra of these…

介观与纳米尺度物理 · 物理学 2020-11-11 A. Garcia-Ruiz , J. J. P. Thompson , M. Mucha-Kruczynski , V. I. Fal'ko

We report multiphonon Raman scattering in graphene samples. Higher order combination modes involving 3 phonons and 4 phonons are observed in single-layer (SLG), bi-layer (BLG), and few layer (FLG) graphene samples prepared by mechanical…

介观与纳米尺度物理 · 物理学 2015-05-30 Rahul Rao , Derek Tishler , Jyoti Katoch , Masa Ishigami

Twisted-bilayer graphene (tBLG) exhibits van Hove singularities in the density of states that can be tuned by changing the twisting angle $\theta$. A $\theta$-defined tBLG has been produced and characterized with optical reflectivity and…

介观与纳米尺度物理 · 物理学 2015-06-22 Ado Jorio , Mark Kasperczyk , Nick Clark , Elke Neu , Patrick Maletinsky , Aravind Vijayaraghavan , Lukas Novotny

In stacks of two-dimensional crystals, mismatch of their lattice constants and misalignment of crystallographic axes lead to formation of moir\'{e} patterns. We show that moir\'{e} superlattice effects persist in twisted bilayer graphene…

In this work we study the symmetry properties of electrons and phonons in graphene systems as function of the number of layers. We derive the selection rules for the electron-radiation and for the electron-phonon interactions at all points…

介观与纳米尺度物理 · 物理学 2013-06-20 L. M. Malard , D. L. Mafra , M. H. D. Guimarães , M. S. C. Mazzoni , A. Jorio

Moir\'e superlattices can induce correlated-electronic phases in twisted van-der-Waals materials. Strongly correlated quantum phenomena emerge, such as superconductivity and the Mott-insulating state. However, moir\'e superlattices produced…

The dispersion of phonons and the electronic structure of graphene systems can be obtained experimentally from the double-resonance (DR) Raman features by varying the excitation laser energy. In a previous resonance Raman investigation of…

介观与纳米尺度物理 · 物理学 2011-03-10 D. L. Mafra , E. A. Moujaes , R. W. Nunes , M. A. Pimenta

We theoretically study in-plane acoustic phonons of graphene/hexagonal boron nitride moir\'e superlattice by using a continuum model. We demonstrate that the original phonon bands of individual layers are strongly hybridized and…

介观与纳米尺度物理 · 物理学 2023-03-03 Lukas P. A. Krisna , Mikito Koshino

Hybridisation of electronic bands of two-dimensional materials, assembled into twistronic heterostructures, enables one to tune their optoelectronic properties by selecting conditions for resonant interlayer hybridisation. Resonant…

We show how the magneto-phonon resonance, particularly pronounced in sp2 carbon allotropes, can be used as a tool to probe the band structure of multilayer graphene specimens. Even when electronic excitations cannot be directly observed,…

介观与纳米尺度物理 · 物理学 2012-09-11 C. Faugeras , P Kossacki , A. A. L. Nicolet , M. Orlita , M Potemski , A. Mahmood , D. M. Basko

The phonon spectra of twisted bilayer graphene (tBLG) are analyzed for a series of 692 twisting angle values in the $[0,30{\degree}]$ range. The evolution of the phonon bandstructure as a function of twist angle is examined using a band…

介观与纳米尺度物理 · 物理学 2020-01-01 Michael Lamparski , Benoit Van Troeye , Vincent Meunier

We present a computational study of the two-phonon Raman spectra of silicene and graphene within a density-functional non-orthogonal tight-binding model. Due to the presence of linear bands close to the Fermi energy in the electronic…

介观与纳米尺度物理 · 物理学 2016-04-29 Valentin N. Popov , Philippe Lambin

In twisted bilayer graphene, long-wavelength lattice fluctuations on the scale of the moir\'e period are dominated by phason modes, i.e., acoustic branches of the incommensurate lattice resulting from coherent superpositions of optical…

介观与纳米尺度物理 · 物理学 2019-10-30 Héctor Ochoa
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